Lithium-embedded electrode material, preparation method thereof, electrode, and battery
A lithium electrode and electrode technology, applied in the field of batteries, can solve problems such as potential safety hazards and poor industrial implementation, and achieve the effects of enhancing selectivity, increasing available lithium ions, and reducing irreversible capacity
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[0025] A method for preparing a lithium intercalation electrode material, comprising the following steps: rolling a carrier film with stabilized lithium metal powder onto the lithium electrode material to be intercalated, and then contacting the lithium electrode material to be intercalated with an electrolyte to stabilize the metal Lithium powder and the lithium electrode material to be intercalated constitute a micro-battery discharge.
[0026] Among them, the stabilized lithium metal powder (English: stabilized lithium powder, SLMP for short) is a product well known to those skilled in the art, which can be prepared by yourself or purchased from a store.
[0027] Stabilized metal lithium powder means that a passivation layer or a protective layer is attached to the surface of the metal lithium powder. The passivation layer or protective layer isolates the internal metal lithium powder from oxygen or moisture and reduces the activity of the metal lithium powder. Stabilized l...
Embodiment approach
[0061] In a preferred embodiment, the electrolytic solution of the present invention is an electrolytic solution used in lithium-ion batteries.
[0062] Among them, the contact method of the lithium electrode material to be intercalated and the electrolyte can be soaking the rolled lithium electrode material to be inserted in the electrolyte, or adding the electrolyte dropwise to the rolled lithium electrode material to be inserted. , so that the electrolyte fully infiltrates the rolled lithium electrode material to be intercalated.
[0063] Preferably, the contact time between the lithium electrode material to be intercalated and the electrolyte is 4 to 20 hours, which can ensure that the metal lithium and the lithium electrode material to be intercalated fully react, so that all lithium metal is converted into lithium ions and intercalated into the lithium electrode material to be intercalated to go.
[0064] More preferably, the electrolyte contact time is 12 hours.
[00...
Embodiment 1
[0082] Carrier film with stabilized lithium metal powder: the areal density of the stabilized lithium metal powder is 0.4mg / cm 2 , the carrier film is polypropylene InteTopp TM AA type film, area 50cm 2 .
[0083] Lithium electrode material to be intercalated: 50cm 2 Graphite flakes (weight 255mg).
[0084] Electrolyte: 1mol / L LiPF 6 / EC+DEC(1:1).
[0085] In a dry workshop with a water content lower than 50ppm, the carrier film with stabilized lithium metal powder and the lithium electrode material to be intercalated are placed on a rolling press for 10 7 Rolling under Pa, the stabilized metal lithium powder is transferred to the lithium electrode material to be intercalated, and then the carrier film is removed. The rolled lithium electrode material to be intercalated is then immersed in the electrolyte for 12 hours, and then dried to remove the electrolyte.
[0086] The obtained lithium intercalation electrode material is denoted as A1.
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