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Silicone oil-based magnetic liquid and preparation method thereof

A magnetic liquid and silicone oil technology, applied in the field of materials, can solve problems such as inability to meet the needs of complex industrial environments, large viscosity changes, etc., and achieve the best magnetic performance and stability, high magnetic saturation strength, and good fluidity.

Active Publication Date: 2022-05-17
TSINGHUA UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0003] In the existing magnetic liquid preparation technology, substances such as ester and diester oil, kerosene, engine oil, and water have been often used as the base carrier liquid of the magnetic liquid, but these conventional base liquids usually have relatively large changes in temperature. Viscosity changes, unable to meet the needs of some complex industrial environments

Method used

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Examples

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preparation example Construction

[0026] The embodiment of the present invention also provides a method for preparing a silicone oil-based magnetic liquid, comprising the following steps:

[0027]a. Modification: add nano magnetic particles into ammonia water and surfactant, stir and react to obtain modified nano magnetic particles; preferably, the reaction temperature is 20-100°C, and the stirring speed is 200-400r / min, The reaction time is 1-60min, the mass ratio of surfactant and ammonia water is 1:(1-2), and the concentration of ammonia water is 25-28%;

[0028] b. Dosing: wash and dry the modified nano-magnetic particles and disperse them in the base carrier liquid. Preferably, wash with deionized water until the conductivity of the eluate is σ≤30 μs / cm, and then wash with acetone for 2~ 4 times, and finally remove acetone by vacuum drying to obtain an initial magnetic liquid, which is added to silicone oil containing a silicone oil emulsifier to obtain a silicone oil-based magnetic liquid.

[0029] In t...

Embodiment 1

[0034] Example 1Fe 3 o 4 Preparation of silicone oil-based magnetic liquid

[0035] 1. Preparation of magnetic nanoparticles

[0036] Weigh 11g of FeCl 3 ·6H 2 O and 9.7 g FeCl 2 4H 2 O, dissolved in 513mL deionized water, in a water bath at 45°C, stirred at 400r / min for 10min to make it uniform; weighed 17g of concentrated ammonia water, added dropwise to the mixed salt solution, kept heating, the reaction temperature was controlled at 40°C, and stirred After 40 minutes, it can be observed that the mixed solution changes rapidly from yellow to black. After the reaction is completed, magnetically separate magnetic nanoparticles to obtain magnetic nanoparticles, and wash them repeatedly with deionized water until the conductivity of the eluate is σ≤100μs / cm;

[0037] 2. Activation

[0038] Place the magnetic nanoparticles obtained above in ferric chloride solution with a pH value of 2 at 1.0moL / L, heat in a water bath to 60°C for 30 minutes, and then wash the magnetic na...

Embodiment 2

[0046] Example 2 γ-Fe 2 o 3 Preparation of silicone oil-based magnetic liquid

[0047] 1. Preparation of magnetic nanoparticles

[0048] Weigh 11g of FeCl 3 ·6H 2 O and 9.7 g FeCl 2 4H 2 O, dissolved in 513mL deionized water, in a water bath at 45°C, stirred at 400r / min for 10min to make it uniform; weighed 17g of concentrated ammonia water, added dropwise to the mixed salt solution, kept heating, the reaction temperature was controlled at 40°C, and stirred After 40 minutes, it can be observed that the mixed solution changes rapidly from yellow to black. After the reaction is completed, magnetically separate magnetic nanoparticles to obtain magnetic nanoparticles, and wash them repeatedly with deionized water until the conductivity of the eluate is σ≤100μs / cm;

[0049] 2. Activation

[0050] Put the magnetic particles obtained above in a 1.0moL / L ferric chloride solution with a pH value of 2, heat in a water bath to 80°C for 30 minutes, and then wash the magnetic partic...

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Abstract

The invention discloses a silicone oil-based magnetic liquid which comprises nano magnetic particles, a base carrier liquid, a surfactant, silicone oil and a silicone oil emulsifier. Wherein the silicone oil emulsifier comprises at least one of alkyl modified silicone oil / siloxane and polyether modified silicone oil / siloxane. In the magnetic liquid, the mass content of the silicone oil and the silicone oil emulsifier is 40-60%, and the molar ratio of the silicone oil to the emulsifier is (1-5): 1. The silicone oil-based magnetic liquid disclosed by the invention has the excellent performances of uniform particle distribution, no agglomeration, no sedimentation and good fluidity, and can stably work at low temperature for a long time.

Description

technical field [0001] The invention belongs to the field of material technology, in particular to a silicone oil-based magnetic liquid, and in particular, to a preparation method of the silicone oil-based magnetic liquid. Background technique [0002] Magnetic liquid is a new type of intelligent material, which is widely used in many high-tech fields such as aerospace, electronic technology, mechanical chemical industry, energy metallurgy, instrumentation, biomedicine, etc. Generally, the magnetic liquid is a colloidal liquid composed of nano-scale magnetic particles highly dispersed in a base carrier liquid (usually an organic solvent or water). Magnetic properties of solids. In general, each nanoparticle surface needs to be provided with enough repulsive force by the coated surfactant to prevent the magnetic particles from agglomerating together under the action of gravity, interparticle magnetic force or van der Waals force. [0003] In the existing magnetic liquid pre...

Claims

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Application Information

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IPC IPC(8): H01F1/44H01F41/00
CPCH01F1/44H01F41/00
Inventor 李德才聂世琳
Owner TSINGHUA UNIV