Crystalline Aluminum Nitride Coating for Scratch Resistance

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Solution Overview

Problem

Existing scratch-resistant coatings for glass ceramics face limitations due to thermal expansion coefficient mismatches, restricting the use of hard materials like aluminum nitride, and require enhanced resistance to wear, polishing, and environmental stresses.

Innovation Solution

A transparent, high-refractive hard material layer based on crystalline aluminum nitride with a hexagonal crystal structure and a preferred (001) orientation, exceeding 50% AlN by weight, is applied using sputtering, providing high scratch resistance, chemical resistance, and mechanical durability while maintaining transparency and optical inconspicuousness.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If aluminum nitride coating is applied to increase scratch resistance, then hardness is improved, but thermal expansion coefficient mismatch causes layer stresses and reduced reliability

Engineering Contradiction:
Improvescratch resistanceVSAvoidlayer stress resistance
Core Design Contradiction:
StrengthVSReliability

Solution Approach 1:

The patent changes the crystal structure parameter of aluminum nitride from amorphous to crystalline hexagonal phase, which fundamentally alters the thermal expansion coefficient to match glass ceramic substrates, thereby reducing layer stresses while maintaining high scratch resistance

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite coating system where crystalline aluminum nitride is combined with specific crystal orientation (c-axis perpendicular to substrate) to achieve both high hardness and thermal compatibility, effectively combining properties that were previously mutually exclusive

Inventive Principle:
Principle #40Composite materials

2Strength

If crystalline structure is used to improve mechanical resistance, then hardness and elasticity are improved, but surface roughness increases leading to more defects

Engineering Contradiction:
Improvemechanical resistanceVSAvoidsurface defects
Core Design Contradiction:
StrengthVSObject-affected harmful factors

Solution Approach 1:

The patent optimizes crystallite size parameter to the nanometer range (5-50 nm), which is sufficient to provide mechanical strength through crystalline structure while small enough to minimize surface roughness and defect formation

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent controls the orientation dimension of crystallites by ensuring c-axis perpendicularity to the substrate surface, which provides mechanical strength in the relevant direction while maintaining smooth surface topology in the lateral dimensions

Inventive Principle:
Principle #17Another dimension (Dimensionality change)

3Strength

If high AlN content is used to improve scratch resistance, then hardness is improved, but transparency decreases

Engineering Contradiction:
Improvescratch resistanceVSAvoidlight transparency
Core Design Contradiction:
StrengthVSIllumination intensity

Solution Approach 1:

The patent changes the crystalline phase and orientation parameters of aluminum nitride, which modifies the optical properties to reduce light scattering while maintaining high hardness, allowing >80% transparency even with high AlN content

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent exploits the anisotropic optical properties of hexagonal crystalline AlN by orienting crystals with c-axis perpendicular to substrate, which minimizes light scattering in the visible spectrum while maintaining mechanical strength

Inventive Principle:
Principle #17Another dimension (Dimensionality change)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The coating achieves superior scratch resistance, wear resistance, and environmental durability with enhanced mechanical properties, including high transparency and resistance to cleaning agents, making it suitable for optical and cooking surfaces.

Implementation Method 1

The coating according to the invention and the correspondingly coated substrate can in particular be produced by sputtering

Methodology Applied
Scientific EffectSputtering: Sputtering

Data Source

PatentEP2942333B1Scratch resistant coatings, substrates with scratch-resistant coatings and method for producing the same
Publication Date: 2017.06.28 SCHOTT AG
  • EP2942333B1 patent drawingFigure 1~4
  • EP2942333B1 patent drawingFigure 5~6b
  • EP2942333B1 patent drawingFigure 7~8

AI summary

The invention relates to a substrate with a coating for increasing scratch resistance, wherein the coating comprises at least one high-refractive-index, transparent hard layer. The hard layer contains crystalline aluminum nitride, which has a hexagonal crystal structure with a predominant (001) preferred orientation of the hexagonal symmetry. The invention further relates to a method for producing a correspondingly coated substrate and its use.