Aligned Carbon Allotrope Electrodes for High-Capacity Batteries

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Solution Overview

Problem

Existing electrochemical energy storage systems, such as lithium-ion batteries, face limitations in intercalation capacity and ion accessibility due to the use of graphite-based negative electrodes, which restricts charging and discharging efficiency.

Innovation Solution

A method involving the application of a suspension containing electrically conductive carbon allotropes like graphene flakes on a substrate, followed by alignment using an electric field and solvent evaporation, either through heating or microwave radiation, to create a homogeneously aligned active material layer that enhances ion diffusion and storage capacity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If graphite-based negative electrodes are used, then the structure is simple and manufacturing is easy, but the intercalation capacity for lithium ions is low and ion accessibility is limited

Engineering Contradiction:
Improveintercalation capacityVSAvoidelectrode structure
Core Design Contradiction:
Quantity of substanceVSDevice complexity

Solution Approach 1:

The patent changes the material parameter from conventional graphite to carbon allotropes (graphene, carbon nanotubes, fullerenes), which have fundamentally different intercalation properties and capacities for lithium ions, thereby resolving the contradiction between capacity and structural simplicity

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent employs composite electrode structures combining carbon allotropes with conductive materials and binders, creating a multi-component system that achieves high intercalation capacity while maintaining structural integrity and manufacturability

Inventive Principle:
Principle #40Composite materials

2Quantity of substance

If carbon allotropes such as graphene are used to increase intercalation capacity, then storage capacity improves, but the production process becomes more complex requiring suspensions and alignment procedures

Engineering Contradiction:
Improvestorage capacityVSAvoidproduction process
Core Design Contradiction:
Quantity of substanceVSDevice complexity

Solution Approach 1:

The patent applies electric or magnetic fields during the suspension application process to pre-align carbon allotropes before the binder sets, ensuring optimal orientation for ion intercalation while integrating the alignment step into the existing manufacturing workflow

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The patent replaces mechanical alignment methods with electric or magnetic field-based alignment, which is more efficient and can be applied uniformly across the entire electrode surface during the coating process itself

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

3Productivity

If carbon allotropes are aligned using electric or magnetic fields, then ion accessibility and diffusion improve, but the manufacturing process complexity increases

Engineering Contradiction:
Improvecharging and discharging efficiencyVSAvoidmanufacturing process
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The patent uses the same electric or magnetic field generation system for both aligning carbon allotropes during coating and potentially for activating or optimizing the electrode performance during operation, reducing overall system complexity

Inventive Principle:
Principle #6Universality (Multi-functionality)

Solution Approach 2:

The patent designs the suspension formulation and application process so that the carbon allotropes self-align under the applied field without requiring additional alignment equipment or post-processing steps, making the process self-contained and efficient

Inventive Principle:
Principle #25Self-service

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach results in improved high-current capability, specific power density, and reduced charging and discharging times, significantly increasing storage capacity and efficiency compared to conventional graphite-based systems.

Implementation Method 1

generating an electric field penetrating the suspension with a predetermined field direction relatively to the substrate to align the carbon allotropes in the field direction

Methodology Applied
Scientific EffectElectric field alignment: Electric Field

Implementation Method 2

The heating takes place by supplying microwave radiation

Methodology Applied
Scientific EffectMicrowave heating: Microwave Radiation

Implementation Method 3

removing the solvent from the suspending medium heating the suspension to evaporate the solvent from the suspending medium

Methodology Applied
Scientific EffectEvaporation: Evaporation

Data Source

PatentEP3109928B1Method for producing an electrode, in particular for electrochemical energy storage and electrode and electrochemical energy storage
Publication Date: 2019.08.14 AIRBUS DEFENCE & SPACE GMBH
  • EP3109928B1 patent drawingFigure 1~3

AI summary

A method for producing an electrode (14) comprises the steps of applying a suspension (6) consisting of a solvent-containing suspension medium (8) and electrically conductive carbon allotropes (10) to a substrate (2), generating an electric field (12) penetrating the suspension (6) with a predetermined field direction to align the carbon allotropes (10) in the field direction, and removing the solvent from the suspension medium (8) to cure the suspension (6) with the carbon allotropes (10) aligned. An electrode (14) produced in this manner results in a higher capacity, a higher charging and discharging rate, i.e., in particular, a higher deliverable electric current and shorter charging and discharging times of secondary batteries.