Acid-Treated Polymerization Reactor Surfaces

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Solution Overview

Problem

In free-radically initiated emulsion polymerization processes, deposits on the inner walls and internals of polymerization reactors impede heat exchange, contaminate the product, and require frequent cleaning, which prolongs polymerization times and affects process economics.

Innovation Solution

Treating the reactor surfaces with an acid solution before applying a deposit-preventing agent, such as condensation products of naphthol and formaldehyde or sodium hydroxymethanesulfinate, improves adhesion and prevents scaling without premature agglomeration, using an aqueous acid solution with suitable acids like ascorbic or citric acid, and applying the antifouling agent with steam.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If the reactor walls are coated with a deposit-preventing agent, then deposit formation is reduced, but the adhesion of the agent to the wall is insufficient

Engineering Contradiction:
Improvedeposit prevention effectivenessVSAvoidadhesion insufficiency
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

The patent applies preliminary action by treating the reactor wall with an acid solution before applying the deposit-preventing agent. This pre-treatment creates a surface that enhances the adhesion of the subsequent coating, ensuring the agent bonds effectively to the wall surface and prevents premature detachment during the polymerization process.

Inventive Principle:
Principle #10Preliminary action

2Reliability

If the reactor is cleaned of deposits after each production cycle, then product contamination is prevented, but polymerization times are significantly lengthened

Engineering Contradiction:
Improveproduct purityVSAvoidpolymerization throughput
Core Design Contradiction:
ReliabilityVSProductivity

Solution Approach 1:

The patent applies preliminary action by coating the reactor walls with a deposit-preventing agent before the polymerization process begins. This preventive coating reduces deposit formation during production, thereby extending the time between cleaning cycles and increasing overall productivity while maintaining product purity.

Inventive Principle:
Principle #10Preliminary action

3Object-generated harmful factors

If steam spray at high temperature is used to apply the deposit-preventing agent, then adhesion is improved, but premature agglomeration in the pipeline occurs

Engineering Contradiction:
Improveadhesion qualityVSAvoidpipeline agglomeration risk
Core Design Contradiction:
Object-generated harmful factorsVSDevice complexity

Solution Approach 1:

The patent applies parameter changes by modifying the pH of the deposit-preventing agent solution to a value below 5 through mixing with an aqueous acid solution. This pH adjustment improves adhesion to the reactor wall while preventing premature agglomeration in the pipeline, as the acidic conditions stabilize the agent until it reaches the application point.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

Significantly reduces deposit formation, maintains reactor efficiency by minimizing heat transfer restrictions, and extends campaign periods in continuous operations without compromising daily output, as demonstrated in the production of vinyl acetate-ethylene copolymers.

Implementation Method 1

the scale preventive agent quickly precipitates on the wall and forms a film

Methodology Applied
Scientific EffectPrecipitation: Precipitation

Implementation Method 2

applying the antifouling agent with steam

Methodology Applied
Scientific EffectHeat transfer: Conduction (thermal)

Data Source

PatentEP3256497B1Method for polymerising ethylenically unsaturated monomers
Publication Date: 2018.09.19 WACKER CHEMIE AG

AI summary

The invention relates to a method for polymerising ethylenically unsaturated monomers by free-radical initiated emulsion polymerisation in an aqueous medium in a polymerisation reactor, wherein the inside walls and optionally also the fittings in the reactor are coated by applying a deposit-inhibiting product before the reactor is filled, characterised in that the surfaces that are to be coated with deposit-inhibiting product are treated with an acid solution.