Antimicrobial Phase-Separable Glass Polymer Composite Surface Treatment

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Solution Overview

Problem

Existing polymer/glass composite articles demonstrate limited antimicrobial efficacy due to insufficient surface concentration and duration of antimicrobial agents, necessitating the development of durable antimicrobial composite articles with controlled antimicrobial activity that do not require activation.

Innovation Solution

A composite article comprising a polysulfone matrix with phase-separable glass particles containing copper-containing antimicrobial agents, where the particles are distributed at a specific volume fraction to ensure effective antimicrobial activity, and surface treatment methods like hand-sanding and plasma treatment are employed to enhance exposure and efficacy.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If polymer/glass composite articles are used to provide antimicrobial properties, then antimicrobial activity is achieved, but the antimicrobial efficacy is insufficient due to low surface concentration of antimicrobial agents

Engineering Contradiction:
Improveantimicrobial efficacyVSAvoidsurface concentration of antimicrobial agents
Core Design Contradiction:
ReliabilityVSQuantity of substance

Solution Approach 1:

The patent applies local quality by creating a phase-segregated structure where copper-containing glass particles are concentrated at the composite surface rather than uniformly distributed throughout the bulk material. This phase separation ensures high local concentration of antimicrobial agents at the surface, directly addressing the insufficient surface concentration problem while maintaining overall composite integrity

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The patent uses composite materials by combining polymer matrix with copper-containing glass particles to create a multi-phase composite structure. The glass particles serve as reservoirs for copper antimicrobial agents, and the phase separation mechanism ensures these agents are positioned at the surface, achieving both structural integrity and antimicrobial functionality

Inventive Principle:
Principle #40Composite materials

2Duration of action of stationary object

If copper-containing glass particles are distributed throughout the composite, then antimicrobial agents are provided, but the duration of antimicrobial action is insufficient

Engineering Contradiction:
Improveduration of antimicrobial actionVSAvoidantimicrobial efficacy
Core Design Contradiction:
Duration of action of stationary objectVSReliability

Solution Approach 1:

The patent applies preliminary action by pre-positioning copper-containing glass particles within the polymer matrix during composite fabrication. These particles are strategically distributed and phase-separated to the surface beforehand, creating a reservoir of antimicrobial agents that will be gradually released over time, ensuring both initial efficacy and sustained long-term action

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The patent achieves continuity of useful action through the phase-separated structure where copper-containing glass particles continuously release antimicrobial copper ions at the surface. This creates a sustained gradient of copper concentration that maintains antimicrobial efficacy over extended periods, preventing microbial regrowth without requiring reapplication

Inventive Principle:
Principle #20Continuity of useful action

3Quantity of substance

If the exterior surface is treated to expose more glass particles, then surface concentration of antimicrobial agents is increased, but the structural integrity may be compromised

Engineering Contradiction:
Improvesurface concentration of antimicrobial agentsVSAvoidstructural integrity
Core Design Contradiction:
Quantity of substanceVSStrength

Solution Approach 1:

The patent applies phase transitions by utilizing the phase separation behavior of copper-containing glass particles within the polymer matrix. During processing or service, these particles naturally segregate to the surface phase, increasing surface concentration of antimicrobial agents without requiring aggressive surface treatments that would compromise structural integrity. The phase transition is controlled and preserves composite strength

Inventive Principle:
Principle #36Phase transitions

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The composite articles achieve significant log reductions in bacteria and viruses, maintaining antimicrobial efficacy for extended periods without external activation, demonstrating improved durability and effectiveness compared to traditional copper oxide-based composites.

Implementation Method 1

a plurality of second phase particles comprising a phase-separable glass with a copper-containing antimicrobial agent

Methodology Applied
Scientific EffectPhase separation:

Implementation Method 2

ensure that the microbes present on the surfaces of such article are in residence for a sufficient duration to be killed or neutralized by the antimicrobial agents within the composite articles

Methodology Applied
Scientific EffectAntimicrobial action:

Data Source

PatentEP3987934B1Antimicrobial phase-separable glass/polymer composite articles and methods for making the same
Publication Date: 2023.11.22 CORNING INC
  • EP3987934B1 patent drawingFigure 1~1A
  • EP3987934B1 patent drawingFigure 1B
  • EP3987934B1 patent drawingFigure 2~3

AI summary

A method of making an antimicrobial composite article, including the steps: providing a matrix comprising a polymeric material; providing a plurality of second phase particles comprising an antimicrobial agent; melting the matrix to form a matrix melt; distributing the plurality of second phase particles in the matrix melt at a second phase volume fraction to form a composite melt; forming a composite article from the composite melt; and treating the composite article to form an antimicrobial composite article having an exterior surface comprising an exposed portion of the matrix and the plurality of second phase particles. The distributing step can employ an extrusion process. The forming a composite article step can employ an injection molding process. The treating step can employ abrading and plasma-treating the article to define the exterior surface.