Reversible CO2 Adsorption via Amine-Functionalized Polymeric Cartridges

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Solution Overview

Problem

Current methods for capturing carbon dioxide from gas mixtures, especially ambient air, are energy-intensive and costly, often requiring pressurized equipment and cryogenic processes, which are impractical for widespread use and can introduce impurities that harm plant growth.

Innovation Solution

A device using polymeric adsorbent cartridges with primary amino functionality, capable of reversible adsorption and desorption through pressure, humidity, and temperature swings, allowing for efficient carbon dioxide capture and release without the need for high-pressure equipment, and employing a heating mechanism to regenerate the adsorbent.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If cryogenic air liquefaction processes are used to produce bottled carbon dioxide, then high-purity carbon dioxide is obtained, but energy consumption increases tremendously and transport costs rise

Engineering Contradiction:
Improvecarbon dioxide purityVSAvoidenergy consumption
Core Design Contradiction:
Manufacturing precisionVSUse of energy by moving object

Solution Approach 1:

The patent changes the operational parameters from extreme conditions (cryogenic temperatures, high pressure) to ambient or mild conditions. The adsorption process operates at atmospheric pressure and moderate temperatures, while desorption uses heated air or nitrogen flow, dramatically reducing energy consumption compared to cryogenic liquefaction while maintaining carbon dioxide purity through selective adsorption by amine-functionalized materials

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent employs porous adsorbent materials with amine functional groups that selectively capture carbon dioxide from air or gas streams. These materials provide high surface area and selective binding sites, enabling purification without energy-intensive processes. The porous structure allows efficient mass transfer and regeneration through temperature or pressure swing methods

Inventive Principle:
Principle #31Porous materials

2Ease of manufacture

If flue gas is used directly for greenhouse plant growth, then costs are reduced compared to bottled carbon dioxide, but noxious components negatively affect plant growth

Engineering Contradiction:
ImprovecostVSAvoidplant growth inhibition
Core Design Contradiction:
Ease of manufactureVSObject-affected harmful factors

Solution Approach 1:

The patent extracts only the beneficial carbon dioxide component from complex gas streams such as flue gas or air, leaving behind noxious components like sulfur oxides, nitrogen oxides, and other contaminants. The amine-functionalized adsorbent selectively binds carbon dioxide, which is then desorbed in a purified form suitable for plant application, maintaining low cost by using air or flue gas as feedstock while eliminating harmful substances

Inventive Principle:
Principle #2Taking out (Extraction)

3Productivity

If solid adsorbent materials are used in packed bed form with pressurized gas, then carbon dioxide capture is achieved, but the system complexity and equipment requirements increase

Engineering Contradiction:
Improvecarbon dioxide capture efficiencyVSAvoidsystem complexity
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The patent employs dynamic operation modes where the system alternates between adsorption and desorption phases. During adsorption, ambient air or gas stream passes through the adsorbent bed to capture carbon dioxide. During desorption, heated inert gas flows through the same bed to release concentrated carbon dioxide. This dynamic switching enables continuous operation and simplifies equipment by using the same hardware for both capture and regeneration

Inventive Principle:
Principle #15Dynamics

Solution Approach 2:

The system operates in periodic cycles of adsorption and temperature-swing desorption. The adsorbent bed is periodically heated to release captured carbon dioxide, then cooled and repressurized for the next adsorption cycle. This periodic operation maintains high productivity while simplifying device design compared to continuous high-pressure systems

Inventive Principle:
Principle #19Periodic action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This method enables the production of high-concentration carbon dioxide gas mixtures with lower energy consumption, increased yield, and reduced costs, providing a reliable and flexible source for plant growth and other applications without introducing harmful contaminants.

Implementation Method 1

a polymeric particular adsorbent for carbon dioxide having a primary amino functionality

Methodology Applied
Scientific EffectAdsorption: Adsorption

Implementation Method 2

reversible adsorption and desorption through pressure, humidity, and temperature swings

Methodology Applied
Scientific EffectChemical adsorption: Chemisorption

Implementation Method 3

employing a heating mechanism to regenerate the adsorbent

Methodology Applied
Scientific EffectDesorption: Desorption

Implementation Method 4

reversible adsorption and desorption through pressure, humidity, and temperature swings

Methodology Applied
Scientific EffectTemperature swing: Heating

Data Source

PatentEP3191211B9Method and device for the reversible adsorption of carbon dioxide
Publication Date: 2022.06.15 SKYTREE BV
  • EP3191211B9 patent drawingFigure 1
  • EP3191211B9 patent drawingFigure 2
  • EP3191211B9 patent drawingFigure 3

AI summary

The present invention relates to a device for the reversible adsorption of carbon dioxide from a gas mixture, comprising at least one adsorbent vessel comprising one or a plurality of gas permeable cartridge vessels of an inert and dimensionally stable material, and each cartridge comprising a suitable polymeric particular adsorbent having a primary amino functionality; to an arrangement including the device, and to a method for ad- and desorption of carbon dioxide.