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High-activity ferric oxide adsorbant and its prepn

An iron oxide and adsorbent technology, applied in the field of water treatment, can solve the problems of chronic biological toxicity of aluminum ions, narrow optimized pH value range, high raw material cost, and achieve the effects of stable adsorption capacity, prolonged operation period and less loss of adsorbent.

Inactive Publication Date: 2004-04-07
TSINGHUA UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, activated alumina has the following disadvantages: the adsorption capacity is low, the applicable optimal pH range is narrow, and its optimal operating pH value is 3. At this pH value, aluminum ions tend to dissolve, and the dissolved aluminum ions have a chronic biological effect. toxicity
Although the above-mentioned new adsorbents have their own advantages, there are still problems such as relatively low adsorption capacity, dissolution of metal ions, or high cost of raw materials.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0022] Prepare a 0.2wt% aqueous solution with PVA with an average molecular weight of 1,845 (polymerization degree 42), and use this solution to dissolve FeCl 3 Prepare FeCl 3 A mixed solution with a concentration of 1.5M. Precipitate the mixed solution with 10M NaOH solution under stirring at room temperature, control the final pH value of the reaction to 2.5, and stir for 30 minutes to complete the reaction. The precipitate was washed with water, dehydrated and dried to obtain adsorbent sample 1. According to the specific surface area measurement, the specific surface area of ​​the adsorbent sample is 165.6m 2 / g, which is 40% higher than that of ordinary hydrated iron oxide; X-ray diffraction results show that the adsorbent is a completely amorphous substance.

[0023] Sample 1 was used for the adsorption of phosphorus in phosphate solution. The adsorption test was carried out at a temperature of 25°C, an initial pH of 3.0, and an initial phosphorus concentration of 50 ...

Embodiment 2

[0025] Prepare a 0.1wt% PVA solution, and use this solution to dissolve Fe 2 (SO 4 ) 3 Prepare a mixed solution with a concentration of 0.2M. The mixed solution was subjected to precipitation reaction with 1M KOH solution under stirring at room temperature, and the final pH value of the reaction was controlled to be 3.5, and the reaction was completed after stirring for 30 minutes. The precipitate was washed with water, dehydrated and dried to obtain adsorbent sample 2.

[0026] Sample 2 was used for the adsorption of phosphorus in phosphate solution. The adsorption test was carried out at a temperature of 25°C, an initial pH of 5.0, and an initial phosphorus concentration of 50 mg / L. Add 0.1g of sample 2 and 0.1g of active powdered alumina to two 100ml water samples respectively, and the measured adsorption amounts after adsorption equilibrium are: sample 2: 28.9mg-P / g; powdered activated alumina: 22.6mg -P / g. Sample 2 is 1.28 times the adsorption capacity per unit weig...

Embodiment 3

[0028] Prepare a 2.0wt% aqueous solution with an average molecular weight of 3 million (polymerization degree 43,000) PAM, and use this solution to dissolve Fe(NO 3 ) 3 Prepare a mixed solution with a concentration of 0.5M. Under room temperature stirring, the mixed solution was hydrolyzed and precipitated with 5M NaOH solution, the final pH of the reaction was controlled to be 4.5, and the reaction was completed after stirring for 30 minutes. The precipitate was washed with water, dehydrated and dried to obtain adsorbent sample 3.

[0029] Sample 3 was used for the adsorption of phosphorus in phosphate solution. The adsorption test was carried out at a temperature of 25°C, an initial pH of 5, and an initial phosphorus concentration of 50 mg / L. To reach the final equilibrium concentration of 0.5mg / L for 100ml of water sample, 0.278g of sample 3 and 0.934g of powdered activated alumina need to be added respectively, and the dosage of sample 3 is 29.8% of activated alumina. ...

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PUM

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Abstract

The present invention relates to water processing technology. The materials including three-valent inorganic ferric salt, alkali and water soluble hydroxyl polymer or amido polymer are synthesized into ferric oxide via deposition reaction inside solvent in normal temperature; and through further water washing, dewatering and drying, high-activity ferric oxide adsorbent is prepared. The adsorbent thus prepared has the advantages of adsorbing capacity as high as 1.2-2.0 times that of active alumina, bulk density 1.5-2.1 times, low material cost and good circulating regeneration performance. It is used in adsorbing dephosphorization process and has small adsorbent filling volume, long operation period and low operation cost.

Description

technical field [0001] The invention relates to an iron oxide adsorbent and a preparation method thereof, belonging to the technical field of water treatment. Background technique [0002] Excessive phosphorus in environmental waters together with other excess nutrients cause eutrophication of water bodies, and the method of preventing eutrophication by removing phosphorus in water bodies has been proved to be the most long-term effective method. Conventional wastewater biological phosphorus removal method and chemical precipitation phosphorus removal method have defects such as strict operating conditions, secondary pollution, and inability to recover phosphorus resources; while adsorption phosphorus removal method has the advantages of simple and reliable operation, recyclable adsorbent and recyclable phosphorus resources. Advantages of recycling. [0003] In the adsorption phosphorus removal process, activated alumina is commonly used as the adsorbent. However, activate...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): B01J20/06B01J20/30
Inventor 黄霞丁文明
Owner TSINGHUA UNIV