Antibody-Drug Conjugate Formulation pH Adjustment

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Solution Overview

Problem

Antibody-drug conjugates (ADCs) face limitations in clinical use due to their tendency to aggregate and reversibly self-associate, which reduces their efficacy and stability, leading to decreased potency and increased toxicity.

Innovation Solution

Formulating ADCs with a benzodiazepine, such as D5 or D5(a), at a pH between 4.0 and 4.5, along with a buffer like succinate and a sugar like trehalose, to reduce reversible self-association, and optionally including a surfactant like polysorbate 20 or a small hydrophobic molecule like betaine to inhibit aggregation.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If ADCs are formulated at conventional pH levels (5.0-7.0), then the formulation is easier to prepare and handle, but reversible self-association occurs significantly, reducing efficacy and stability

Engineering Contradiction:
Improvestability and efficacy of ADCVSAvoidformulation complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The patent applies parameter changes by adjusting the pH of the formulation to a specific range of 4.0-4.5, which is lower than conventional pH levels. This pH adjustment fundamentally changes the electrostatic interactions between ADC molecules, reducing reversible self-association and improving stability and efficacy without significantly complicating the formulation process

Inventive Principle:
Principle #35Parameter changes

2Reliability

If ADCs are formulated without aggregation inhibitors, then the formulation is simpler, but aggregation occurs, reducing clinical efficacy

Engineering Contradiction:
Improveclinical efficacy of ADCVSAvoidformulation composition complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The patent uses parameter changes by adjusting pH to 4.0-4.5 to prevent aggregation, eliminating the need for additional aggregation inhibitor excipients. This approach maintains clinical efficacy while keeping the formulation composition relatively simple

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent introduces trehalose as an intermediary substance that stabilizes ADC monomers and prevents aggregation. Trehalose acts as a protective agent that mediates between the ADC molecules and the aqueous environment, preventing harmful interactions while maintaining formulation simplicity

Inventive Principle:
Principle #24Intermediary (Mediator)

3Reliability

If ADCs exhibit reversible self-association, then the formulation requires fewer stabilizing excipients, but the potency and therapeutic effectiveness decrease

Engineering Contradiction:
Improvepotency of ADCVSAvoidamount of stabilizing excipients
Core Design Contradiction:
ReliabilityVSQuantity of substance

Solution Approach 1:

The patent applies parameter changes by setting pH to 4.0-4.5, which reduces reversible self-association and maintains high potency. This allows the formulation to use minimal amounts of stabilizing excipients while preserving therapeutic effectiveness

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The formulation significantly reduces reversible self-association by up to 90%, enhancing the stability and potency of ADCs, thereby improving their therapeutic effectiveness and safety by maintaining higher monomer levels and reducing viscosity.

Implementation Method 1

ADCs are able to aggregate to each other through various mechanisms, including covalent bonding and hydrophobic interactions

Methodology Applied
Scientific EffectHydrophobic interactions: Hydrophobe

Implementation Method 2

WO 2015/075201 A1 describes surfactant free lyophilized formulations of antibody-drug conjugates

Methodology Applied
Scientific EffectSurfactant action: Surfactant

Data Source

PatentEP3380525B1Pharmaceutical formulations and methods of use thereof
Publication Date: 2023.11.08 IMMUNOGEN INC
  • EP3380525B1 patent drawingFigure 1
  • EP3380525B1 patent drawingFigure 2A~2B
  • EP3380525B1 patent drawingFigure 3

AI summary

This disclosure is directed to antibody-drug conjugates. More specifically, this disclosure is directed to compositions comprising (i) antibody-drug conjugates comprising benzodiazepines, and (ii) a small hydrophobic molecule, methods of treatment using the compositions, and methods of formulating the compositions. Furthermore, this disclosure is directed to methods of reducing reversible self-association in antibodies and in antibody-drug conjugates.