ASA Emulsion Particle Size Control via Dilution

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Solution Overview

Problem

The existing process for manufacturing an emulsion of alkenyl succinic anhydride (ASA) in an aqueous solution of cationic starchy material results in unstable particle size distribution over time, deviating from the optimal range of 1 µm to 1.5 µm, which is crucial for effective hydrophobization and bonding properties in paper production.

Innovation Solution

The process involves producing an aqueous solution of cationic starchy material with a dry matter content between 7% and 12%, mixing ASA with it to achieve a dry weight ratio of less than 1, emulsifying in a single pass without recirculation, and diluting the emulsion by a factor of 1.5 to 3.5 to stabilize the particle size.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Object-affected harmful factors

If the emulsion is manufactured without temperature increase, then hydrolysis of ASA is avoided, but the particle size distribution becomes unstable over time

Engineering Contradiction:
Improvehydrolysis of ASAVSAvoidparticle size distribution stability
Core Design Contradiction:
Object-affected harmful factorsVSStability of the object's composition

Solution Approach 1:

The patent changes the concentration parameter by diluting the emulsion to specific ranges (0.5-5% cationic starch, 0.05-0.5% ASA) to stabilize particle size distribution. This parameter adjustment prevents particle aggregation while maintaining emulsion stability during storage and paper machine operations.

Inventive Principle:
Principle #35Parameter changes

2Reliability

If coarse particles are present in the emulsion, then hydrophobization properties are improved, but clogging of paper machine materials and steam entrainment occur

Engineering Contradiction:
Improvehydrophobization propertiesVSAvoidclogging and steam entrainment
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

The patent optimizes the particle size parameter by controlling emulsion concentration and composition to achieve a narrow size distribution centered around 1-2 µm. This parameter control ensures particles are fine enough to avoid clogging and steam entrainment while maintaining sufficient hydrophobization effectiveness.

Inventive Principle:
Principle #35Parameter changes

3Object-generated harmful factors

If fine particles are used in the emulsion, then clogging is prevented, but particles pass through the fibrous mat and are lost in process water

Engineering Contradiction:
Improveclogging preventionVSAvoidparticle loss in process water
Core Design Contradiction:
Object-generated harmful factorsVSLoss of substance

Solution Approach 1:

The patent identifies and applies an optimal particle size range (1-2 µm average diameter) that balances two opposing requirements: fine enough to prevent clogging of machinery, yet coarse enough to be retained by the fibrous mat during paper formation. This optimal parameter range maximizes particle utilization while preventing both clogging and loss.

Inventive Principle:
Principle #35Parameter changes

4Ease of manufacture

If the emulsion particle size is not centered on 1 µm to 1.5 µm, then manufacturing is easier, but bonding effectiveness and hydrophobic properties are reduced

Engineering Contradiction:
Improveemulsion production flexibilityVSAvoidparticle size control
Core Design Contradiction:
Ease of manufactureVSManufacturing precision

Solution Approach 1:

The patent establishes specific parameter ranges for emulsion concentration (0.5-5% cationic starch, 0.05-0.5% ASA) that naturally produce the desired particle size distribution (1-2 µm average) through the emulsification process. These parameter specifications make the precision particle size control achievable through straightforward manufacturing adjustments.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach ensures a stable particle size distribution of the emulsion over extended periods, maintaining optimal hydrophobization properties and preventing clogging issues, while avoiding the risks of hydrolysis and particle loss during paper machine shutdowns.

Implementation Method 1

the function of such compositions is to avoid the coalescence of the ASA particles by positive ionization of the surface of the particles

Methodology Applied
Scientific EffectIonization: Ionisation

Implementation Method 2

this allows good contact between the ASA and the cellulose fibers. The emulsion in question is an emulsion of ASA in an aqueous solution of cationic starchy material

Methodology Applied
Scientific EffectEmulsion: Emulsion

Data Source

PatentEP2904146B1Process for producing a stable emulsion of alkenyl succinic anhydride (ASA) in an aqueous solution of cationic amylaceous material, emulsion obtained and use thereof
Publication Date: 2017.07.05 ROQUETTE FRERES SA

AI summary

The present invention relates to a method for producing an emulsion of alkenyl succinic anhydride (ASA) in an aqueous solution of cationic amylaceous material; this process does not implement a loop for recirculating the product at the level of the emulsifying unit, and performs a dilution of the emulsion once the latter has been produced; a product which has a particle size that is simultaneously fine, monodisperse and stable over time is achieved. An effective process which is simple to implement, in particular on a paper production site, for providing an emulsion which may be stored during the periods when the paper machine is stopped for cleaning or maintenance operations, is thus provided.