Preparation method of microcapsule soil conditioner with dual intelligent response to temperature and pH
The technology of soil conditioner and microcapsule is applied in the field of preparation of microcapsule soil conditioner with dual intelligent response to temperature and pH, and can solve the problem of poor pH sensitivity of chitosan, inability to adjust acid-base soil at the same time, and no temperature Response and other problems, to achieve high drug coating rate, good biodegradability, and low price.
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Embodiment 1
[0032] Dissolve 10g of chitosan in 200mL of 0.1mol / L HCl solution, then add it into 200mL of β-cyclodextrin aqueous solution containing 8g, stir for 1 hour; then gradually add 25% glutaraldehyde, 12mL, 70℃ within 30min The mixture was stirred for 6 hours; then 70 mL of 1 mol / L NaOH aqueous solution was added to precipitate the product; finally, it was washed with acetone and water, and dried in vacuo to obtain CS-g-CD.
[0033] According to -NH 2 : MAA: NIPAM molar ratio is 1:4:4, add 50mL deionized water to CS-g-CD prepared above, MAA, NIPAM respectively at 10g, 0.069g, 0.0905g; ultrasonic 20min, N 2 Protect and stir for 30min, heat to 80°C; then add initiator ammonium persulfate APS 0.0003g, N 2 Protected and stirred for 2 hours; then the temperature was lowered from 80°C to 50°C, 0.1mL glutaraldehyde was added, and reacted for 2 hours; finally, it was washed repeatedly with acetone and deionized water, and the modified CS-g-CD was obtained by vacuum drying .
[0034] Dis...
Embodiment 2
[0038] Dissolve 20g of chitosan in 200mL of 0.1mol / L HCl solution, then add it into 200mL of β-cyclodextrin aqueous solution containing 16g, stir for 1 hour; then gradually add 25% glutaraldehyde, 24mL, 70℃ within 30min The mixture was stirred for 6 hours; then 70 mL of 1 mol / L NaOH aqueous solution was added to precipitate the product; finally, it was washed with acetone and water, and dried in vacuo to obtain CS-g-CD.
[0039] According to -NH 2 : MAA: NIPAM molar ratio is 1:4:4, the prepared CS-g-CD and MAA, NIPAM were added 50mL deionized water at 20g, 0.138g, 0.181g; ultrasonic 20min, N 2 Protect and stir for 30min, heat to 80°C; then add initiator ammonium persulfate APS 0.0006g, N 2 Protected and stirred for 2 hours; then the temperature was lowered from 80°C to 50°C, 0.2mL glutaraldehyde was added, and reacted for 2 hours; finally, it was washed repeatedly with acetone and deionized water, and the modified CS-g-CD was obtained by vacuum drying .
[0040] Dissolve 20...
Embodiment 3
[0044] Dissolve 30g of chitosan in 200mL of 0.1mol / L HCl solution, then add it to 200mL of β-cyclodextrin aqueous solution containing 24g, stir for 1 hour; then gradually add 25% glutaraldehyde within 30min, 36mL, 70℃ The mixture was stirred for 6 hours; then 70 mL of 1 mol / L NaOH aqueous solution was added to precipitate the product; finally, it was washed with acetone and water, and dried in vacuo to obtain CS-g-CD.
[0045] According to -NH 2 : MAA: NIPAM molar ratio is 1:4:4, the prepared CS-g-CD and MAA, NIPAM were added 50mL deionized water at 30g, 0.207g, 0.2715g; ultrasonic 20min, N 2 Protect and stir for 30min, heat to 80°C; then add initiator ammonium persulfate APS 0.0009g, N 2 Protected and stirred for 2 hours; then the temperature was lowered from 80°C to 50°C, 0.3mL glutaraldehyde was added, and reacted for 2 hours; finally, it was washed repeatedly with acetone and deionized water, and the modified CS-g-CD was obtained by vacuum drying .
[0046] Dissolve the...
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