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A kind of fiber/polyurethane/polylactic acid blend and preparation method thereof

A technology of polylactic acid and blends, which is applied in the field of fiber/polyurethane/polylactic acid blends and their preparation, can solve the problems of reduced tensile strength and unsatisfactory toughening results, and achieve improved elongation at break and improved Tensile strength, glass transition temperature, and the effect of increasing tensile strength

Active Publication Date: 2021-01-15
GUILIN ELECTRICAL EQUIP SCI RES INST
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, when the content of polyurethane is 20%, the elongation at break of polylactic acid is only increased by 3.3 times, while the tensile strength is reduced by 33% (see section 2.1 of the literature for details), and its toughening result is obviously not enough ideal

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0033] 1) Take 8 kg of PEGA with a number-average molecular weight of 1800 and 1.824 kg of isocyanate (MDI) in a reaction kettle. After mixing evenly, keep the system at 85°C and keep it warm for 2 hours; then cool the system down to 60°C and stir. Add 0.176kg alcohol chain extender (EG), mix evenly, heat up to 70°C for 5h, heat the reaction for 5h, take out the reaction material, and mature it in an oven at 120°C for 4h to obtain TPU; the hard segment of the obtained TPU is The mass ratio in the TPU is 20%, the mass ratio of the soft segment in the TPU is 80%, and the melt index of the TPU obtained is 8g / 10min (under the test condition of 190°C / 2.16kg, the same below);

[0034] 2) get the ramie fiber that length is 2-4mm and place temperature and be 60 ℃, concentration be that 4wt% NaOH aqueous solution soaks 3h, take out, place temperature after draining is 60 ℃, concentration is the KH550 solution (pH of 3wt%) =3, the solvent is a mixed solvent composed of water and absolut...

Embodiment 2

[0042] 1) Take 9kg of PPA with a number-average molecular weight of 2500 and 0.974kg of isocyanate (MDI) in a reactor, mix well, keep the system at 85°C, and keep the temperature for 2 hours; then cool the system to 60°C, and stir Add 0.026kg of alcohol chain extender (BD), mix evenly, raise the temperature to 70°C and keep it warm for 5 hours, take out the reaction material, and mature it in an oven at 120°C for 4 hours to obtain TPU. The hard segment of the obtained TPU is The mass ratio that accounts for in TPU is 10%, and the mass ratio that soft segment accounts for in TPU is 90%, and the melt index of gained TPU is 11g / 10min;

[0043] 2) getting length is that the jute fiber of 2-4mm is placed in temperature and is 60 ℃, concentration is that 15wt% NaOH aqueous solution soaks 3h, takes out, puts temperature after draining and is 80 ℃, concentration is the KH550 solution (pH of 5wt%) =4, the solvent is a mixed solvent composed of water and absolute ethanol in a volume rat...

Embodiment 3

[0059] 1) Take 8.5kg of PEGA with a number average molecular weight of 2500 and 1.371kg of isocyanate (MDI) in a reactor, mix well, keep the system at 90°C, and keep it warm for 2 hours; then cool the system down to 60°C, stirring Add 0.129kg of alcohol chain extender (EG), mix evenly, heat up to 70°C for 4h, heat the reaction for 4h, take out the material obtained from the reaction, and mature it in an oven at 120°C for 4h to obtain TPU; the obtained TPU medium hard segment The mass ratio that accounts for in TPU is 15%, and the mass ratio that soft segment accounts for in TPU is 85%, and the melting index of gained TPU is 18g / 10min;

[0060] 2) getting the sisal fiber of 2-4mm in length and placing it in a KOH aqueous solution with a temperature of 60°C and a concentration of 12wt% for 3h, taking it out, draining it and placing it in a KH550 solution with a temperature of 60°C and a concentration of 3wt% ( pH=4, the solvent is a mixed solvent composed of water and absolute e...

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Abstract

The invention discloses a fiber / polyurethane / polylactic acid blend and a preparation method thereof. The fiber / polyurethane / polylactic acid blend is prepared from polyester type thermoplastic polyurethane, polylactic acid and a fiber, wherein the use level of the fiber is 10% to 30% of the sum of the masses of the polyester type thermoplastic polyurethane and the polylactic acid; in the sum, whichis 100%, of the masses of the polyester type thermoplastic polyurethane and the polylactic acid, the mass ratio for which the polyester type thermoplastic polyurethane accounts is 5% to 20%; the polylactic acid accounts for the balance; the polyester type thermoplastic polyurethane is polyester type thermoplastic polyurethane which is of an amorphous structure; in percentage by mass, a soft segment accounts for 75% to 90% of the mass of the polyester type thermoplastic polyurethane; and a hard segment accounts for the balance. Compared with pure polylactic acid, the blend provided by the invention is not obviously decreased in glass-transition temperature while being obviously improved in elongation at break and tensile strength.

Description

technical field [0001] The invention relates to a polylactic acid modified material, in particular to a fiber / polyurethane / polylactic acid blend and a preparation method thereof. Background technique [0002] The demand for biodegradable plastics is increasing due to the increasing problems of "white waste" and the shortage of petroleum resources and environmental pollution caused by traditional plastics. Polylactic acid (PLA) is regarded as the most promising biodegradable plastic because of its outstanding characteristics such as good processability, mechanical properties, transparency, and sufficient and renewable raw material sources. However, the high brittleness of polylactic acid has become the biggest obstacle restricting its wide application. In order to improve the brittleness and toughness of polylactic acid, many enterprises and scientific research institutes have carried out a lot of modification research on polylactic acid. [0003] At present, the brittle mo...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C08L67/04C08L1/02C08L75/08
CPCC08L67/04C08L2205/03C08L1/02C08L75/08
Inventor 陈志平冯羽风戴展鹏唐培勇
Owner GUILIN ELECTRICAL EQUIP SCI RES INST