Triacylglyceride Oil Purification With Auxiliary-Agent Crystallization

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Solution Overview

Problem

Existing methods are inadequate for effectively removing chlorinated precursors of monochloropropandiol esters (MCPDEs) during the oil refining process, which can lead to the formation of potentially harmful compounds like 3-MCPD esters, posing a challenge to the plant oil refining industry and requiring oils with high 3-MCPD content to be discarded.

Innovation Solution

A method involving the use of auxiliary agents with different melting points and higher polarity than the triacylglyceride oils to trap and separate chlorinated substances by crystallization, reducing the availability of chlorine donors during refining, thereby minimizing the formation of MCPD esters.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If chlorination of acylglycerides is performed at high temperatures during oil refining, then the oil refining process can be completed, but chlorinated contaminants such as MCPD esters are formed

Engineering Contradiction:
Improveoil refining process completionVSAvoidMCPD ester formation
Core Design Contradiction:
ProductivityVSObject-generated harmful factors

Solution Approach 1:

The patent applies preliminary action by removing chlorinated precursors from the oil before the high-temperature refining process. This is achieved through crystallization of auxiliary agents that trap these precursors, preventing them from acting as chlorine donors during subsequent deodorization and refining steps, thus eliminating MCPD ester formation while maintaining productive refining operations

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The patent uses auxiliary agents as intermediaries to trap chlorinated precursors. These auxiliary agents act as mediators between the chlorinated substances and the oil matrix, sequestering the harmful precursors in a separate crystalline phase that can be removed, thereby protecting the oil from contamination during high-temperature processing

Inventive Principle:
Principle #24Intermediary (Mediator)

2Device complexity

If chlorinated precursors are not removed before deodorisation, then the refining process is simpler, but chlorine donors are available to generate MCPD esters

Engineering Contradiction:
Improverefining process simplicityVSAvoidMCPD ester generation
Core Design Contradiction:
Device complexityVSObject-generated harmful factors

Solution Approach 1:

The patent performs preliminary removal of chlorinated precursors through crystallization of auxiliary agents before the deodorization step. This preliminary action eliminates the chlorine donor pool without adding complex chemical treatment steps, maintaining process simplicity while preventing MCPD ester generation during the subsequent deodorization operation

Inventive Principle:
Principle #10Preliminary action

3Object-generated harmful factors

If auxiliary trapping agents are used to remove chlorinated precursors, then MCPD ester formation is reduced, but additional crystallization and separation steps are required

Engineering Contradiction:
ImproveMCPD ester reductionVSAvoidcrystallization and separation steps
Core Design Contradiction:
Object-generated harmful factorsVSDevice complexity

Solution Approach 1:

The patent utilizes parameter changes by exploiting differences in melting points and polarity between the auxiliary trapping agents and the oil components. By selecting auxiliary agents with specific physical parameters (lower melting point, higher polarity), the system achieves selective crystallization and phase separation, enabling effective MCPD ester reduction through physically-based parameter differentiation rather than complex chemical processes

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method significantly reduces the quantity of chlorinated precursors in refined oils, allowing for lower temperature deodorization and minimizing trans-fatty acid formation, resulting in oils with low or no MCPDEs, suitable for various refining practices.

Implementation Method 1

The trapped chlorinated substances may then be physically separated by crystallising either the auxiliary agents from the oil or vice versa

Methodology Applied
Scientific EffectSolubilization: Solvation

Implementation Method 2

The trapped chlorinated substances may then be physically separated by crystallising either the auxiliary agents from the oil or vice versa

Methodology Applied
Scientific EffectCrystallization: Crystallisation

Implementation Method 3

separating solid and liquid phases of the product of step (b)

Methodology Applied
Scientific EffectPhase separation: Phase Change

Data Source

PatentEP3764803B1Purification of triacylglyceride oils
Publication Date: 2025.10.01 SOCIETE DES PRODUITS NESTLE SA
  • EP3764803B1 patent drawingFigure 1
  • EP3764803B1 patent drawingFigure 2
  • EP3764803B1 patent drawingFigure 3

AI summary

A method for purification of a triacylglyceride oil comprising the steps: (a) admixing the triacylglyceride oil with an auxiliary trapping agent, wherein the melting temperatures of the triacylglyceride oil and the auxiliary trapping agent are substantially different, wherein the auxiliary trapping agent is soluble in the triacylglyceride oil, and wherein the auxiliary trapping agent is more polar than the triacylglyceride oil; (b) (i) crystallising the auxiliary trapping agent by cooling the mixture of step (a) below the melting temperature of the auxiliary trapping agent, wherein the auxiliary trapping agent has a higher melting temperature than the triacylglyceride oil; or (ii) crystallising the triacylglyceride oil by cooling the mixture of step (a) below the melting 10 temperature of the triacylglyceride oil, wherein the triacylglyceride oil has a higher melting temperature than the auxiliary trapping agent; and (c) separating solid and liquid phases of the product of step (b).