Barrier Film Refractive Index Stack for Humidity-Stable Color

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Solution Overview

Problem

Liquid crystal display devices using quantum dots in wavelength conversion sheets experience color instability due to changes in spectral transmission spectra caused by swelling of organic coating layers in high humidity environments, affecting the color purity and quality of the display.

Innovation Solution

A barrier film comprising specific refractive index relationships and layer configurations, including inorganic oxide and organic coating layers, is applied to wavelength conversion sheets to maintain color stability by controlling the spectral transmission spectrum.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If a barrier film with organic coating layer is used to protect quantum dot-containing layer, then protection against moisture and oxygen is improved, but color stability deteriorates due to swelling in high humidity environments

Engineering Contradiction:
Improveprotection of quantum dot-containing layerVSAvoidcolor stability
Core Design Contradiction:
ReliabilityVSStability of the object's composition

Solution Approach 1:

The patent applies parameter changes by precisely controlling the thickness of the organic coating layer (70-480 nm) and the optical path difference (Expression 1: d1 = (nB×tB + nD×tD)/λ0) to compensate for swelling effects. By optimizing these parameters, the barrier film maintains both protective function and color stability despite humidity-induced swelling.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses a composite barrier film structure combining inorganic oxide layers (Al2O3, SiO2, TiO2) with organic coating layers. This composite structure provides both moisture/oxygen barrier properties from the inorganic layers and controlled optical properties from the organic layers, resolving the contradiction between protection and color stability.

Inventive Principle:
Principle #40Composite materials

2Reliability

If the thickness of organic coating layer is increased to improve barrier properties, then protection against moisture and oxygen is improved, but color accuracy deteriorates due to excessive swelling

Engineering Contradiction:
Improvebarrier propertyVSAvoidcolor accuracy
Core Design Contradiction:
ReliabilityVSManufacturing precision

Solution Approach 1:

The patent establishes a specific thickness range for the organic coating layer (70-480 nm) that balances barrier properties and color accuracy. Within this range, the layer provides sufficient protection while limiting swelling-induced color shifts. The upper limit of 480 nm is specifically set to prevent excessive swelling that would degrade color accuracy.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent applies different material properties to different layers: the inorganic oxide layers provide dense barrier properties for moisture and oxygen blocking, while the organic coating layers provide controlled optical properties and additional protection. This local differentiation of material qualities optimizes both barrier performance and color stability.

Inventive Principle:
Principle #3Local quality

3Device complexity

If a simple single-layer barrier film is used, then device complexity is reduced, but color stability deteriorates due to insufficient control of spectral transmission

Engineering Contradiction:
Improvebarrier film structureVSAvoidspectral transmission characteristics
Core Design Contradiction:
Device complexityVSStability of the object's composition

Solution Approach 1:

The patent segments the barrier film into multiple functional layers: light-transmitting base material, inorganic oxide layer A, organic coating layer B, inorganic oxide layer C, and organic coating layer D. Each layer serves a specific function (structural support, barrier protection, optical control), and their combined effect stabilizes spectral transmission characteristics while maintaining manageable device complexity.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The patent employs a composite multi-layer structure combining different materials (PET base material, Al2O3/SiO2/TiO2 inorganic oxide layers, polyvinyl alcohol organic coating layers) with complementary properties. This composite structure provides both the barrier functionality and the optical control needed for color stability, overcoming the limitations of simple single-layer films.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The barrier film effectively suppresses color changes in liquid crystal display devices, ensuring consistent color purity and quality over time by stabilizing the spectral transmission characteristics.

Implementation Method 1

it is preferable to protect the surfaces of both sides of a quantum dot-containing layer with a barrier film

Methodology Applied
Scientific EffectBarrier film protection:

Implementation Method 2

an organic coating layer of the barrier film swells to change the waveform of the spectral transmission spectrum of the barrier film

Methodology Applied
Scientific EffectSwelling:

Implementation Method 3

The particle size of the quantum dot is smaller than the Bohr radius of an exciton of the compound semiconductor, and thus the quantum confinement effect appears

Methodology Applied
Scientific EffectQuantum confinement effect:

Implementation Method 4

a reflectance at an interface between the inorganic oxide layer A and the organic coating layer B is larger than a reflectance at an interface between the light-transmitting base material and the inorganic oxide layer A

Methodology Applied
Scientific EffectOptical interference: Interference

Data Source

PatentEP4202506B1Barrier film, wavelength conversion sheet using same, backlight and liquid crystal display device
Publication Date: 2025.11.26 DAI NIPPON PRINTING CO LTD
  • EP4202506B1 patent drawingFigure 1~2
  • EP4202506B1 patent drawingFigure 3
  • EP4202506B1 patent drawingFigure 4

AI summary

Provided is a barrier film that can suppress a change in color when applied to a wavelength conversion sheet. A barrier film for a wavelength conversion sheet, comprising an inorganic oxide layer A, an organic coating layer B, an inorganic oxide layer C, and an organic coating layer D in presented order on a light-transmitting base material; wherein refractive indexes of the inorganic oxide layer A, the organic coating layer B, the inorganic oxide layer C, and the organic coating layer D are defined as nA, nB, nc, and nD, respectively; thicknesses of the organic coating layer B and the organic coating layer D are defined as tB and tD, respectively; nA and nc are larger than nB and nD; and d1 represented by the following expression 1 represents a range of x ± 0.10 wherein x is an integer of 2 to 13. d1 = nB × tB/112.5 nm + nD × tD/112.5 nm (Expression 1)