Lithium secondary battery and method for manufacturing lithium secondary battery
A lithium secondary battery, lithiation technology, applied in secondary battery, electrolyte battery manufacturing, lithium battery, etc., to achieve high energy density, suppress internal short circuit, and improve safety effects
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Embodiment 1
[0134] 1. Preparation of an isolation layer with a volume expansion layer disposed thereon
[0135] First, Si (Sigma-Aldrich, 2 , and the barrier layer provided with the volume expansion layer showed an air permeability of 273 sec / 100 cc. Based on the volume before lithiation, the Si inorganic particles showed a volume expansion rate of 300% after lithiation. In addition, the inorganic particles were used in an amount of 80 parts by weight based on 100 parts by weight of the volume expansion layer.
[0136] 2. Preparation of negative electrode with protective layer
[0137] A pre-prepared binder solution of 5 wt% PVDF-HFP (5% HFP, Mw 800,000) was spin-coated on Li metal (thickness 20 μm, Honjo) at 2000 rpm for 1 min, and dried at room temperature for 12 h, thereby A Li negative electrode provided with a protective layer is obtained.
[0138] 3. Preparation of Cathode
[0139] First, LiNi as the positive electrode active material 0.8 co 0.1 mn 0.1 o 2 (NCM811), FX35 as ...
Embodiment 2
[0147] The isolation layer and the cell were obtained and evaluated in the same manner as in Example 1, except that the composition of the volume expansion layer was Si:PVDF=9:1. Here, the thickness of the volume expansion layer is 0.5 μm, and the loading amount is 1.01 g / m 2 , and the barrier layer provided with the volume expansion layer exhibited an air permeability of 258 sec / 100 cc. In addition, the inorganic particles were used in an amount of 90 parts by weight based on 100 parts by weight of the volume expansion layer.
Embodiment 3
[0149] Obtain and evaluate the isolation layer and the cell in the same manner as in Example 1, except that the volume expansion layer has a thickness of 1 μm and a loading capacity of 1.98 g / m 2 , and the barrier layer provided with the volume expansion layer exhibited an air permeability of 281 sec / 100 cc.
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