Battery Separator Adhesive Layer Balancing Antistatic and Electrode Adhesion

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Solution Overview

Problem

Conventional separators with a polyvinylidene fluoride (PVDF) layer face challenges in maintaining adhesiveness to electrodes due to static electricity issues, which are exacerbated by the use of surfactants intended to prevent static, leading to decreased handleability and battery performance.

Innovation Solution

A separator for non-aqueous secondary batteries featuring a porous substrate with an adhesive layer containing a polyvinylidene fluoride type resin and lithium imide salt, which prevents static electricity while maintaining adhesiveness, using lithium bis(trifluoromethanesulfonyl)imide or lithium bis(pentafluoroethanesulfonyl)imide, and optionally a heat-resistant layer with an inorganic filler.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of operation

If a PVDF layer is provided on the separator to prevent static electricity, then handleability is enhanced, but adhesiveness to electrode is lowered

Engineering Contradiction:
ImprovehandleabilityVSAvoidadhesiveness to electrode
Core Design Contradiction:
Ease of operationVSStrength

Solution Approach 1:

The invention applies different functional properties to different regions of the separator structure. The PVDF layer is localized on the outer surface to provide antistatic properties, while the inner surface maintains high adhesiveness for electrode bonding. This spatial differentiation of properties allows the separator to simultaneously achieve good handleability and strong electrode adhesion without compromise.

Inventive Principle:
Principle #3Local quality

2Object-affected harmful factors

If a surfactant is used to reduce static electricity, then electrostatic propensity is reduced, but adhesiveness between adhesive layer and electrode is lowered

Engineering Contradiction:
Improveelectrostatic propensityVSAvoidadhesiveness between adhesive layer and electrode
Core Design Contradiction:
Object-affected harmful factorsVSStrength

Solution Approach 1:

The invention extracts and removes the harmful surfactant component from the separator system entirely. Instead of using surfactants to manage static electricity, the patent employs an alternative approach by controlling the PVDF layer composition and structure, thereby eliminating the need for surfactants and preserving the adhesive layer's bonding capability to the electrode.

Inventive Principle:
Principle #2Taking out (Extraction)

3Ease of operation

If a layer containing PVDF is provided on the separator to prevent static electricity, then handleability is enhanced, but conveyance performance and yield decrease due to adsorption of foreign substances

Engineering Contradiction:
ImprovehandleabilityVSAvoidconveyance performance and yield
Core Design Contradiction:
Ease of operationVSProductivity

Solution Approach 1:

The PVDF layer is strategically positioned and controlled in thickness to provide antistatic properties only where needed on the separator surface, while maintaining sufficient porosity and appropriate composition to prevent excessive foreign substance adsorption. This localized application with controlled properties balances handleability improvement with maintenance of conveyance performance and manufacturing yield.

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution enhances adhesiveness to electrodes, prevents static electricity, and improves battery characteristics by balancing antistatic performance with adhesive strength, resulting in improved handleability and battery performance.

Implementation Method 1

PVDF has a property of being susceptible to static electricity... the separator contains a lithium imide salt

Methodology Applied
Scientific EffectElectrostatic prevention: Electrostatics

Implementation Method 2

an adhesive layer that is provided on at least one side of the porous substrate and that contains a polyvinylidene fluoride type resin... adhesiveness between an electrode and a separator

Methodology Applied
Scientific EffectAdhesive bonding: Adhesive

Data Source

PatentUS20250219247A1Separator for non-aqueous secondary battery and non-aqueous secondary battery
Publication Date: 2025.07.03 TEIJIN LTD

AI summary

An embodiment of the present invention provides a separator for a non-aqueous secondary battery, including a porous substrate; and an adhesive layer that is provided on at least one side of the porous substrate and that contains a polyvinylidene fluoride type resin, in which the separator contains a lithium imide salt.