Battery Powder Leaching Sequence for Cobalt Nickel Recovery

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Solution Overview

Problem

Existing methods for leaching metals from lithium ion battery waste face challenges in achieving sufficient leaching of cobalt and nickel while preventing the dissolution of copper, which complicates the separation and recovery processes.

Innovation Solution

A method involving multiple leaching steps, where the first leaching step terminates before copper dissolution, and the second leaching step continues until copper is dissolved, allowing for the efficient leaching of cobalt and nickel while separating copper.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If the leaching time is extended to improve the leaching rate of cobalt and nickel, then the leaching rate of cobalt and nickel is improved, but copper begins to be dissolved which complicates separation and removal

Engineering Contradiction:
Improveleaching rate of cobalt and nickelVSAvoidcopper dissolution
Core Design Contradiction:
ProductivityVSObject-generated harmful factors

Solution Approach 1:

The patent divides the leaching process into multiple sequential leaching steps with different termination conditions. In the first leaching step, leaching is terminated before copper dissolution begins, while in subsequent steps, leaching continues after copper dissolution starts. This segmentation allows selective leaching of cobalt and nickel in early steps while permitting copper dissolution in later steps, resolving the contradiction between improving leaching rate and preventing harmful copper dissolution.

Inventive Principle:
Principle #1Segmentation

2Ease of operation

If the leaching is terminated before copper begins to be dissolved to enable easy copper removal, then copper can be easily separated by solid-liquid separation, but the leaching rate of cobalt and nickel is insufficient

Engineering Contradiction:
Improvecopper separation easeVSAvoidleaching rate of cobalt and nickel
Core Design Contradiction:
Ease of operationVSProductivity

Solution Approach 1:

The patent applies preliminary action by conducting initial leaching steps that terminate before copper dissolution, thereby preparing a leached solution with high cobalt and nickel content but minimal copper contamination. This preliminary leaching establishes a foundation for easy copper separation. Subsequent leaching steps then continue after copper dissolution begins to further improve cobalt and nickel extraction, while the copper can still be removed through solid-liquid separation of the resulting leached residue.

Inventive Principle:
Principle #10Preliminary action

3Productivity

If multiple leaching steps are implemented to improve cobalt and nickel leaching, then the leaching rate of cobalt and nickel is improved, but the process complexity increases

Engineering Contradiction:
Improveleaching rate of cobalt and nickelVSAvoidleaching process complexity
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The patent employs parameter changes by varying the termination conditions of different leaching steps rather than changing physical equipment or adding complex apparatus. The first leaching step terminates before copper dissolution (ORP < 0 mV), while subsequent steps terminate after copper dissolution begins (ORP ≥ 0 mV). This simple parameter change in termination timing allows multiple leaching steps to be implemented without significantly increasing process complexity, as the same leaching equipment and reagents are used throughout.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach improves the leaching rate of cobalt and nickel while facilitating the easy removal of copper, thereby enhancing the efficiency and cost-effectiveness of the metal recovery process.

Implementation Method 1

battery powder is brought into contact with an acidic leaching solution to dissolve in the acidic leaching solution metals such as nickel, cobalt, manganese, aluminum and iron

Methodology Applied
Scientific EffectDissolution: Solvation

Implementation Method 2

the copper can be in a solid state at the end of the leaching, and this can lead to easy separation and removal of the solid copper from the leaching solution

Methodology Applied
Scientific EffectSolid-liquid separation: Sedimentation

Data Source

PatentEP4278020B1Method for leaching metal and method for recovering metal
Publication Date: 2025.01.22 JX METALS CIRCULAR SOLUTIONS CO LTD
  • EP4278020B1 patent drawingFigure 1~2
  • EP4278020B1 patent drawingFigure 3
  • EP4278020B1 patent drawingFigure 4

AI summary

A method for leaching at least one metal in battery powder containing at least copper and one or more of cobalt and nickel, the method including a leaching process repeating multiple times, wherein the leaching process includes: a first leaching step of leaching at least one metal in the battery powder in an acidic leaching solution, terminating the leaching before the copper begins to be dissolved, and removing a leached residue from the resulting leached solution; and a second leaching step of leaching at least one metal in the leached residue of the first leaching step in an acidic leaching solution, and terminating the leaching after the copper begins to be dissolved to obtain a leached solution, wherein the leached solution obtained in the second leaching step of the leaching process is used as an acidic leaching solution in a first leaching step of a leaching process followed by said leaching process, and wherein a leached residue is removed from a leached solution in a second leaching step of at least one leaching process.