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Visualized oxygen sensing detection biosensor preparation method

A biosensor and oxygen sensing technology, applied in the field of biosensors, can solve the problems of low sensitivity of colorimetric oxygen sensors, and achieve high resolution, high sensitivity, and good stability

Inactive Publication Date: 2008-10-15
XIAMEN UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0003] The purpose of the present invention is to provide a low cost, high sensitivity, good resolution, high accuracy and other characteristics for the existing colorimetric oxygen sensor with low sensitivity and relatively limited detection range, which can realize the treatment Preparation method of biosensor for visual oxygen sensing and detection of visualized and rapid determination of analytes

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0017] Mix TEOS, APTMS, ultrapure water and methanol at a volume ratio of 1:8.8:20:101.3, take 13.10 mL into a polytetrafluoroethylene beaker, stir at room temperature for 1 hour; seal the polytetrafluoroethylene beaker with parafilm , perforate a few small holes on the sealing film to facilitate the volatilization of methanol, place the polytetrafluoroethylene beaker in a 30°C incubator for 48h; then add 1mL of 2×10 -3 mol / L green quantum dot solution and 0.3mL Cd precursor solution (CdCl 2 Mix with thioglycolic acid at a molar ratio of 1:2.4 and dilute with ultrapure water to a concentration of 2×10 -3 mol / L, use 1.0mol / L NaOH to adjust the pH of the solution to 9 to obtain the Cd precursor solution), put the mixed solution in a 30°C incubator and store it in the dark for 4h, then take 40μL on a glass slide (48×12.4×0.9 , mm) was uniformly coated on the film, and placed in a 30°C incubator to avoid light and dry to obtain a quantum dot layer with stable luminescence.

[00...

Embodiment 2

[0020] Mix TEOS, APTMS, ultrapure water and methanol at a volume ratio of 1:8.8:20:101.3, take 13.10 mL into a polytetrafluoroethylene beaker, stir at room temperature for 1 hour; seal the polytetrafluoroethylene beaker with parafilm , perforate a few small holes on the sealing film to facilitate the volatilization of methanol, place the polytetrafluoroethylene beaker in a 30°C incubator for 48h; then add 1mL of 2×10 -5 mol / L green quantum dot solution and 0.3mL Cd precursor solution (CdCl 2 Mix with thioglycolic acid at a molar ratio of 1:2.4 and dilute with ultrapure water to a concentration of 2×10 -5 mol / L, use 1.0mol / L NaOH to adjust the pH of the solution to 10 to obtain the Cd precursor solution), put the mixed solution in a 30°C incubator and store it in the dark for 4h, then take 60μL on a glass slide (48×12.4×0.9, mm) evenly, and placed in a 30°C incubator to avoid light and dry to obtain a quantum dot layer with stable luminescence.

[0021] Measure TMOS and DiMe-...

Embodiment 3

[0024] Mix TEOS, APTMS, ultrapure water and methanol at a volume ratio of 1:8.8:20:101.3, take 13.10 mL into a polytetrafluoroethylene beaker, stir at room temperature for 1 hour; seal the polytetrafluoroethylene beaker with parafilm , perforate a few small holes on the sealing film to facilitate the volatilization of methanol, place the polytetrafluoroethylene beaker in a 30°C incubator for 48h; then add 1mL of 5×10 -4 mol / L green quantum dot solution and 0.3mL Cd precursor solution (CdCl 2 Mix with thioglycolic acid at a molar ratio of 1:2.4 and dilute with ultrapure water to a concentration of 5×10 -4mol / L, using 1.0mol / L NaOH to adjust the pH of the solution to 11 to obtain the Cd precursor solution), put the mixed solution in a 30°C incubator and store it in the dark for 4h, then take 50μL on a glass slide (48×12.4×0.9 , mm) was uniformly coated on the film, placed in a 30°C incubator and dried in the dark to obtain a quantum dot layer with stable luminescence.

[0025]...

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PUM

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Abstract

The invention discloses a method for preparing a biosensor for visual oxygen sense detection, relating to a biosensor. The invention provides the method for preparing the biosensor for visual oxygen sense detection which is characterized by low cost, high sensibility, good resolution, high accuracy and so on, comprising the following steps that: tetraethoxy-silicane, 3- aminopropyl- trimethoxy silane, ultrapure water and methanol are uniformly mixed; green quantum-dot solution and Cd precursor solution are added and a quantum-dot layer with stable luminescence is obtained by film coating on a glass sheet; oxygen radix silane and dimethyl dimethoxy silane are added into HCl for heating; lower layer gel solution is taken off to be mixed with tetrahydrofuran solution of PtF<20>TPP and then the mixture is coated on the quantum-dot layer for film forming; TMOS and DiMe-DMOS are uniformly mixed; HCl water solution is added and the lower layer gel solution is left after hydrolysis; polyvinyl alcohol water solution and the gel solution are mixed; supernatant liquid is taken to be mixed with phosphate buffer solution which is dissolved with microorganisms or enzymes, and uniform film-coating forming is performed on the surface of an oxygen sensing layer.

Description

technical field [0001] The invention relates to a biosensor, in particular to a preparation method of a biosensor for visual oxygen sensing and detection. Background technique [0002] Oxygen sensors are widely used in oceanography, meteorology, biology, environmental science and life science and other fields. At present, most oxygen sensors are based on pressure, electrochemistry, and photochemistry to achieve quantitative oxygen content measurement. The measurement process requires the assistance of large-scale scientific instruments, cumbersome and complicated data acquisition and processing processes, not only the detection cost is high, but also requires professional expertise. technical personnel, limiting the application of such sensors in real-time online detection and daily life. Evans et al. (Anal.Chem.2006, 78, 5645-5652; Journal of Fluorescence.2006, 16, 201-206) have reported the research work of using colorimetric method to detect oxygen content. Rapid visual...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): G01N21/76G01N33/48C12Q1/00
Inventor 陈曦王旭东陈海旭王小茹
Owner XIAMEN UNIV