Acetone Purification via Three-Column Rectification and Oxidative Treatment

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Solution Overview

Problem

Current methods for purifying acetone from cumene hydroperoxide decomposition products are inefficient in removing low molecular weight impurities, leading to reduced purity and quality due to the presence of aldehydes and other unsaturated compounds, which are not effectively removed by simple distillation or existing chemical treatment processes.

Innovation Solution

A three-column rectification process is employed, where an alkaline reagent and an oxidative reagent are added to the first column to form high molecular weight impurities, which are then separated and further purified in subsequent columns, with the second column operating at atmospheric pressure to achieve high purity acetone with low acetaldehyde levels and extended KT-Test times.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of manufacture

If simple distillation methods are used to purify acetone, then the process is simple and equipment requirements are minimal, but impurities such as aliphatic aldehydes, olefins and other low molecular weight compounds remain in the product, reducing purity and quality

Engineering Contradiction:
Improveprocess simplicityVSAvoidacetone purity
Core Design Contradiction:
Ease of manufactureVSManufacturing precision

Solution Approach 1:

The purification process is divided into three separate rectification columns operating in sequence, each targeting specific impurity ranges. The first column removes low molecular weight impurities, the second column further purifies acetone, and the third column removes high molecular weight impurities. This segmentation allows each column to be optimized for specific separation tasks, achieving high purity acetone while maintaining operational simplicity.

Inventive Principle:
Principle #1Segmentation

2Manufacturing precision

If chemical treatment with alkali metal hydroxides is used to remove low-boiling aldehydes, then aldehydes condense to high-boiling aldols that can be removed by distillation, but the aldol derivatives decompose in the reboiler producing low-boiling aldehydes again, resulting in product with lower than desired KT-Test values

Engineering Contradiction:
Improvealdehyde removal efficiencyVSAvoidproduct quality consistency
Core Design Contradiction:
Manufacturing precisionVSReliability

Solution Approach 1:

An oxidative reagent is introduced in the first rectification column to oxidize aldehydes to carboxylic acids before the distillation process. This preliminary oxidation prevents aldehydes from condensing and decomposing in subsequent columns, as the oxidized products remain stable at distillation temperatures. This eliminates the recurring aldehyde formation problem and ensures consistent product quality.

Inventive Principle:
Principle #10Preliminary action

3Manufacturing precision

If three rectification columns are used in sequence with the second column operated under reduced pressure, then acetone purity is improved, but operating costs increase and operating capacity decreases

Engineering Contradiction:
Improveacetone purityVSAvoidoperating capacity
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

All three rectification columns are operated at atmospheric pressure rather than reduced pressure. This parameter change maintains high separation efficiency and acetone purity while avoiding the increased operating costs and reduced operating capacity associated with vacuum operation. The atmospheric pressure operation simplifies equipment requirements and enhances productivity.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method produces high-quality acetone with an acetaldehyde level of less than 5 ppm and a KT-Test time of greater than 11 hours, significantly improving purity and reducing operational costs by maximizing equipment utilization and minimizing capital expenditures for modernization.

Implementation Method 1

removing a top fraction from the first column by distillation to form a first bottom fraction comprising an acetone mixture

Methodology Applied
Scientific EffectDistillation: Distillation

Implementation Method 2

adding an alkaline reagent and an oxidative reagent into the first column to form high molecular weight impurities

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 3

causing low-boiling aldehydes to condense to high-boiling aldols

Methodology Applied
Scientific EffectCondensation reaction: Chemical Bonding

Data Source

PatentEP2370388B1Method for purifying acetone
Publication Date: 2013.07.31 SABIC INNOVATIVE PLASTICS IP BV
  • EP2370388B1 patent drawingFigure 1

AI summary

A method for purifying a crude acetone raw material using three columns in sequence comprises the steps of feeding the crude acetone raw material into a first column; adding an alkaline reagent and an oxidative reagent into the first column; feeding the first bottom fraction to a second rectification column; optionally adding an alkaline reagent to the second column above the charge point of the bottom fraction; separating a purified acetone from the high molecular weight impurities and removing the purified acetone as a top fraction by distillation in the second column, forming a second bottom fraction comprising an acetone mixture comprising high molecular weight impurities; feeding the second bottom fraction to a third rectification column; removing a top fraction from the third column; and returning the top fraction removed from the third column to the first column, wherein the second rectification column is operated at atmospheric pressure.