一种镍和助剂金属M掺杂的钛硅分子筛M-Ni-ETS-10的制备方法及其应用

The preparation method of titanium-silicon molecular sieve M-Ni-ETS-10 doped with Ni and auxiliary metal M solves the problems of excessive hydrogenation of acetylene and poor selectivity of ethylene in the existing catalyst process, and achieves high hydrogenation activity and stability, which is suitable for industrial ethylene production.

CN117654613BActive Publication Date: 2026-07-17XIAN ORIGIN CHEM TECH

Patent Information

Authority / Receiving Office
CN · China
Patent Type
Patents(China)
Current Assignee / Owner
XIAN ORIGIN CHEM TECH
Filing Date
2023-12-06
Publication Date
2026-07-17

AI Technical Summary

Technical Problem

Existing catalysts suffer from poor C2H4 selectivity due to excessive acetylene hydrogenation, as well as problems such as unsaturated hydrocarbon polymerization and coking, and catalyst sintering during acetylene hydrogenation. These issues result in short catalyst life and make it difficult to achieve both high hydrogenation activity and high olefin selectivity.

Method used

A method for preparing Ni-doped titanium-silicon molecular sieve M-Ni-ETS-10 was adopted. The Ni-doped titanium-silicon molecular sieve was synthesized by hydrothermal reaction. The high specific surface area of ​​ETS-10 and the spatial isolation effect of the auxiliary metal M enabled the active component Ni to have good dispersibility, reducing the excessive hydrogenation and polymerization of ethylene on the Ni surface and improving the ethylene selectivity and stability of the catalyst.

Benefits of technology

It improves the ethylene selectivity and stability of the catalyst, reduces the ethylene loss rate, extends the catalyst's service life, and lowers the cost, making it suitable for industrial applications.

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Abstract

本发明公开了一种镍和助剂金属M掺杂的钛硅分子筛M‑Ni‑ETS‑10的制备方法,该方法采用钛源、硅源、碱源、氟化物、镍源和助剂金属源为原料,通过水热反应合成得到M‑Ni‑ETS‑10;本发明将含有乙炔和氢气的气体通过预活化的M‑Ni‑ETS‑10进行催化加氢反应。本发明通过Ni掺杂在ETS‑10形成晶格缺陷使与之相邻的骨架氧具有强碱性,降低了Ni对炔烃与烯烃加氢中间体的吸附强度,减少了乙烯的过度加氢和聚合反应导致的催化剂结焦失活,提高了催化剂的乙烯选择性和稳定性,同时提高了活性组分Ni的分散性,增强对乙炔的吸附选择性,并提高其加氢活性,减少了乙烯的过度加氢和聚合,降低了原料中乙烯的损失率。
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