Aligned Alpha-Gamma Spectrometry for In Situ Alpha Emitter Quantification

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Solution Overview

Problem

Current methods for characterizing nuclear wastes, such as gamma and neutron spectrometry, are inadequate for identifying and quantifying alpha emitters due to interference from other radionuclides and are sensitive to high-density matrices, while vacuum chamber alpha spectrometry is time-consuming and expensive, making it unsuitable for industrial applications.

Innovation Solution

A system comprising an alignment device for aligning an alpha detector and a gamma detector with a sample between them, using a material that allows gamma radiation to pass, enabling simultaneous alpha and gamma spectrometry measurements under ambient conditions, and a collimation grid to enhance energy resolution, allowing for in situ radiological characterization of alpha emitters.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Measurement precision

If vacuum chamber alpha spectrometry is used to determine quantitative inventory of alpha-emitting radionuclides, then measurement precision is improved, but productivity is worsened due to time-consuming and expensive sample preparation

Engineering Contradiction:
Improvequantitative inventory determinationVSAvoidindustrial production rate
Core Design Contradiction:
Measurement precisionVSProductivity

Solution Approach 1:

The invention changes the operating conditions from vacuum to ambient pressure, eliminating the need for vacuum chamber preparation. This parameter change allows direct measurement of alpha-emitting radionuclides without time-consuming sample preparation, thereby improving productivity while maintaining measurement precision through the use of appropriate detectors and analysis methods

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention extracts the sample preparation step from the measurement process by using ambient pressure alpha spectrometry with collimation grids. This eliminates the need for vacuum chamber preparation and chemical separation, allowing direct measurement and significantly reducing preparation time and costs

Inventive Principle:
Principle #2Taking out (Extraction)

2Ease of operation

If gamma spectrometry is used for characterisation of nuclear wastes, then ease of operation is improved, but measurement precision is worsened due to interference from other radionuclides and sensitivity to high-density matrices

Engineering Contradiction:
Improvenon-destructive measurementVSAvoididentification and quantification of alpha emitters
Core Design Contradiction:
Ease of operationVSMeasurement precision

Solution Approach 1:

The invention segments the measurement capabilities by combining gamma spectrometry (for easy non-destructive measurement) with alpha spectrometry under ambient conditions (for precise alpha emitter identification). This segmentation allows each technique to contribute its strengths: gamma for operational ease and alpha for measurement precision regarding alpha emitters

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The invention merges gamma spectrometry and alpha spectrometry into a single integrated system. By combining these two measurement techniques, the system achieves both the operational ease of gamma spectrometry and the measurement precision for alpha emitters, resolving the contradiction between ease of operation and measurement precision

Inventive Principle:
Principle #5Merging (Combining)

3Productivity

If atmospheric pressure alpha spectrometry is used without collimation, then productivity is improved by eliminating preparation steps, but measurement precision is worsened due to significant deterioration of alpha spectrum

Engineering Contradiction:
Improvemeasurement speedVSAvoidalpha spectrum quality
Core Design Contradiction:
ProductivityVSMeasurement precision

Solution Approach 1:

The invention introduces a collimation grid as an intermediary element in the ambient pressure alpha spectrometry system. This collimation grid selectively transmits alpha particles while blocking others, thereby improving the quality of the alpha spectrum without requiring time-consuming sample preparation, thus maintaining both productivity and measurement precision

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

Enables accurate, in situ, and cost-effective identification and quantification of alpha emitters in nuclear wastes without destructive sample preparation, facilitating real-time radiological characterization and reducing measurement time and costs.

Implementation Method 1

at least one portion of which, delimited by the upper and lower faces and including the alignment axis, is made of a material able to let the gamma radiations pass

Methodology Applied
Scientific EffectGamma radiation transmission: Absorption (EM radiation)

Implementation Method 2

an alpha detector (3), equipped with a collimation grid, able to provide alpha spectrometry measurements

Methodology Applied
Scientific EffectAlpha particle detection: Photoelectric Effect

Implementation Method 3

a gamma detector (4) able to provide gamma spectrometry measurements

Methodology Applied
Scientific EffectGamma radiation detection: Photoelectric Effect

Implementation Method 4

an alpha detector (3), equipped with a collimation grid, able to provide alpha spectrometry measurements

Methodology Applied
Scientific EffectAlpha particle collimation: Filter (optical)

Data Source

PatentUS12360264B2System for correlating alpha and gamma spectrometry measurements for in situ radiological characterisation of a sample
Publication Date: 2025.07.15 COMMISSARIAT A LENERGIE ATOMIQUE ET AUX ENERGIES ALTERNATIVES
  • US12360264B2 patent drawing
  • US12360264B2 patent drawing
  • US12360264B2 patent drawing

AI summary

A system is provided for correlating gamma spectrometry measurements and alpha spectrometry measurements of a same sample comprising radionuclides. The system includes at least a gamma detector able to provide gamma spectrometry measurements; an alpha detector able to provide alpha spectrometry measurements, equipped with a collimation grid; and means for acquiring and analysing alpha spectrometry and gamma spectrometry measurements.