Hetero-atom doped titanium composite material, and preparation method and application thereof
A composite material and heteroatom technology, applied in the field of inorganic functional materials, can solve the problems of supercapacitor application reports and scientific research, the performance is not very good, the specific capacitance is not very high, etc., to achieve huge application potential and industrial value, excellent electrical performance effect
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Embodiment 1
[0053] S1: Hexachloro-1,3-butadiene, elemental titanium and pyridine were subjected to a closed reaction at a reaction pressure of 3MPa and 200°C for 6 hours;
[0054] Wherein, the mass ratio of the hexachloro-1,3-butadiene to elemental titanium is 1:2, and the molar ratio of hexachloro-1,3-butadiene to pyridine is 30:0.1;
[0055] S2: After the reaction, the pressure was released to normal pressure, and naturally cooled to room temperature, the obtained solid was fully washed 3 times with deionized water, and vacuum-dried at 80°C for 10 hours to obtain a dry sample;
[0056] S3: The dried sample was treated at a high temperature of 350° C. for 2 hours under nitrogen protection to obtain the heteroatom-doped titanium composite material, which was named CL1.
Embodiment 2-7
[0057] Embodiment 2-7: the investigation of reaction temperature in step S1
[0058] Except that the reaction temperature in step S1 was replaced by 180°C, 220°C, 160°C, 240°C, 140°C, and 260°C, the other operations were all the same, so that the examples 2-7 were carried out in sequence, and the obtained complex Atom-doped titanium composites were named CL2, CL3, CL4, CL5, CL6 and CL7 in sequence.
Embodiment 8-13
[0059] Embodiment 8-13: the investigation of high temperature treatment temperature in step S3
[0060] Except that the high-temperature treatment temperature in step S3 was replaced by 300°C, 400°C, 250°C, 450°C, 200°C, and 500°C, the other operations were all unchanged, so that Examples 8-13 were carried out in sequence, and the obtained The heteroatom-doped titanium composites were named CL8, CL9, CL10, CL11, CL12 and CL13 in sequence.
[0061] Preparation of capacitor electrodes
[0062] The preparation method of the capacitor electrode comprises the following steps:
[0063] (A) Weigh the heteroatom-doped titanium composite material CL1, acetylene black, and PTFE (polytetrafluoroethylene) emulsion (the mass ratio of the three is 80:10:10), add an appropriate amount of ethanol, mix well, and keep stirring to form a paste When it is in shape, apply it to the foamed nickel;
[0064] (B) drying, drying, and pressing the nickel foam coated with the heteroatom-doped titanium...
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