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A method for efficient remediation of mercury-contaminated soil

A remediation method and mercury pollution technology are applied in the field of remediation of mercury-contaminated soil and mercury-contaminated soil remediation through leaching, which can solve the problems of low secondary pollution, low mercury residue, and low leaching efficiency of mercury-contaminated soil, and achieve the effect. Good, strong elution ability, improved elution effect

Active Publication Date: 2020-02-04
AEROSPACE KAITIAN ENVIRONMENTAL TECH CO LTD
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0006] Aiming at the defects in the method of rinsing and repairing mercury-contaminated soil in the prior art, the purpose of the present invention is to provide a method that can realize the efficient elution of various valence states of mercury in mercury-contaminated soil, with low mercury residue and causing secondary pollution to the environment. A method for repairing mercury-contaminated soil with a low degree of pollution. After leaching and repairing, the removal rate of mercury in the soil can reach more than 90%, which solves the problem of low leaching efficiency of general mercury-contaminated soil.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0051] The contaminated farmland soil around a mercury mine in Guizhou was taken, and the mercury content in the soil was 7.8 mg / kg. After the soil was naturally air-dried, it was ground and passed through a 20-mesh sieve for use. Configure the oxidizing agent and each eluent respectively, wherein the oxidizing agent is to add 4% potassium persulfate solution to 5% HCl solution, the volume ratio is 1:10, the concentration of thiosulfate solution is 0.1moL / L, citric acid The concentration is 1moL / L, the concentration of potassium iodide is 0.1moL / L, the mass percentage concentration of sodium sulfide is 5%, and the addition amount of sodium hydroxide is 1.5% of the amount of sodium sulfide. Weigh 5g of the pretreated soil into a 100mL centrifuge tube, add deionized water to keep the soil moist, and then add the prepared oxidant potassium persulfate solution to control the potassium persulfate in the potassium persulfate solution and the mercury in the mercury-contaminated soil. ...

Embodiment 2

[0061] Get the same soil as in Example 1, and through the same air-drying, grinding and sieving process, configure the oxidizing agent and each eluent respectively, wherein the oxidizing agent is that 4% sodium persulfate solution is added in 5% HCl solution, The volume ratio is 1:10, and the eluent is a mixed solution of ammonium thiosulfate, citric acid, sodium iodide, sodium sulfide and sodium hydroxide, wherein the concentration of ammonium thiosulfate is 0.1moL / L, and the concentration of citric acid is 1moL / L L, the concentration of sodium iodide is 0.1moL / L, the mass percent concentration of sodium sulfide is 5%, and the addition of sodium hydroxide is 1.5% of the amount of sodium sulfide. Take the pretreated soil 5g in the 100mL centrifuge tube, and the next steps are all the same as in Example 1. After air-drying, the soil mercury content measured is 0.79mg / kg, which is higher than the value in Example 1, but lower than "Soil Environmental Quality Standard" (GB15618-1...

Embodiment 3

[0063]Get the same soil as in Example 1, and through the same air-drying, grinding and sieving process, configure the oxidizing agent and each eluent respectively, wherein the oxidizing agent is that 4% potassium persulfate solution is added in 5% HCl solution, The volume ratio is 1:10, and the eluent is a mixed solution of potassium thiosulfate, tartaric acid, potassium iodide, sodium sulfide and sodium hydroxide, wherein the concentration of potassium thiosulfate is 0.1moL / L, the concentration of tartaric acid is 1moL / L, and the concentration of potassium iodide It is 0.1moL / L, the mass percent concentration of sodium sulfide is 5%, and the addition amount of sodium hydroxide is 1.5% of the sodium sulfide consumption. Take the pretreated soil 5g in the 100mL centrifuge tube, and the next steps are all the same as in Example 1. After the air-drying process, the soil mercury content measured is 0.83mg / kg, which is higher than the value in Example 1, but lower than "Soil Enviro...

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PUM

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Abstract

The invention discloses an efficient repair method for mercury pollution soil. The method includes the steps that the mercury pollution soil is subjected to oxidation treatment with an acidic persulfate solution at first; then the soil pH is adjusted to 7 or above; afterwards, elution with a thiosulfate solution and elution with mixed liquor of organic acid and iodate are conducted in sequence; and finally mixed liquor of sodium sulphide and sodium hydroxide is adopted for elution. By the adoption of the method, mercury in various valence states in the mercury pollution soil can achieve efficient elution, the quantity of mercury residues is small, secondary pollution to the environment is avoided and cost is low.

Description

technical field [0001] The invention relates to a method for repairing mercury-contaminated soil, in particular to a method for repairing mercury-contaminated soil by leaching, and belongs to the technical field of heavy metal soil treatment. Background technique [0002] In recent years, with the rapid development of industry and agriculture, a large amount of mercury has been released in the process of production and use, making the soil polluted by mercury more and more serious. The main sources of soil mercury pollution are atmospheric deposition, sewage irrigation, industrial pollution sources (coal-burning, chlor-alkali industry, battery factory, smelting, papermaking and other industries), agricultural pollution sources (use of pesticides and fertilizers), mercury-containing waste (thermometers, waste battery, etc.) mishandled, etc. Mercury and its compounds in the soil can enter the human body through the food chain, causing great harm to the human body. Therefore,...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B09C1/08B09C1/02
CPCB09C1/02B09C1/08
Inventor 邵乐史学峰韩凤刘晓月李昌武
Owner AEROSPACE KAITIAN ENVIRONMENTAL TECH CO LTD