Amine Solvent Viscosity Reduction for Acid Gas Removal

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Solution Overview

Problem

Existing solvents for removing acid gases like hydrogen sulphide and carbon dioxide from natural gas and synthesis gas have limitations in viscosity, loading capacity, and energy consumption, which affect the efficiency and cost of gas purification processes.

Innovation Solution

A solvent composition comprising MDEA, thiodiglycol, amino ethyl piperazine, and potassium carbonate, optimized to reduce viscosity and enhance absorption kinetics, allowing for efficient removal of acid gases at high partial pressures with reduced energy consumption.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Speed

If conventional solvents are used for removing acid gases, then acid gas removal capability is achieved, but viscosity is high which reduces absorption kinetics

Engineering Contradiction:
Improveabsorption kineticsVSAvoidviscosity
Core Design Contradiction:
SpeedVSForce

Solution Approach 1:

The patent changes the chemical composition parameters of the solvent system by incorporating specific ratios of MDEA (30-45 wt%), AEP (5-10 wt%), thiodiglycol (10-25 wt%), and potassium carbonate (0.1-2.0 wt%). This parameter optimization reduces viscosity to less than 11 cP at 40°C while maintaining effective acid gas removal capability, thereby improving absorption kinetics without sacrificing removal efficiency.

Inventive Principle:
Principle #35Parameter changes

2Quantity of substance

If solvent concentration is increased to improve loading capacity, then acid gas absorption capacity increases, but viscosity increases reducing fluidity

Engineering Contradiction:
Improveloading capacityVSAvoidviscosity
Core Design Contradiction:
Quantity of substanceVSForce

Solution Approach 1:

The patent creates a composite solvent system combining multiple components (MDEA, AEP, thiodiglycol, potassium carbonate, and water) in optimized proportions. This composite formulation achieves high loading capacity for acid gases while maintaining low viscosity through synergistic interactions between components, particularly the role of thiodiglycol and potassium carbonate in reducing overall system viscosity despite high active solvent concentrations.

Inventive Principle:
Principle #40Composite materials

3Productivity

If high partial pressure conditions are used to improve absorption efficiency, then acid gas removal effectiveness increases, but energy consumption increases

Engineering Contradiction:
Improveabsorption efficiencyVSAvoidenergy consumption
Core Design Contradiction:
ProductivityVSUse of energy by moving object

Solution Approach 1:

The patent optimizes operational parameters including temperature (15-90°C) and pressure (10-150 bar) ranges for the absorption process. By maintaining the solvent at optimized composition, the system achieves high absorption efficiency even at moderate conditions, reducing the energy penalty associated with extreme pressure and temperature requirements while maintaining deep removal of CO2 and H2S.

Inventive Principle:
Principle #35Parameter changes

4Speed

If solvent composition is optimized for low viscosity, then absorption kinetics improve, but loading capacity may be reduced

Engineering Contradiction:
Improveabsorption kineticsVSAvoidloading capacity
Core Design Contradiction:
SpeedVSQuantity of substance

Solution Approach 1:

The patent employs a composite solvent formulation where MDEA provides high loading capacity through chemical absorption mechanisms, while thiodiglycol and potassium carbonate contribute to viscosity reduction. The amine activator AEP enhances the overall absorption kinetics. This composite approach allows simultaneous optimization of loading capacity, kinetics, and viscosity by leveraging the complementary properties of each component.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solvent achieves improved acid gas absorption kinetics and selectivity, reducing the overall energy consumption and operational costs by maintaining a low viscosity and efficient gas separation, enabling deep removal of CO2 and H2S without additional treatment steps.

Implementation Method 1

aqueous solution containing water, thiodiglycol, Methyl Diethanol Amine (MDEA), amine ethyl piperazine (AEP) as amine activator and potassium carbonate

Methodology Applied
Scientific EffectChemical absorption: Absorption (physical)

Implementation Method 2

an aqueous solution containing water, thiodiglycol, Methyl Diethanol Amine (MDEA)

Methodology Applied
Scientific EffectPhysical absorption: Absorption (physical)

Implementation Method 3

Additionally, this disclosure relates to an absorbent liquid, which has a more optimal viscosity and load carrying capacity, that can be used in a purification process for removal of acid gases

Methodology Applied
Scientific EffectViscosity reduction effect:

Data Source

PatentEP3247484B1Solvent and method for removing acid gases from a gaseous mixture
Publication Date: 2023.09.20 CARBON CLEAN SOLUTIONS
  • EP3247484B1 patent drawingFigure 1
  • EP3247484B1 patent drawingFigure 2
  • EP3247484B1 patent drawingFigure 3

AI summary

A solvent and method for removing carbon dioxide from a gaseous mixture flow with high carbon dioxide partial pressures are disclosed. The solvent includes a secondary or tertiary amine, an amine activator, a physical solvent (e.g., thioalkanol), and a carbonate buffer. The solvent contains less than about 60% by weight of water and is in a single liquid phase.