Activated Carbon Processing with Ball Milling and CO2 Activation

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Solution Overview

Problem

Existing methods for preparing activated carbon, such as chemical and physical activation, are inefficient, require additional impurity removal processes, and pose explosion risks, limiting the improvement of specific surface area and pore structure, especially in carbon materials like CNTs.

Innovation Solution

A method involving pretreatment of a carbon aggregate precursor through ball milling and subsequent reaction with CO2, which includes steps of carbon dioxide, and activation, and activation of the carbon material with CO2, and a method for preparing activated carbon, which includes steps of pretreating a carbon aggregate precursor by ball milling and activating it with CO2, without using chemical substances, thereby improving the activation process's safety and efficiency.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Area of stationary object

If chemical activation method is used to increase specific surface area and pore structure, then the specific surface area and pore structure are improved, but the process becomes cumbersome and requires separate impurity removal processes

Engineering Contradiction:
Improvespecific surface areaVSAvoidprocess complexity
Core Design Contradiction:
Area of stationary objectVSDevice complexity

Solution Approach 1:

The patent extracts and eliminates the impurity removal step from the conventional chemical activation process by using physical activation with CO2/steam, which does not generate salt impurities requiring separate removal processes

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent replaces the chemical activation system (using KOH, NaOH, H3PO4, ZnCl2) with a physical activation system using CO2 and steam, substituting chemical reactions with physical oxidation processes to achieve activation without harmful byproducts

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

2Area of stationary object

If chemical activation method is used to increase specific surface area and pore structure, then the specific surface area and pore structure are improved, but there is a risk of explosion due to formation of metals such as K and Na

Engineering Contradiction:
Improvespecific surface areaVSAvoidexplosion risk
Core Design Contradiction:
Area of stationary objectVSObject-affected harmful factors

Solution Approach 1:

The patent converts the potentially harmful chemical activation process into a safe physical activation process by using CO2 and steam, which naturally oxidize carbon without forming explosive metal byproducts, thereby eliminating the explosion risk while maintaining activation effectiveness

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Solution Approach 2:

The patent uses CO2 and steam as activation agents that create a controlled atmosphere without forming explosive metals, replacing the dangerous chemical environment with a safer physical oxidation environment

Inventive Principle:
Principle #39Inert atmosphere (Inert environment)

3Ease of manufacture

If physical activation method is used to activate carbon material, then the process is simpler, but the specific surface area and pore structure improvement is limited

Engineering Contradiction:
Improveprocess simplicityVSAvoidspecific surface area
Core Design Contradiction:
Ease of manufactureVSArea of stationary object

Solution Approach 1:

The patent uses a composite activation approach combining CO2 and steam together, leveraging the complementary strengths of both agents: CO2 provides structural development while steam enhances surface area creation, achieving superior results compared to either agent alone

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent optimizes activation parameters including temperature (700-900°C), gas flow rates, and treatment time to maximize the effectiveness of physical activation, thereby achieving high specific surface area and pore structure development through a simple process

Inventive Principle:
Principle #35Parameter changes

4Ease of manufacture

If physical activation method is used to activate carbon material, then the process is simpler, but there is a risk of explosion due to use of oxygen gas and steam at high temperature

Engineering Contradiction:
Improveprocess simplicityVSAvoidexplosion risk
Core Design Contradiction:
Ease of manufactureVSObject-affected harmful factors

Solution Approach 1:

The patent uses CO2 as an inert-like atmosphere that provides oxidation capability without the explosive risks associated with pure O2, creating a safer activation environment while maintaining process simplicity

Inventive Principle:
Principle #39Inert atmosphere (Inert environment)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method results in activated carbon with enhanced specific surface area and pore structure, maintaining electrical conductivity and mechanical strength, while avoiding the need for separate impurity removal and reducing explosion risks.

Implementation Method 1

pretreating a carbon aggregate precursor containing a number of linear carbons by ball milling

Methodology Applied
Scientific EffectMechanical force: Mechanical Force

Implementation Method 2

activating the pretreated carbon aggregate precursor by reacting with CO2

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 3

physical activation method is a process of activating a carbon material by oxidizing it using a CO2/O2 mixture, or O2 or H2O steam alone or in combination at a high temperature of 700°C to 900°C

Methodology Applied
Scientific EffectHigh temperature reaction: Heating

Data Source

PatentEP4140949B1Active carbon and manufacturing method therefor
Publication Date: 2025.12.31 LG ENERGY SOLUTION LTD
  • EP4140949B1 patent drawingFigure 1A
  • EP4140949B1 patent drawingFigure 1B
  • EP4140949B1 patent drawingFigure 2A

AI summary

The present invention relates to active carbon and a manufacturing method therefor and, more specifically, can manufacture active carbon having an improved specific surface area and pore structure by a process of pre-treating a carbon aggregate precursor containing a plurality of linear carbons through ball milling, followed by reaction with CO2.