Aryl Siloxane Encapsulants for LED Heat Stability

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Solution Overview

Problem

Aryl group-containing siloxane compositions used in light emitting devices discolor at temperatures above 170°C, leading to reduced light output and altered color, due to oxidation of aryl components forming chromophores.

Innovation Solution

Incorporating an alkaline earth metal into the aryl group-containing siloxane compositions during formation, which reduces discoloration at high temperatures without altering curing conditions or affecting physical properties, making them suitable for use as encapsulating layers in light emitting devices.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If aryl group-containing siloxane compositions are used in light emitting devices, then light transmission and barrier properties are provided, but discoloration occurs at temperatures above 170°C due to oxidation of aryl components

Engineering Contradiction:
Improveheat stabilityVSAvoiddiscoloration
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

An alkaline earth metal compound acts as an intermediary substance between the aryl group-containing siloxane composition and oxygen, preventing oxidation of the aryl components. The metal compound serves as a sacrificial agent that reacts with oxygen or radical species before they can oxidize the aryl groups, thereby preventing chromophore formation and discoloration while maintaining the encapsulant's light transmission and barrier properties

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The invention converts the harmful oxidation reaction into a beneficial protective mechanism by introducing alkaline earth metal compounds that preferentially react with oxygen and radical species. The metal compounds undergo oxidation themselves, sacrificing their stability to protect the aryl groups from oxidation. This transforms the potential harm of high-temperature oxidation into a protective effect where the metal compound absorbs the oxidative stress

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

2Illumination intensity

If conventional encapsulating layers are used to protect LEDs, then physical protection is provided, but discoloration reduces light output and alters color

Engineering Contradiction:
Improvelight outputVSAvoiddiscoloration
Core Design Contradiction:
Illumination intensityVSObject-generated harmful factors

Solution Approach 1:

The alkaline earth metal compounds convert the harmful discoloration effect into a beneficial protective mechanism. By sacrificing their own stability through preferential oxidation reactions, these compounds prevent the oxidation of aryl groups that would otherwise form chromophores and reduce light output. The metal compounds absorb oxidative stress, maintaining the encapsulant's optical properties including light transmission and color rendering

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Solution Approach 2:

The alkaline earth metal compounds serve as intermediary substances between the aryl group-containing siloxane composition and oxidative environments. These metal compounds intercept oxygen and radical species, preventing them from attacking the aryl groups. This intermediary action preserves the encapsulant's illumination intensity and color properties by blocking the oxidation pathway before chromophores can form

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The inclusion of alkaline earth metal stabilizes the siloxane compositions at high temperatures, maintaining consistent light transmission and barrier properties, ensuring effective protection of LEDs while preventing discoloration.

Implementation Method 1

discolor at temperatures above 170°C, leading to reduced light output and altered color, due to oxidation of aryl components forming chromophores

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 2

the reaction product of: (A) an organopolysiloxane having at least two alkenyl groups per molecule; (B) an organopolysiloxane having at least two silicon-bonded hydrogen atoms per molecule; and (C) a heat stabilizing composition comprising an alkaline earth metal; in the presence of (D) a hydrosilylation catalyst

Methodology Applied
Scientific EffectHydrosilylation: Chemical Bonding

Data Source

PatentUS9550866B2Aryl group-containing siloxane compositions including alkaline earth metal
Publication Date: 2017.01.24 DOW TORAY CO LTD

AI summary

An aryl group-containing siloxane composition is formed by introducing an alkaline earth-metal as a part of the reaction product of an organopolysiloxane having at least two alkenyl groups per molecule and an organopolysiloxane having at least two silicon-bonded hydrogen atoms per molecule in the presence of a hydrosilylation catalyst, wherein at least one of the organopolysiloxanes includes an aryl group. The alkaline earth metal may be introduced via a heat stability composition or may alternatively be pre-reacted with the organopolysiloxane having at least two alkenyl groups per molecule. The aryl group-containing siloxane compositions may be utilized as an encapsulating layer for a light emitting device.