Antireflective Coating Composition Phase Separation

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Solution Overview

Problem

Existing anti-reflection films require complex multi-layer manufacturing processes and suffer from weak interfacial adhesion, leading to delamination issues, and existing single-coating solutions struggle with phase separation and functionality.

Innovation Solution

An anti-reflective coating composition comprising hollow particles coated with a fluorine-based compound, a photopolymerizable compound, and a solvent, which allows for smooth phase separation into multiple layers during a single coating process, enhancing interfacial bonding and scratch resistance.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If a multi-layer structure (hard coat layer, high refractive index layer, low refractive index layer) is used, then anti-reflection performance is improved, but manufacturing process complexity increases

Engineering Contradiction:
Improveanti-reflection performanceVSAvoidmanufacturing process complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The patent combines multiple functional layers (hard coat layer and low refractive index layer) into a single coating composition that can be applied in one wet coating process. The composition contains polymer resin, inorganic particles for hardness, and hollow particles for low refractive index, all integrated in one formulation that phase-separates during drying to form the multi-layer structure automatically.

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The single coating composition is designed to phase-separate into distinct layers during the drying process. The inorganic particles and hollow particles separate into different regions, forming a multi-layer structure with a hard coat layer containing inorganic particles and a low refractive index layer containing hollow particles, achieving layer segmentation without multiple coating steps.

Inventive Principle:
Principle #1Segmentation

2Ease of manufacture

If a wet method with separate processes for each layer is used, then manufacturing cost is reduced, but interfacial adhesion deteriorates

Engineering Contradiction:
Improvemanufacturing costVSAvoidinterfacial adhesion
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent merges multiple coating processes into a single wet coating step by formulating a unified composition containing all necessary components (polymer resin, inorganic particles, hollow particles). This single coating process eliminates the need for separate processes for each layer, reducing manufacturing complexity while maintaining strong interfacial adhesion throughout the film structure.

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The coating composition is a composite material containing polymer resin as binder, inorganic particles for hardness, and hollow particles for low refractive index. This composite structure allows all functional components to be integrated in one layer that phase-separates during drying, achieving both cost reduction and strong interfacial adhesion.

Inventive Principle:
Principle #40Composite materials

3Productivity

If a single coating process is used, then manufacturing process is simplified, but phase separation is not smooth leading to functional deterioration

Engineering Contradiction:
Improvemanufacturing process simplificationVSAvoidphase separation quality
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The patent carefully controls composition parameters including the types and amounts of polymer resin, inorganic particles, and hollow particles. By adjusting these parameters, the composition achieves optimal phase separation behavior during drying, forming distinct layers with proper functional distribution. The refractive index and surface energy of components are specifically selected to facilitate smooth phase separation.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The single coating composition is designed with components that have different local properties - inorganic particles for hardness in the hard coat layer, hollow particles for low refractive index in the low refractive index layer. During phase separation, these components automatically distribute to appropriate regions based on their physical and chemical properties, achieving local quality differentiation without multiple coating steps.

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution enables the formation of a film with excellent scratch resistance and anti-reflection properties through a simplified manufacturing process, minimizing delamination and improving reflectivity reduction.

Implementation Method 1

hollow particles coated with a fluorine-based compound having refractive index of 1.3∼1.4

Methodology Applied
Scientific EffectRefraction: Refraction

Implementation Method 2

surface tension of 10∼25 mN/m on the surface

Methodology Applied
Scientific EffectSurface tension: Surface Tension

Implementation Method 3

a photopolymerizable compound, a photopolymerization initiator

Methodology Applied
Scientific EffectPhotopolymerization: Photopolymerisation

Data Source

PatentEP2557130B1Antireflective coating composition, antireflective film, and preparation method thereof
Publication Date: 2016.09.28 LG CHEM LTD

AI summary

This disclosure relates to an anti-reflective coating composition that is divided into at least two layers through phase separation after monolayer coating, more particularly an anti-reflective coating composition comprising hollow particles coated with a fluorine-based compound having refractive index of 1.3~1.4 and surface tension of 10-25 mN/m on the surface, an anti-reflection film manufactured therefrom, and a method of manufacturing the same. In the anti-reflective coating composition of the present invention, at least two layers may be spontaneously formed only by single coating due to smooth phase separation in the coating layer. Particularly, since an interface of each layer formed by phase separation is substantially chemically bonded or crosslinked, delamination of each layer may be minimized. And, a film with excellent scratch resistance and anti-reflection may be manufactured by a more simplified method using the anti-reflective coating composition of the present invention.