Acidic Post-CMP Cleaning Composition for Copper Wafer Surface Roughness Control

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Solution Overview

Problem

Conventional post-CMP cleaning solutions are ineffective in removing contaminants like Cu-BTA complexes and copper oxides from wafer surfaces after the Cu-CMP process, leading to increased wafer surface roughness and reliability issues in subsequent semiconductor manufacturing processes.

Innovation Solution

An acidic cleaning composition comprising polyamino-polycarboxylic acids, hydroxycarboxylic acids, and surfactants, with a pH of 1 to 5, is used to effectively remove metallic and non-metallic particulates, controlling the etching rate and enhancing wettability, thereby preventing redeposition of contaminants and minimizing wafer surface roughness.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional post-CMP cleaning solutions containing ammonium hydroxide and amines are used, then contaminants can be removed from the wafer surface, but the cleaning solution produces fishy odors and amines poison the photoresist leading to reliability issues

Engineering Contradiction:
Improvephotoresist reliabilityVSAvoidfishy odor and amine poisoning
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

The invention changes the chemical parameters of the cleaning solution by using organic acids (formic acid, acetic acid, propionic acid, or butyric acid) instead of conventional ammonium hydroxide-based solutions. This parameter change eliminates the fishy odor and prevents amine poisoning of photoresist while maintaining effective contaminant removal capabilities

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention employs readily available organic acids that can be easily disposed of after use, replacing the problematic amine-based solutions. These organic acids provide effective cleaning without the harmful side effects and can be discarded without special handling requirements

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

2Reliability

If strong cleaning agents are used to remove contaminants like Cu-BTA complexes and copper oxides, then cleaning effectiveness improves, but wafer surface roughness increases

Engineering Contradiction:
Improvecleaning effectivenessVSAvoidwafer surface roughness
Core Design Contradiction:
ReliabilityVSManufacturing precision

Solution Approach 1:

The invention optimizes the strength parameters of the cleaning solution by using mild organic acids with controlled concentrations (0.1-10% for formic acid, 0.1-5% for acetic acid, etc.). These parameter settings provide sufficient cleaning power to remove Cu-BTA complexes and copper oxides while maintaining low etching rates that preserve wafer surface smoothness

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention employs dynamic control of the cleaning process by adjusting the organic acid concentration and contact time to achieve optimal cleaning effectiveness. The solution strength is tuned to provide just enough cleaning power without excessive etching, adapting the cleaning action to the specific contamination level on the wafer surface

Inventive Principle:
Principle #15Dynamics

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The acidic cleaning composition efficiently removes contaminants while maintaining low copper etching rates, ensuring smooth subsequent processes like thin layer deposition and photolithography by effectively removing BTA and copper residues, thus enhancing device reliability and yield.

Implementation Method 1

an acidic cleaning composition that is useful for removing the contaminants (such as abrasives, metal complexes, and organic compounds) from a wafer surface after a chemical mechanical polishing (CMP) process

Methodology Applied
Scientific EffectChemical dissolution:

Implementation Method 2

at least one polyamino-polycarboxylic acid, or salt thereof

Methodology Applied
Scientific EffectComplexation:

Implementation Method 3

The conventional post-CMP cleaning solution also usually included a surfactant which is also called a wetting agent that is able to lower the surface tension of the post-CMP cleaning solution, allowing easier spreading

Methodology Applied
Scientific EffectSurface tension reduction: Surface Tension

Implementation Method 4

the extent of copper etching is very low after using the acidic cleaning composition of the present invention for removing the contaminants from the wafer surface after a CMP process

Methodology Applied
Scientific EffectChemical etching:

Data Source

PatentUS7763577B1Acidic post-CMP cleaning composition
Publication Date: 2010.07.27 VIBRANTZ CORP

AI summary

An acidic post-CMP cleaning composition includes at least one polyamino-polycarboxylic acid, or salt thereof; at least one hydroxycarboxylic acid, or salt thereof; and the remainder being substantially water. The acidic cleaning composition also includes a surfactant. The acidic post-CMP cleaning composition has a pH of 1 to 5, and is useful for removing the contaminants from the wafer surface after a CMP process without making roughness worse.