A kind of triazolopyrimidine compound and its synthesis and application
An azolopyrimidine and compound technology, which is applied in the field of triazolopyrimidine compounds to achieve the effect of excellent prevention effect
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[0030] The present invention also provides a preparation method for the compound represented by the formula (1), which may include: hydrolyzing the compound represented by the formula (4) in a mixed aqueous solution of sulfuric acid and acetic acid, and the hydrolysis reaction makes the compound represented by the formula (4) The-COOC 2 h 5 The group is converted into a -COOH group;
[0031]
[0032] In formula (4), R 1 , R 2 , R 3 , R 4 and R 5 The groups represented respectively are the same as R in the formula (1) 1 , R 2 , R 3 , R 4 and R 5 The groups represented are the same.
[0033] Wherein, the conditions of the hydrolysis reaction may include: contacting the compound of the structure shown in formula (4) with a mixed aqueous solution of sulfuric acid and acetic acid, based on 1 mol of the compound of the structure shown in formula (4), the amount of the mixed aqueous solution It is 2-15ml, preferably, the consumption of described mixed aqueous solution ...
Embodiment 1-34
[0084] Examples 1-34 are used to illustrate the preparation method of the triazolopyrimidine compounds of the present invention.
[0085] (I): Synthesis of compounds with structures shown in formula (4):
[0086]
[0087] 0.1 mol of the compound shown in the formula (2) (that is, in the structure shown in the formula (2), R 4 and R 5 The represented group is the same as the group specifically listed in Table 1) was dissolved in 20ml toluene to obtain a solution, and the solution was contacted and reacted with sodium hydride according to the conditions listed in Table 2 under the condition of an ice-water bath, and after 60 minutes of reaction Make this reaction mixture respectively with the compound of structure shown in formula (3) (that is, in the structure shown in described formula (3), R 1 , R 2 and R 3 Represented group is the same as the group specifically enumerated in table 1), and carries out reflux reaction according to the reaction conditions listed in table...
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