一种具有压电响应性的PVDF基中空纤维纳滤膜的制备方法及应用

A one-step method was used to prepare PVDF-based hollow fiber nanofiltration membranes. By introducing piezoelectric carbon-based materials and optimizing the β-crystal form to form an internal electric field, the problem of poor selective separation performance of hollow fiber nanofiltration membranes was solved, achieving efficient separation of multivalent/monovalent ions, and applicable to various membrane configurations.

CN120115022BActive Publication Date: 2026-07-17TIANJIN POLYTECHNIC UNIV

Patent Information

Authority / Receiving Office
CN · China
Patent Type
Patents(China)
Current Assignee / Owner
TIANJIN POLYTECHNIC UNIV
Filing Date
2025-04-04
Publication Date
2026-07-17

AI Technical Summary

Technical Problem

Existing hollow fiber nanofiltration membranes have poor selective separation performance in mixed ion separation, making them difficult to commercialize. Traditional preparation methods are complex and costly, making it difficult to achieve efficient separation of multivalent/monovalent ions.

Method used

A PVDF-based hollow fiber nanofiltration membrane was prepared using a one-step method. By introducing a carbon-based material with piezoelectric properties through non-solvent phase separation-interface polymerization (NIPS-IP) technology, the β-crystal content of PVDF was optimized, forming a continuous channel and generating an internal electric field within the membrane, thereby enhancing the surface charge density and achieving a triple synergistic effect.

Benefits of technology

It simplifies the preparation process, improves the pure water flux and divalent cation removal rate of the membrane, reduces the monovalent cation removal rate, solves the problems of poor separation efficiency and industrialization in traditional methods, and is suitable for various membrane configurations.

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Abstract

本发明提供了一种具有压电响应性的PVDF基中空纤维纳滤膜的制备方法及应用。具体而言,首先将一定比例的PVDF、无机致孔剂、具有压电性质的碳基导电材料、有机反应单体(TMC)、有机溶剂配制成均匀的黏稠分散液,然后将多元胺分子与水按一定比例混合作为芯液,最后通过“非溶剂致相分离‑界面聚合”同步制备技术(NIPS‑IP)纺丝,一步制成具有压电响应性的PVDF中空纤维纳滤膜。该方法操作简便且制备的纳滤膜β‑PVDF晶型含量高(β晶型相对占比不低于90%)。此外,分散液中添加可形成连续相的具有压电性质的碳基导电材料不仅可进一步提高β‑PVDF晶型的含量,而且与PVDF结合后可在膜内形成连续通路并在纳滤压力驱动下显著提升膜的表面电荷密度以及在膜本体产生内电场,通过“尺寸筛分‑表面强静电作用‑内电场强化”的三重协同作用增强对“多价 / 一价”混合离子的选择分离性能。
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