Azeotropic Distillation Reactant as Entrainer

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Solution Overview

Problem

Current azeotropic distillation methods for producing allyl alcohol require high energy consumption without significantly improving separation performance, necessitating a reduction in energy usage without compromising separation efficiency.

Innovation Solution

Supplying a portion of the reactant as an azeotropic entrainer in the distillation step, where the reactant acts as both a reactant and an entrainer, enhancing separation performance and reducing energy consumption by minimizing the mixing of high-boiling components and water load.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Use of energy by moving object

If conventional azeotropic distillation is used for separating allyl alcohol from reaction products, then separation is achieved, but energy consumption is high

Engineering Contradiction:
Improveenergy consumptionVSAvoidseparation performance
Core Design Contradiction:
Use of energy by moving objectVSReliability

Solution Approach 1:

The reactant (allyl acetate) serves dual functions: as a reactant in the hydrolysis reaction and as an azeotropic entrainer in the distillation process. This self-service approach eliminates the need for separate entrainer addition and reduces energy consumption while maintaining effective separation performance.

Inventive Principle:
Principle #25Self-service

Solution Approach 2:

The patent applies multi-functionality by having the reactant (allyl acetate) perform two roles simultaneously: participating in the hydrolysis reaction to produce allyl alcohol and acting as an azeotropic entrainer to facilitate water separation during distillation. This dual role reduces overall process complexity and energy requirements.

Inventive Principle:
Principle #6Universality (Multi-functionality)

2Productivity

If all reactant is supplied to the reaction step, then reaction efficiency is maximized, but separation performance in distillation is insufficient

Engineering Contradiction:
Improvereaction efficiencyVSAvoidseparation performance
Core Design Contradiction:
ProductivityVSReliability

Solution Approach 1:

The patent changes the operational parameter by supplying a portion (1-10 mass%, preferably 3-8 mass%) of the reactant to the distillation column as an azeotropic entrainer rather than directing all reactant to the reaction step. This parameter adjustment optimizes both reaction efficiency and separation performance simultaneously.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach improves separation performance in azeotropic distillation while reducing energy consumption, specifically by recycling a high percentage of unreacted reactant as an entrainer, thereby lowering the energy required for the distillation process.

Implementation Method 1

An azeotropic phenomenon takes place in a combination of two or more components which may provide a maximum azeotropic point or a minimum azeotropic point. In an 'azeotropic distillation' utilizing the azeotropic phenomenon, when a substance (generally called an 'entrainer' or 'auxiliary agent') capable of forming an azeotropic mixture with at least one of any of at least two substances

Methodology Applied
Scientific EffectAzeotropic phenomenon:

Implementation Method 2

a distillation step for separating and refining (or purifying) reaction product(s)

Methodology Applied
Scientific EffectDistillation: Distillation

Data Source

PatentEP1981833B1Azeotropic distillation method
Publication Date: 2014.04.02 RESONAC HOLDINGS CORP
  • EP1981833B1 patent drawingFigure 1~2
  • EP1981833B1 patent drawingFigure 3~4
  • EP1981833B1 patent drawingFigure 5~6

AI summary

An azeotropic distillation method, comprising a reaction step, a distillation step for separating and refining a reaction product, and a recovery step for collecting a reactant after the distillation step; wherein at least one component constituting the reactant in the reaction step can act as an entrainer for the azeotropic distillation in the distillation step; and a portion of the reactant capable of acting as the entrainer is supplied to the distillation step.