Modified nickel-manganese lithium ion battery cathode material and preparation method thereof
A technology for ion batteries and positive electrode materials, which is applied in the direction of battery electrodes, circuits, electrical components, etc., and can solve problems such as affecting charge and discharge performance, decline in charge and discharge performance, and reduction in capacitance
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[0013] The invention provides a method for preparing a positive electrode material of a modified nickel-manganese lithium ion battery. The preparation method comprises the following steps: (1) dissolving divalent nickel source, divalent manganese source and citric acid in water, and continuously mixing Heating reaction under conditions, after cooling, adding lithium source compound for mixing, and then calcining; wherein, the molar ratio of divalent nickel source, divalent manganese source and lithium source compound is 0.65-0.75:0.25-0.35:1; (2 ) ultrasonically disperse the calcined product in absolute ethanol containing thioacetamide, and then heat the reaction.
[0014] Through the above technical scheme, the charge-discharge performance and cycle performance of the modified nickel-manganese lithium-ion battery cathode material obtained in the present invention are greatly improved. Compared with the existing nickel-manganese lithium-ion battery cathode material, the modifie...
Embodiment 1
[0038]A method for preparing a positive electrode material of a modified nickel-manganese lithium ion battery, the preparation method comprising the following steps:
[0039] (1) Dissolve nickel nitrate, manganese nitrate and citric acid in water, the concentration of divalent nickel ions is 0.03mol / L, heat and react at 80°C for 8 hours under continuous mixing conditions, after cooling, add lithium nitrate for mixing, and then Calcined at 300°C for 4h;
[0040] Wherein, the molar ratio of nickel nitrate, manganese nitrate and lithium nitrate is 0.75:0.25:1, and the consumption of citric acid is 0.08 mol relative to 1 mol of nickel nitrate;
[0041] (2) Ultrasonic disperse the calcined product in absolute ethanol containing thioacetamide for 15 minutes, and then heat the reaction at 120°C for 14 hours, wherein, relative to 8 g of the calcined product, thioacetamide The amount of amide added was 0.15 mol, and the amount of absolute ethanol was 50 mL.
Embodiment 2
[0043] A method for preparing a positive electrode material of a modified nickel-manganese lithium ion battery, the preparation method comprising the following steps:
[0044] (1) Dissolve nickel nitrate, manganese nitrate and citric acid in water, the concentration of divalent nickel ions is 0.06mol / L, heat and react at 95°C for 3 hours under continuous mixing conditions, after cooling, add lithium nitrate for mixing, and then Calcined at 600°C for 1h;
[0045] Wherein, the molar ratio of nickel nitrate, manganese nitrate and lithium nitrate is 0.75:0.25:1, relative to 1 mol of nickel nitrate, the consumption of citric acid is 0.1 mol;
[0046] (2) Ultrasonic disperse the calcined product in absolute ethanol containing thioacetamide for 5 minutes, and then heat the reaction at 190°C for 10 hours, wherein, relative to 8 g of the calcined product, thioacetamide The amount of amide added was 0.3 mol, and the amount of absolute ethanol was 150 mL.
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