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A kind of preparation method of filling modified polyurethane film

A polyurethane membrane and modification technology, applied in separation methods, chemical instruments and methods, membrane technology, etc., can solve problems such as reducing permeation flux

Inactive Publication Date: 2019-06-25
BEIJING TECHNOLOGY AND BUSINESS UNIVERSITY
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, in practical applications, it is difficult for a single polymer membrane material to have both high permeation flux and target component selectivity, that is, the separation factor of pervaporation membranes with high permeation flux is generally low, and it is necessary to improve Its separation factor must be at the expense of reducing its permeate flux

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0015] 1) Preparation of porous silicon-manganese composite particles

[0016] (1) Weigh 2.00g solid KMnO 4 powder and 0.36 g solid MnSO 4 ·H 2 O, respectively dissolved in 60mL deionized water, mechanically stirred until completely dissolved, to obtain solution A; solution A was transferred to a hydrothermal kettle, and the hydrothermal kettle was kept at 160°C for 24 hours, and then filtered, washed, and dried. 1.5g black δ-MnO was obtained 2 solid;

[0017] (2) The resulting δ-MnO 2 Disperse in 60mL of deionized water containing 0.5% (mass content) surfactant CTAB, and ultrasonicate for 20 minutes to obtain suspension B; weigh 0.81g of solid NaSiO 3 9H 2 O, dissolved in 60mL of water to obtain solution C; then put suspension B in a water bath at 80°C, add dropwise solution C to suspension B under stirring, and obtain cloudy solution D after the addition; Transfer to a 200mL hydrothermal kettle with a Teflon liner, put the hydrothermal kettle into a blast drying oven,...

Embodiment 2

[0022] 1) Preparation of porous silicon-manganese composite particles

[0023] Weigh 4.00g solid KMnO 4 powder and 0.73 g solid MnSO 4 ·H 2 O, was added to 80mL of 0.5% CTAB aqueous solution with a mass concentration of 0.5%, and mechanically stirred until completely dissolved to obtain solution A; weigh 6.2g of solid NaSiO 3 9H 2 O, dissolved in 80mL water to obtain solution B; at room temperature, add solution B dropwise to solution A, and keep stirring, to obtain cloudy solution C; transfer C to a volume of 200mL In a hydrothermal kettle lined with vinyl fluoride, put the hydrothermal kettle into a blast drying oven, keep it warm at 160°C for 24 hours; then cool down naturally, filter, wash, and finally dry at 110°C overnight to obtain SiO 2 The porous silicon-manganese composite particles with a content of 30% are denoted as p-Mn30Si.

[0024] 2) Preparation of porous inorganic composite particles filled polyurethane membrane

[0025] Weigh 6.0g of polyurethane parti...

Embodiment 3

[0028] 1) Preparation of porous silicon-manganese composite particles

[0029] (1) Weigh 4.00g solid KMnO 4 powder and 0.73 g solid MnSO 4 ·H 2 O, respectively dissolved in 80mL deionized water, mechanically stirred until completely dissolved, to obtain solution A; solution A was transferred to a hydrothermal kettle, and the hydrothermal kettle was kept at 160°C for 24 hours, and then filtered, washed, and dried. 1.5g black δ-MnO was obtained 2 solid;

[0030] (2) The resulting δ-MnO 2 Disperse in 80mL deionized water containing 0.5% (mass content) surfactant CTAB, and ultrasonicate for 20 minutes to obtain suspension B; weigh 14.46g of solid NaSiO 3 9H 2 O, dissolved in 80mL water to obtain solution C; then place suspension B in a water bath at 80°C, add solution C to suspension B dropwise under stirring, and obtain cloudy solution D after the addition is complete; D Transfer to a 200mL hydrothermal kettle with a polytetrafluoroethylene liner, put the hydrothermal kett...

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Abstract

The invention discloses a preparing method of filling modified polyurethane film, and belongs to the field of separation of pervaporation film. The preparing method comprises the steps of firstly conducting a co-hydrothermal method or a substep-hydrothermal method to obtain a porous silicomanganese compound particle, then adding the particle into a polyurethane matrix film-casting solution, casting the film-casting solution into film on a polytetrafluoroethylene board, conducting heat treatment on the film at the temperature of 80 DEG C for 4 hours, and conducting vacuum heat-treatment at the temperature of 150 DEG C for 5 hours to obtain the polyurethane film filled by the porous inorganic compound particle. A modifier can simultaneously improve permeation flux and separation factor of the polyurethane film; meanwhile, the preparing process is simple, raw materials are cheap and easy to obtain, and the filled polyurethane film is characterized by being large in permeation flux, high in pervaporatio separation index (PSI) and the like. Through the addition of a proper amount of porous inorganic compound particles, the polyurethane film is excellent in pervaporatio of a low-concentration phenol aqueous solution, when the mass percentage of phenol reaches 0.3% and the operation temperature is 80 DEG C, the separation factor is 9.40-14.53, the permeation flux is 17.76-32.61kg. micrometer. m <-2>.h<-1>, and PSI can reach 441.35 kg. micrometer. m <-2>.h<-1> maximumly.

Description

Technical field: [0001] The invention relates to a preparation method of a filled modified polyurethane membrane, which belongs to the technical field of pervaporation membrane separation. Background technique: [0002] As an emerging membrane separation process, pervaporation technology has the characteristics of low energy consumption, high separation efficiency, and simple process, especially in the separation process of azeotropes, heat-sensitive substances, and low-concentration organic wastewater. Advantage. The key to pervaporation technology lies in the properties of the membrane material. In general, the target component should be preferentially adsorbed and permeated through the membrane material as much as possible to prevent the permeation of other components, so as to achieve the purpose of separating the target component. However, in practical applications, it is difficult for a single polymer membrane material to have both high permeation flux and target comp...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01D67/00B01D53/22B01D71/48
CPCB01D53/228B01D67/0079B01D71/48
Inventor 朱秋锋叶宏冯旭东宋伟伟汪苹
Owner BEIJING TECHNOLOGY AND BUSINESS UNIVERSITY