Alcohol Oxidation Catalyst Gold Copper

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Solution Overview

Problem

Existing processes for oxidizing alcohols, particularly fatty alcohols, to produce carbonyl compounds face challenges in achieving high yield and selectivity while minimizing degradation products and waste organic solvents, and require economically and environmentally viable catalyst solutions.

Innovation Solution

A process using a catalyst comprising a gold compound and a copper compound, in the presence of oxygen or oxygen-containing gases, to oxidize ethoxylated alcohols, achieving high yield and selectivity with minimized degradation and allowing for easy catalyst recovery and reuse.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If high reaction temperature (100-270°C) is used for oxidation with noble metal catalyst, then oxidation reaction proceeds efficiently, but the ether link in the desired product degrades

Engineering Contradiction:
Improveoxidation reaction efficiencyVSAvoidether link degradation
Core Design Contradiction:
ProductivityVSObject-affected harmful factors

Solution Approach 1:

The patent changes the temperature parameter from high (100-270°C) to low (20-95°C) range, enabling efficient oxidation while preserving the ether link. This is achieved by combining specific noble metal catalysts (Pd, Pt, Rh, Ir, Ru) with oxygen-containing gases under controlled low-temperature conditions, fundamentally altering the reaction parameters to avoid degradation while maintaining productivity.

Inventive Principle:
Principle #35Parameter changes

2Object-generated harmful factors

If oxygen-containing gases are used as oxidant, then environmental and economic requirements are improved, but yield and selectivity are insufficient for industrial use

Engineering Contradiction:
Improveenvironmental impact and wasteVSAvoidyield and selectivity
Core Design Contradiction:
Object-generated harmful factorsVSProductivity

Solution Approach 1:

The patent employs composite catalyst systems combining multiple noble metals (Pd, Pt, Rh, Ir, Ru) with oxygen-containing gases to achieve high yield and selectivity. This composite approach enhances catalytic activity and selectivity, making the environmentally friendly oxygen-based oxidation process industrially viable with improved productivity while maintaining green chemistry principles.

Inventive Principle:
Principle #40Composite materials

3Productivity

If noble metal catalysts are used for oxidation, then catalytic activity is improved, but catalyst cost and environmental viability are compromised

Engineering Contradiction:
Improvecatalytic activityVSAvoidcatalyst cost and environmental impact
Core Design Contradiction:
ProductivityVSObject-generated harmful factors

Solution Approach 1:

The patent optimizes catalyst parameters by using noble metals in controlled amounts (0.1-10 wt%) under low-temperature conditions with oxygen-containing gases. This parameter optimization reduces catalyst loading requirements, lowering cost while improving environmental viability. The specific combination of noble metal type, concentration, and reaction conditions achieves high activity with minimal environmental impact.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process achieves high yield and selectivity in producing carbonyl compounds with reduced waste and enables cost-effective and environmentally friendly industrial application by enhancing catalytic performance and stability.

Implementation Method 1

oxidizing an alcohol for the production of its corresponding carbonyl compounds wherein the oxidation is performed with oxygen or gases containing oxygen

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 2

in the presence of a catalyst comprising at least a gold compound and a copper compound

Methodology Applied
Scientific EffectCatalysis: Catalysis

Data Source

PatentEP3297985B1Process for oxidation of alcohols using oxygen-containing gases
Publication Date: 2021.08.11 RHODIA OPERATIONS SAS

AI summary

A process of oxidizing an alcohol for the production of its corresponding carbonyl compounds is disclosed, wherein the oxidation is performed with oxygen or gases containing oxygen in the presence of a catalyst comprising at least a gold compound and a copper compound. Said alcohol oxidation by gaseous oxidant can achieve a high yield and selectivity with minimized degradation products or waste organic solvents.