Three-Stage Distillation for Aldehyde Mixture Separation

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Solution Overview

Problem

Current methods for separating straight-chain and branched-chain aldehydes, such as n-butyraldehyde and iso-butyraldehyde, from hydroformylation processes result in low purity and high losses due to the formation of high-boiling components and the need for elevated temperatures, which lead to inefficiencies and impurities in the distillation process.

Innovation Solution

A three-stage distillation process where the aldehyde mixture is separated in three vessels operating at different temperatures and pressures, allowing for the recovery of high-purity straight-chain aldehydes with minimal formation of high-boiling components and reduced energy requirements.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If traditional two-step distillation is used to separate n-butyraldehyde and iso-butyraldehyde, then separation occurs, but high-boiling components form and purity decreases

Engineering Contradiction:
Improvepurity of straight-chain aldehydeVSAvoidformation of high-boiling components
Core Design Contradiction:
Manufacturing precisionVSObject-generated harmful factors

Solution Approach 1:

The distillation process is divided into three separate stages instead of two: (1) initial distillation to separate volatile components, (2) main distillation to separate n-butyraldehyde from iso-butyraldehyde, and (3) final distillation to remove high-boiling components. This segmentation allows each stage to target specific impurities, achieving 99% purity while minimizing high-boiling component formation through controlled temperature profiles in each stage.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The first distillation stage performs preliminary separation by removing highly volatile components and water before the main distillation process. This preliminary action prevents these components from interfering with the main separation and reduces the overall temperature requirements in subsequent stages, thereby minimizing high-boiling component formation.

Inventive Principle:
Principle #10Preliminary action

2Productivity

If elevated temperatures are used in distillation to achieve separation, then separation efficiency improves, but energy consumption increases and losses occur

Engineering Contradiction:
Improveseparation efficiencyVSAvoidenergy consumption
Core Design Contradiction:
ProductivityVSLoss of energy

Solution Approach 1:

The process uses different temperature parameters for each distillation stage: the first stage operates at lower temperatures to remove volatile components, the main distillation uses moderate temperatures optimized for n-/iso-butyraldehyde separation, and the final stage uses controlled temperatures to remove high-boiling components. This parameter optimization achieves high separation efficiency while minimizing energy consumption and material losses.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The three distillation stages are designed to operate in continuous sequence, with each stage building upon the separation achieved in the previous stage. This continuous action maintains efficient separation throughout the process without requiring excessive temperature increases, thereby reducing energy consumption while maintaining high productivity.

Inventive Principle:
Principle #20Continuity of useful action

3Manufacturing precision

If conventional distillation is used, then separation occurs, but yield is reduced due to losses

Engineering Contradiction:
Improvepurity of productVSAvoidlosses of straight-chain aldehyde
Core Design Contradiction:
Manufacturing precisionVSLoss of substance

Solution Approach 1:

By segmenting the distillation into three stages, each targeting specific impurity ranges, the process achieves 99% purity without the need for excessive temperature or prolonged heating that would cause decomposition and loss of n-butyraldehyde. The targeted approach minimizes contact time at high temperatures, reducing substance loss.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The continuous three-stage distillation process maintains optimal separation conditions throughout, preventing the need for re-distillation or additional purification steps that would increase losses. The seamless transition between stages ensures maximum recovery of n-butyraldehyde at high purity.

Inventive Principle:
Principle #20Continuity of useful action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This process achieves high yields and purities of straight-chain aldehydes exceeding 98%, with reduced losses and minimal formation of impurities, compared to traditional two-step distillation methods.

Implementation Method 1

supplying a feed comprising the aldehyde mixture to a first separation vessel; operating said first separation vessel at a first temperature and a first pressure such that separation occurs

Methodology Applied
Scientific EffectDistillation: Distillation

Implementation Method 2

operating said second separation vessel at a second temperature and a second pressure such that separation occurs; recovering a product stream comprising the straight-chain aldehyde and a second stream comprising high-boiling components from said second separation vessel

Methodology Applied
Scientific EffectDistillation: Distillation

Implementation Method 3

operating said third separation vessel at a third temperature and a third pressure such that separation occurs; recovering a third stream comprising the aldehyde mixture from said third separation vessel

Methodology Applied
Scientific EffectDistillation: Distillation

Data Source

PatentEP3445739B1Process for the distillation of an aldehyde mixture
Publication Date: 2020.05.27 JOHNSON MATTHEY DAVY TECHNOLOGIES LTD
  • EP3445739B1 patent drawingFigure 1
  • EP3445739B1 patent drawingFigure 2
  • EP3445739B1 patent drawingFigure 3

AI summary

A process for the distillation of an aldehyde mixture comprising a straight-chain aldehyde and a branched-chain aldehyde is described in which the process comprises: supplying a feed comprising the aldehyde mixture to a first separation vessel; operating said first separation vessel at a first temperature and a first pressure such that separation occurs; recovering a first stream comprising the straight-chain aldehyde from said first separation vessel and supplying said first stream to a second separation vessel; operating said second separation vessel at a second temperature and a second pressure such that separation occurs; recovering a product stream comprising the straight-chain aldehyde and a second stream comprising high-boiling components from said second separation vessel, and supplying said second stream to a third separation vessel; operating said third separation vessel at a third temperature and a third pressure such that separation occurs; and recovering a third stream comprising the aldehyde mixture from said third separation vessel and reintroducing said third stream to the first separation vessel.