Metal-Ion Electrochemical Cell Capacity Regeneration via Anode Potential Derivative

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Solution Overview

Problem

Existing methods for evaluating and regenerating the capacity of metal-ion electrochemical accumulators, such as lithium-ion batteries, are not precise and easy to implement, and often require additional components or complex architectures that increase fragility and weight, while also inducing overvoltages due to incomplete charge state measurements.

Innovation Solution

A method involving the determination of the time derivative of the potential of one electrode, particularly the anode, to estimate capacity loss and facilitate spontaneous regeneration without additional terminals or imposed currents, using a regeneration component with an ionic insulation element like paraffin film that melts to enable ion exchange under controlled temperature or other parameters.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of repair

If additional terminals and imposed currents are used for capacity regeneration, then regeneration capability is improved, but device complexity and fragility increase

Engineering Contradiction:
Improvecapacity regeneration capabilityVSAvoidadditional terminals and control electronics
Core Design Contradiction:
Ease of repairVSDevice complexity

Solution Approach 1:

The battery uses its own existing terminals and internal electrochemical potential to drive the regeneration process. The anode serves dual functionality as both operational electrode and reference for regeneration, eliminating need for additional terminals. The system self-regulates through potential difference between anode and regeneration material.

Inventive Principle:
Principle #25Self-service

Solution Approach 2:

The anode is given dual functionality: it serves as the negative electrode during normal operation and as the reference electrode for capacity regeneration. The existing terminals are used for both charge/discharge operations and regeneration, making the system multi-functional without additional components.

Inventive Principle:
Principle #6Universality (Multi-functionality)

2Difficulty of detecting and measuring

If traditional capacity evaluation methods are used, then measurement is simplified, but precision and accuracy deteriorate

Engineering Contradiction:
Improvecapacity evaluation simplicityVSAvoidcapacity loss measurement accuracy
Core Design Contradiction:
Difficulty of detecting and measuringVSMeasurement precision

Solution Approach 1:

The method uses feedback from the battery's own potential measurements during charging to evaluate capacity loss. The potential difference between anode and cathode provides real-time information about state of charge and capacity degradation, enabling accurate measurement without external equipment.

Inventive Principle:
Principle #23Feedback

Solution Approach 2:

The patent replaces complex external measurement equipment with electrochemical potential measurements that are inherently available during normal battery operation. The electrochemical potential difference serves as a natural sensor for capacity evaluation.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

3Speed

If imposed currents are applied for regeneration, then regeneration speed is improved, but overvoltages and harmful effects increase

Engineering Contradiction:
Improveregeneration speedVSAvoidovervoltages and electrode degradation
Core Design Contradiction:
SpeedVSObject-generated harmful factors

Solution Approach 1:

The regeneration process is driven by the battery's own electrochemical potential difference rather than external current imposition. The anode's potential relative to the regeneration material naturally drives ion transfer, eliminating overvoltages and harmful effects associated with forced current application.

Inventive Principle:
Principle #25Self-service

Solution Approach 2:

The method changes the driving parameter from external current to internal electrochemical potential. By utilizing the natural potential difference between electrodes and regeneration material, the system achieves regeneration without the harmful side effects of imposed currents.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach allows for precise evaluation and regeneration of accumulator capacity, reducing the need for complex electronics and additional terminals, and prevents overvoltages by enabling spontaneous ion insertion without current imposition, thus extending battery life and efficiency.

Implementation Method 1

an ionic insulation element like paraffin film that melts to enable ion exchange under controlled temperature or other parameters

Methodology Applied
Scientific EffectMelting: Melting

Implementation Method 2

determination of the time derivative of the potential of one electrode, particularly the anode, to estimate capacity loss and facilitate spontaneous regeneration without additional terminals or imposed currents

Methodology Applied
Scientific EffectIon insertion: Ion Exchange

Data Source

PatentEP3319150B1Method for regenerating the capacity of a metal-ion electrochemical cell
Publication Date: 2022.07.06 COMMISSARIAT A LENERGIE ATOMIQUE ET AUX ENERGIES ALTERNATIVES
  • EP3319150B1 patent drawingFigure 1~4
  • EP3319150B1 patent drawingFigure 5A~6C
  • EP3319150B1 patent drawingFigure 7

AI summary

The present invention relates to a method for evaluating the quantity of exchangeable metal ions in a metal-ion electrochemical accumulator, for the purpose of capacity regeneration, the method comprising determining the time derivative of the potential of one of the two electrodes.