Battery Cell Stack Corrosion Resistance via Cushion Member

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Solution Overview

Problem

In redox flow batteries, the electrical resistance between the current collector plate and the end bipolar plate increases due to repeated charging and discharging, degrading battery performance, primarily caused by electrolytic corrosion from water entry during pressure changes.

Innovation Solution

The battery cell stack design includes materials for the current collector plate and end bipolar plate with a corrosion potential difference of 0.35 V or less, and optionally a deformable cushion member, to prevent electrolytic corrosion and maintain low electrical resistance.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If a current collector plate and end bipolar plate are used in a battery cell stack, then electrical connection is established for current collection, but electrical resistance increases due to electrolytic corrosion from water entry during pressure changes

Engineering Contradiction:
Improveelectrical connection stabilityVSAvoidelectrolytic corrosion
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

A cushion member is introduced as an intermediary component between the current collector plate and the end bipolar plate. This cushion member serves multiple functions: it maintains electrical connection stability, prevents direct contact that would lead to electrolytic corrosion, and accommodates pressure changes during battery operation. The cushion member acts as a mediator that resolves the contradiction between establishing electrical connection and preventing corrosion.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The cushion member is designed as a sacrificial component that can be easily replaced. It is positioned to absorb the harmful effects of pressure changes and potential corrosion, protecting the more valuable current collector plate and end bipolar plate. This approach follows the principle of using a less critical component to protect critical components.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

2Duration of action of moving object

If pressure changes occur during charging and discharging cycles, then battery operation is enabled, but water enters the battery cell stack causing increased electrical resistance

Engineering Contradiction:
Improvecharging and discharging cyclesVSAvoidwater entry
Core Design Contradiction:
Duration of action of moving objectVSObject-affected harmful factors

Solution Approach 1:

The cushion member is pre-installed between the current collector plate and the end bipolar plate to provide protective cushioning before water entry or corrosion can occur. This pre-positioned cushioning element anticipates pressure changes and potential water intrusion, maintaining separation and preventing direct contact between metallic components that would lead to corrosion during charging and discharging cycles.

Inventive Principle:
Principle #11Beforehand cushioning (Prior cushioning)

3Reliability

If materials with different corrosion potentials are used for current collector plate and end bipolar plate, then electrical connection is established, but galvanic corrosion occurs increasing electrical resistance

Engineering Contradiction:
Improveelectrical connectionVSAvoidgalvanic corrosion
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

The cushion member serves as an intermediary barrier between the current collector plate and the end bipolar plate, which are made of materials with different corrosion potentials. By preventing direct contact between these dissimilar metals, the cushion member eliminates the galvanic couple that would otherwise cause galvanic corrosion, while still maintaining the necessary electrical connection for current collection.

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This configuration effectively suppresses the increase in electrical resistance between the current collector plate and the end bipolar plate, ensuring stable battery performance even with repeated charging and discharging cycles.

Implementation Method 1

a cushion layer (cushion member) which is deformable in the thickness direction is provided between a current collector plate and an end bipolar plate

Methodology Applied
Scientific EffectElastic deformation: Elasticity

Implementation Method 2

two members in contact with each other between the current collector plate and the end bipolar plate are made of materials such that, when an accelerated test satisfying the following conditions 1 to 3 is performed, the electrical resistance value between the current collector plate and the end bipolar plate after the accelerated test is 1.05 times or less the electrical resistance value between the current collector plate and the end bipolar plate before the accelerated test

Methodology Applied
Scientific EffectElectrolytic corrosion: Electrolysis

Data Source

PatentEP3046173B1Battery cell stack and redox flow battery
Publication Date: 2022.09.21 SUMITOMO ELECTRIC INDUSTRIES LTD
  • EP3046173B1 patent drawingFigure 1
  • EP3046173B1 patent drawingFigure 2
  • EP3046173B1 patent drawingFigure 3

AI summary

Provided is a battery cell stack in which the electrical resistance between a current collector plate and an end bipolar plate is unlikely to increase when charging and discharging are repeated. A battery cell stack includes a current collector plate electrically connected to each of a pair of end bipolar plates located at both ends in the stacking direction. In the battery cell stack, two members in contact with each other between the current collector plate and the end bipolar plate are made of materials such that, when an accelerated test satisfying the following conditions 1 to 3 is performed, the electrical resistance value between the current collector plate and the end bipolar plate after the accelerated test is 1.05 times or less the electrical resistance value between the current collector plate and the end bipolar plate before the accelerated test: Condition 1 is that a cycle includes applying pressure over one minute to achieve a predetermined pressure, maintaining the predetermined pressure for one minute, and bringing the predetermined pressure back to the atmospheric pressure over one minute; Condition 2 is that the predetermined pressure is set to be the atmospheric pressure + 0.1 MPa; and Condition 3 is that the number of cycles is set to 18.