A composite film with thermochromic, antifogging and self-repairing functions and its preparation method
A self-healing and anti-fog technology, applied in coatings and other directions, can solve the problems of less research on coatings, and achieve the effects of superior performance, wide application range, and simple preparation process
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[0045] On the other hand, an embodiment of the present invention provides a method for preparing a composite film with thermochromic, anti-fog and self-repairing functions, the method comprising the following steps:
[0046] 1) Prepare a sol solution containing silica hollow sphere nanoparticles: dissolve polyacrylic acid in ammonia water, disperse it ultrasonically, then add it dropwise in absolute ethanol, stir to obtain a mixed solution; add tetraethoxysilane dropwise into the mixed solution and stirred to obtain a sol solution containing silica hollow sphere nanoparticles;
[0047] 2) Preparation of a sol solution containing a tetravalent vanadium precursor: adding vanadium pentoxide and oxalic acid to ethanol, stirring and reacting to obtain a sol solution containing a tetravalent vanadium precursor;
[0048] 3) Prepare a sol solution containing a hydrophobized silica precursor: mix tetraethoxysilane, water, ethanol and hydrochloric acid, stir and react to obtain a silica...
Embodiment 1
[0067] Embodiment 1 contains the preparation of the sol solution of silica hollow sphere nanoparticles
[0068] Dissolve 0.2 grams of polyacrylic acid in 4.5 milliliters of ammonia water, and ultrasonically disperse for 10 minutes; then add dropwise into a container loaded with 90 milliliters of absolute ethanol, and stir for 15 minutes to obtain a mixed solution; 1.5 milliliters of tetraethoxy Silane was added dropwise to the mixed solution at a rate of 45 microliters per minute; after the dropwise addition, the resulting solution was stirred at room temperature (25° C.) for 10 hours to obtain a sol solution containing silica hollow sphere nanoparticles, wherein, The average particle diameter of silica hollow sphere nanoparticles is 38 nanometers (as figure 1 shown).
[0069] Change the quality of polyacrylic acid, when the quality of polyacrylic acid is 0.4 gram and 0.7 gram respectively, the average particle diameter of the silica hollow sphere nanoparticle in the sol solu...
Embodiment 2 2
[0071] The preparation of embodiment 2 silicon dioxide-vanadium dioxide composite film
[0072] (1) Preparation of sol solution containing silica hollow sphere nanoparticles: dissolve 0.1 to 0.3 grams of polyacrylic acid in 4.5 milliliters of ammonia water, ultrasonically disperse for 10 minutes; then add dropwise to a container loaded with 90 milliliters of absolute ethanol , stirred for 15 minutes to obtain a mixed solution; 2 to 3 ml of tetraethoxysilane was added dropwise to the mixed solution at a rate of 45 microliters per minute; Stirring was carried out for 10 hours to obtain a sol solution containing silica hollow sphere nanoparticles;
[0073] (2) Preparation of a sol solution containing a tetravalent vanadium precursor: add vanadium pentoxide and oxalic acid to ethanol, wherein the molar ratios of vanadium pentoxide and oxalic acid are 1:2.5, 1:3 and 1:4.5 respectively and stir the reaction , to obtain a sol solution containing a tetravalent vanadium precursor, dil...
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