Azeotropic Composition for Trifluoropropyne Separation

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

The existing processes for producing 2,3,3-tetrafluoropropene suffer from significant losses of the desired product during purification due to the close boiling points of 2,3,3-tetrafluoropropene and light organic impurities like trifluoropropyne, leading to reduced overall yield.

Innovation Solution

An azeotropic or quasi-azeotropic composition comprising hydrochloric acid and trifluoropropyne is used to facilitate the separation of 2,3,3-tetrafluoropropene from trifluoropropyne by forming an azeotropic or quasi-azeotropic mixture with hydrochloric acid, allowing for effective distillation and minimizing the loss of 2,3,3-tetrafluoropropene.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If a distillation column is used to separate light organic impurities like trifluoropropyne from 2,3,3,3-tetrafluoropropene, then the desired product can be purified, but significant losses of the desired product occur due to the close boiling points of the two compounds

Engineering Contradiction:
Improvepurity of 2,3,3,3-tetrafluoropropeneVSAvoidloss of 2,3,3,3-tetrafluoropropene
Core Design Contradiction:
Manufacturing precisionVSLoss of substance

Solution Approach 1:

The patent uses hydrofluoric acid as an intermediary substance that selectively reacts with trifluoropropyne to form a fluoroformate intermediate. This mediator enables selective transformation of the impurity without affecting the desired product, resolving the contradiction between purification and product loss caused by close boiling points.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent changes the chemical parameter of the impurity by reacting it with hydrofluoric acid to form a fluoroformate with different physical properties. This parameter change (chemical transformation) allows subsequent separation based on the new properties rather than relying on distillation of the original compounds with close boiling points.

Inventive Principle:
Principle #35Parameter changes

2Manufacturing precision

If intermediate distillation is performed to remove light organic impurities, then the purity of the desired product is improved, but the overall yield of the process is reduced due to product loss

Engineering Contradiction:
Improvepurity of 2,3,3,3-tetrafluoropropeneVSAvoidoverall yield of the process
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

Hydrofluoric acid serves as a mediator that selectively targets the impurity for chemical transformation. This intermediary approach enables purification while preserving the majority of the desired product, thereby maintaining both high purity and overall yield.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

By changing the chemical state of the impurity through reaction with hydrofluoric acid, the process enables selective removal without the need for energy-intensive distillation that causes product loss, thus preserving both purity and productivity.

Inventive Principle:
Principle #35Parameter changes

3Manufacturing precision

If hydrochloric acid is separated from reaction products via distillation, then hydrochloric acid can be recovered without fluorinated impurities, but the process becomes complex and time-consuming

Engineering Contradiction:
Improvepurity of recovered hydrochloric acidVSAvoidcomplexity of separation process
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The patent extracts and removes fluorinated impurities from the hydrochloric acid stream through selective chemical reaction. This extraction approach simplifies the overall separation process by eliminating the need for complex multi-stage distillation systems while achieving high purity hydrochloric acid recovery.

Inventive Principle:
Principle #2Taking out (Extraction)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The use of the azeotropic composition significantly reduces the amount of trifluoropropyne in the purified 2,3,3-tetrafluoropropene stream, minimizing losses and improving the overall yield by effectively separating the two compounds with close boiling points.

Implementation Method 1

An azeotropic or quasi-azeotropic composition comprising hydrochloric acid and trifluoropropyne is used to facilitate the separation of 2,3,3-tetrafluoropropene from trifluoropropyne by forming an azeotropic or quasi-azeotropic mixture with hydrochloric acid, allowing for effective distillation

Methodology Applied
Scientific EffectAzeotropic distillation: Distillation

Data Source

PatentEP3423427B1Azeotropic or quasi-azeotropic composition comprising trifluoropropyne
Publication Date: 2020.01.01 ARKEMA FRANCE SA

AI summary

The invention relates to an azeotropic or quasi-azeotropic composition comprising hydrochloric acid and trifluoropropyne. The invention also relates to a method for separating 2,3,3,3-tetrafluoropropene and trifluoropropyne from a composition A containing 2,3,3,3-tetrafluoropropene and trifluoropropyne, said method comprising the steps of bringing said composition A into contact with an inorganic compound in order to form a composition B; and distilling composition B in order to from a first flow B1 containing trifluoropropyne and the inorganic compound, and a second flow B2 containing 2,3,3,3-tetrafluoropropene.