Aqueous Inkjet Ink Colloidal Stability via Resin Mediators

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Solution Overview

Problem

White inks in inkjet color sets face challenges due to early sedimentation of titanium oxide nanoparticles, leading to colloidal instability, short shelf-life, and reduced print opacity, which affects jetting performance and substrate coating.

Innovation Solution

The development of aqueous inkjet ink compositions that include a solvent system comprising water, specific organic solvents, and resin particles, which enhances colloidal stability, jetting performance, and opacity, while maintaining durability and water-fastness on various substrates.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Speed

If titanium oxide nanoparticles are used in low viscosity aqueous mixtures, then jetting performance is improved, but colloidal stability deteriorates leading to early sedimentation

Engineering Contradiction:
Improvejetting performanceVSAvoidcolloidal stability
Core Design Contradiction:
SpeedVSStability of the object's composition

Solution Approach 1:

The patent introduces resin particles as intermediary components that interact with titanium oxide nanoparticles through surface forces. These resin particles act as mediators that prevent direct nanoparticle aggregation and sedimentation, while maintaining the low viscosity required for jetting performance. The resin particles create a stabilizing matrix that keeps nanoparticles dispersed without requiring high viscosity binders.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The invention creates a composite inkjet ink system combining titanium oxide nanoparticles with specific resin particles in an aqueous medium. This composite formulation leverages the high opacity of titanium oxide while using the resin component to provide colloidal stability. The synergistic interaction between the nanoparticle and resin phases enables both jetting performance and long-term stability that neither component could achieve alone.

Inventive Principle:
Principle #40Composite materials

2Illumination intensity

If white pigment concentration is increased to improve opacity, then print quality is improved, but sedimentation rate increases reducing shelf-life

Engineering Contradiction:
ImproveopacityVSAvoidshelf-life
Core Design Contradiction:
Illumination intensityVSDuration of action of stationary object

Solution Approach 1:

Resin particles serve as intermediary structures that surround and stabilize titanium oxide nanoparticles even at high concentrations. The resin-nanoparticle interactions prevent aggregation and sedimentation, allowing the formulation to maintain high opacity through increased pigment loading without sacrificing shelf-life. The resin matrix acts as a protective intermediary that keeps nanoparticles uniformly dispersed.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent optimizes the concentration ratios of titanium oxide nanoparticles to resin particles, and adjusts the size parameters of both components. By controlling the size distribution and concentration parameters within specific ranges, the formulation achieves maximum opacity while maintaining colloidal stability and extended shelf-life, resolving the trade-off between pigment loading and sedimentation resistance.

Inventive Principle:
Principle #35Parameter changes

3Ease of manufacture

If standard aqueous formulations are used, then manufacturing simplicity is maintained, but coating uniformity and water-fastness are insufficient

Engineering Contradiction:
Improveformulation simplicityVSAvoidcoating uniformity
Core Design Contradiction:
Ease of manufactureVSManufacturing precision

Solution Approach 1:

The invention develops a composite aqueous formulation combining titanium oxide nanoparticles with specifically selected resin particles. This composite approach enhances coating uniformity and water-fastness through the synergistic interaction between components, while maintaining relative manufacturing simplicity. The resin particles provide film-forming properties and adhesion that improve coating quality without requiring complex processing steps.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent employs resin particles with specific local properties (size, surface characteristics, composition) that are optimized for interaction with titanium oxide nanoparticles. This local optimization of resin particle characteristics enhances coating uniformity and durability in specific application areas, allowing the formulation to achieve superior performance while maintaining ease of manufacture through a relatively simple two-component system.

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The ink compositions exhibit excellent colloidal stability, extended latency and decap time, high opacity, and improved coating properties, ensuring consistent and high-quality print performance.

Implementation Method 1

exhibit excellent colloidal stability and jetting performance, extended latency and decap time

Methodology Applied
Scientific EffectColloidal stability: Colloid

Implementation Method 2

One obstacle is early sedimentation of white pigment (generally titanium oxide nanoparticles) and lack of long-term colloidal stability

Methodology Applied
Scientific EffectSedimentation: Sedimentation

Implementation Method 3

In low viscosity mixtures, such as aqueous inkjet ink compositions

Methodology Applied
Scientific EffectViscosity modification:

Implementation Method 4

They also exhibit excellent coating properties, including uniform film-formation, wetting and spread

Methodology Applied
Scientific EffectSurface tension: Surface Tension

Implementation Method 5

white pigment (generally titanium oxide nanoparticles) have a very high density

Methodology Applied
Scientific EffectLight scattering: Scattering

Implementation Method 6

high opacity

Methodology Applied
Scientific EffectLight absorption: Absorption (EM radiation)

Implementation Method 7

excellent coating properties, including uniform film-formation, wetting and spread

Methodology Applied
Scientific EffectCapillary action: Capillary Action

Implementation Method 8

durability and water-fastness on a variety of substrates

Methodology Applied
Scientific EffectAdhesion: Adhesive

Data Source

PatentUS11781025B2Aqueous inkjet ink compositions
Publication Date: 2023.10.10 XEROX CORP

AI summary

Aqueous inkjet ink compositions are provided. In an embodiment, such an aqueous inkjet ink composition comprises a solvent system comprising water, a first organic solvent, and a second organic solvent, wherein the second organic solvent is an alkanediol having from 2 to 8 carbon atoms and the second organic solvent is present at an amount of from greater than 0 weight % to about 8 weight %; a white pigment; and resin particles. Methods of making and using the aqueous inkjet ink compositions are also provided.