Alkyl-Modified Copolymer Thickener for Electrolyte Stability

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Solution Overview

Problem

Conventional copolymers of (meth)acrylic acid and alkyl (meth)acrylate ester exhibit poor water solubility and significant viscosity changes in the presence of electrolytes, making it difficult to maintain consistent viscosity and transparency in cosmetic applications.

Innovation Solution

A copolymer comprising 100 parts by mass of (meth)acrylic acid, 1.5 to 4.5 parts by mass of alkyl (meth)acrylate ester with 18 to 24 carbon atoms, and 0 to 0.1 parts by mass of a compound with two or more ethylenically unsaturated groups, along with 1.5 to 4.5 parts by mass of a nonionic surfactant, which is copolymerized to produce a neutralized viscous liquid with improved dispersibility and stability in the presence of electrolytes.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional copolymers of (meth)acrylic acid and alkyl (meth)acrylate ester are used, then they can provide thickening function in cosmetics, but they exhibit poor water solubility and significant viscosity changes in the presence of electrolytes

Engineering Contradiction:
Improveviscosity stabilityVSAvoidwater solubility
Core Design Contradiction:
ReliabilityVSAdaptability or versatility

Solution Approach 1:

The patent creates a composite polymer structure by copolymerizing three components: (meth)acrylic acid (provides carboxyl groups for thickening), alkyl (meth)acrylate ester with 18-24 carbon atoms (improves water solubility and prevents precipitation), and a compound with two or more ethylenically unsaturated groups (enhances structural stability). This composite material approach resolves the contradiction by combining materials with complementary properties to achieve both viscosity stability and water solubility.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent optimizes specific compositional parameters: the alkyl group is restricted to 18-24 carbon atoms (narrowing the range from conventional 8-30 carbons), the electrolyte concentration is controlled at 0.1-10 mass%, and the polymer concentration is maintained at 0.1-1 mass%. These parameter changes ensure the copolymer maintains stable viscosity and solubility across varying conditions.

Inventive Principle:
Principle #35Parameter changes

2Strength

If the copolymer concentration is increased to maintain viscosity, then thickening effect is improved, but light transmittance decreases and the liquid becomes less transparent

Engineering Contradiction:
Improvethickening effectVSAvoidlight transmittance
Core Design Contradiction:
StrengthVSIllumination intensity

Solution Approach 1:

The patent optimizes the polymer concentration parameter to 0.1-1 mass%, which is a relatively low concentration range. Within this optimized parameter range, the copolymer achieves effective thickening while maintaining high light transmittance and transparency, resolving the contradiction between thickening effect and transparency.

Inventive Principle:
Principle #35Parameter changes

3Adaptability or versatility

If electrolyte concentration is increased to improve product formulation, then functional ingredients can be added, but copolymer precipitation occurs and viscosity decreases

Engineering Contradiction:
Improveformulation flexibilityVSAvoidviscosity maintenance
Core Design Contradiction:
Adaptability or versatilityVSReliability

Solution Approach 1:

The copolymer's composite structure, particularly the inclusion of alkyl (meth)acrylate ester with 18-24 carbon atoms, provides electrolyte resistance that prevents precipitation. This allows the formulation to maintain flexibility for adding functional ingredients while preserving viscosity stability even at electrolyte concentrations of 0.1-10 mass%.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The resulting copolymer produces a neutralized viscous liquid with excellent water dispersibility, stable viscosity, and high transparency, even in the presence of electrolytes, suitable for use as a thickener in cosmetics.

Implementation Method 1

reacting a specified amount of an olefinic unsaturated carboxylic acid monomer, a specified amount of an alkyl (meth)acrylate ester, and a crosslinking agent

Methodology Applied
Scientific EffectCrosslinking: Chemical Bonding

Implementation Method 2

1.5 to 4.5 parts by mass of a nonionic surfactant

Methodology Applied
Scientific EffectSurfactant action: Surfactant

Data Source

PatentUS11725072B2Alkyl-modified carboxyl group-containing copolymer, thickener containing said copolymer, and method for preparing said copolymer
Publication Date: 2023.08.15 SUMITOMO SEIKA CHEM CO LTD

AI summary

Provided is an alkyl-modified carboxyl group-containing copolymer with which a neutralized viscous liquid can be prepared which has excellent dispersibility in water, has a viscosity that does not change greatly regardless of addition of an electrolyte, and has high transparency in the presence of an electrolyte. This alkyl-modified carboxyl group-containing copolymer contains: 100 parts by mass of a (meth)acrylic acid; 1.5-4.5 parts by mass of a (meth)acrylic acid alkyl ester, in which an alkyl group has 18-24 carbon atoms; and 0-0.1 parts by mass of a compound having two or more ethylenically unsaturated groups, wherein the copolymer contains 1.5-4.5 parts by mass of a nonionic surfactant.