Alkaline Delamination of Multilayer Films for Polyolefin Recycling

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Solution Overview

Problem

Current recycling processes for polyolefin mixed streams face challenges in efficiently separating and purifying desired polyolefins due to contamination from non-polyolefin materials and poor mechanical properties of cross-linked polyolefins, leading to low recycling rates and high waste generation.

Innovation Solution

A combined washing/delamination process using an alkaline aqueous solution is employed to treat polyolefin mixed recycling streams. This process involves selecting and enriching the desired polyolefin, milling into flakes, treating with an alkaline solution for delamination, rinsing to remove residues, and sorting to isolate the desired polyolefin, thereby improving the yield and purity of recycled polyolefins.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If multilayer films are removed from polyolefin mixed recycling streams, then contamination is reduced, but polyolefin recovery is lost

Engineering Contradiction:
Improvepurity of recycled polyolefinVSAvoidpolyolefin recovery
Core Design Contradiction:
Manufacturing precisionVSLoss of substance

Solution Approach 1:

The multilayer film is segmented into separate layers through delamination, allowing the polyolefin layer to be separated from contaminating layers. This enables recovery of the polyolefin while removing contamination sources.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

An alkaline aqueous solution acts as an intermediary medium to facilitate delamination of the multilayer films. The solution enables separation of layers without requiring removal of the entire multilayer structure, thus preserving polyolefin recovery while reducing contamination.

Inventive Principle:
Principle #24Intermediary (Mediator)

2Loss of substance

If delamination procedures are added to the recycling process, then polyolefin recovery is improved, but process complexity increases

Engineering Contradiction:
Improvepolyolefin recoveryVSAvoidprocess steps
Core Design Contradiction:
Loss of substanceVSDevice complexity

Solution Approach 1:

The delamination step is merged with the existing washing step in the recycling process. By combining these two functions into a single integrated step using an alkaline aqueous solution, the process achieves improved polyolefin recovery without proportionally increasing process complexity.

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The alkaline aqueous solution serves multiple functions simultaneously: it acts as both a washing medium and a delamination agent. This multi-functionality reduces the need for separate dedicated delamination equipment and procedures, thereby limiting the increase in process complexity.

Inventive Principle:
Principle #6Universality (Multi-functionality)

3Ease of manufacture

If simple washing is used, then process economy is maintained, but delamination efficiency is insufficient

Engineering Contradiction:
Improveprocess economyVSAvoiddelamination efficiency
Core Design Contradiction:
Ease of manufactureVSProductivity

Solution Approach 1:

The washing solution parameters are changed from neutral to alkaline, which fundamentally alters its interaction with multilayer films. This parameter change enables the solution to perform both washing and delamination functions effectively, maintaining process economy while significantly improving delamination efficiency.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process effectively delaminates multilayer films, removes contaminants, and enhances the yield of desired polyolefins, thereby improving the efficiency and economy of polyolefin recycling while minimizing waste.

Implementation Method 1

treating the recycling stream (B) enriched in the desired polyolefin (PO) in flaked form with an alkaline aqueous solution

Methodology Applied
Scientific EffectAlkaline hydrolysis: Hydrolysis

Data Source

PatentUS20250115729A1Combined washing/delamination process for multilayer film-containing recycling streams
Publication Date: 2025.04.10 BOREALIS AG

AI summary

A method for achieving the simultaneous washing/delamination of multilayer films via treatment with an alkaline aqueous solution during a mechanical recycling process, thereby improving the yield and/or purity of a desired polyolefin.