Lithium-Ion Anode Cyclic Compound Coating High-Temperature Stability

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Solution Overview

Problem

Current lithium ion secondary batteries face challenges in achieving superior battery characteristics, particularly in high-temperature storage conditions, where the anode configuration significantly impacts performance, and existing solutions like cyclic polyether and cryptand do not fully address the need for improved performance and stability.

Innovation Solution

Incorporating a cyclic compound with specific structures, such as the first, second, and third cyclic compounds, into the anode of lithium ion secondary batteries, which utilize metal elements and halogen atoms for coordinate bonding, allowing for efficient lithium insertion and extraction while suppressing expansion and contraction of the anode active material layer during charge and discharge.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional cyclic polyether or cryptand is used in the anode, then some battery characteristic improvement is achieved, but superior battery characteristic and stability especially under high-temperature storage conditions cannot be obtained

Engineering Contradiction:
Improvebattery characteristic stabilityVSAvoidperformance under high-temperature storage
Core Design Contradiction:
ReliabilityVSAdaptability or versatility

Solution Approach 1:

The patent employs a composite anode material comprising graphite particles coated with a specific cyclic compound containing metal elements (M1-M4) and halogen atoms (Y1-Y4). This composite structure combines the high capacity of graphite with the protective and stabilizing properties of the cyclic compound, achieving superior battery characteristics and high-temperature stability that neither material could achieve alone.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The invention modifies the chemical composition and structure of the anode by incorporating a cyclic compound with specific parameters: metal elements (M1-M4) coordinated with halogen atoms (Y1-Y4), where n1-n4 are specific integers. This parameter optimization enhances the anode's electrochemical performance and thermal stability, resolving the contradiction between general reliability and high-temperature adaptability.

Inventive Principle:
Principle #35Parameter changes

2Reliability

If the anode configuration is modified to improve battery characteristic, then performance is enhanced, but device complexity increases

Engineering Contradiction:
Improvebattery characteristicVSAvoidanode configuration complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The cyclic compound is applied as a pre-formed coating on the graphite particles before electrode assembly. This preliminary action creates a stable, protective layer that simplifies the overall manufacturing process while enhancing battery characteristics, avoiding the need for complex post-processing or multi-step anode construction.

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The use of these cyclic compounds enhances battery characteristics by improving charge-discharge efficiency, reducing electrical resistance, and maintaining high capacity retention, leading to superior performance and stability compared to batteries without these compounds.

Implementation Method 1

the cyclic compound contains one or more of a first cyclic compound represented by the following formula (1), a second cyclic compound represented by the following formula (2), and a third cyclic compound represented by the following formula (3)

Methodology Applied
Scientific EffectCoordinate bonding: Chemical Bonding

Implementation Method 2

suppressing expansion and contraction of the anode active material layer during charge and discharge

Methodology Applied
Scientific EffectExpansion and contraction: Thermal Expansion

Data Source

PatentEP3621135B1Negative electrode for lithium-ion rechargeable battery, and lithium-ion rechargeable battery
Publication Date: 2022.06.01 MURATA MFG CO LTD
  • EP3621135B1 patent drawingFigure 1
  • EP3621135B1 patent drawingFigure 2
  • EP3621135B1 patent drawingFigure 3

AI summary

A lithium ion secondary battery includes a cathode, an anode, and an electrolytic solution. The anode contains a cyclic compound and the cyclic compound contains one or more of a first cyclic compound, a second cyclic compound, and a third cyclic compound.