High Density Battery Separator Optimizing Ion Permeability

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Solution Overview

Problem

Existing batteries face deterioration in capacity due to repeated charging and discharging, particularly when the area density of the positive electrode active material layer exceeds a certain threshold, leading to decreased energy density and cycle lifespan.

Innovation Solution

A battery design incorporating a positive electrode with a lithium cobalt composite oxide, a porous separator with specific structural parameters, and a gel electrolyte, where the area density of the positive electrode active material layer is maintained at 27 mg/cm² or greater, and the separator's film resistance, thickness, porosity, and tortuosity are optimized to mitigate over-voltage and enhance ion permeability.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If the area density of the positive electrode active material layer is increased to improve energy density, then the battery capacity deteriorates due to repeated charging and discharging

Engineering Contradiction:
Improvearea density of positive electrode active material layerVSAvoidcycle characteristics
Core Design Contradiction:
Quantity of substanceVSReliability

Solution Approach 1:

The patent applies parameter changes by precisely controlling the area density of the positive electrode active material layer to be 27 mg/cm² or more, while simultaneously optimizing separator parameters (film resistance, thickness, porosity, tortuosity) to resolve the contradiction between high energy density and good cycle characteristics

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses a porous separator with specifically controlled porosity (30-80%) and pore size (0.03-1 μm) to improve ion permeability while maintaining structural integrity during repeated charging and discharging, thereby preventing capacity deterioration despite high area density

Inventive Principle:
Principle #31Porous materials

2Quantity of substance

If the area density of the positive electrode active material layer is increased, then energy density is improved, but over-voltage occurs leading to electrolyte solution decomposition

Engineering Contradiction:
Improvearea density of positive electrode active material layerVSAvoidover-voltage and electrolyte solution decomposition
Core Design Contradiction:
Quantity of substanceVSObject-generated harmful factors

Solution Approach 1:

The patent introduces the separator as an intermediary component between the positive electrode and negative electrode, with optimized film resistance (0.01-10 μm) and porosity parameters that mediate ion transport to prevent over-voltage and electrolyte solution decomposition while maintaining high area density

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent changes the physical parameters of the separator (film resistance, thickness, porosity, tortuosity) to create optimal ion transport conditions that prevent over-voltage generation, allowing the battery to operate with high area density without electrolyte decomposition

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This configuration improves the cycle characteristics by maintaining energy density and reducing capacity deterioration, while preventing electrolyte solution decomposition and clogging, thus extending the battery's lifespan.

Implementation Method 1

the separator's film resistance, thickness, porosity, and tortuosity are optimized to mitigate over-voltage and enhance ion permeability

Methodology Applied
Scientific EffectIon permeability: Permeation

Implementation Method 2

application of an electrolyte solution as an electrolyte and a matrix polymer compound that retains the electrolyte solution has been performed for the sake of liquid leakage resistance

Methodology Applied
Scientific EffectGel electrolyte: Gel

Data Source

PatentEP3059793B1Battery, battery pack, electronic device, electric vehicle and electric storage device
Publication Date: 2019.10.02 MURATA MFG CO LTD
  • EP3059793B1 patent drawingFigure 1
  • EP3059793B1 patent drawingFigure 2
  • EP3059793B1 patent drawingFigure 3A~3B

AI summary

Provided is a battery in which an area density S (mg/cm2) of a positive electrode active material layer is 27 mg/cm2 or greater, and a porous film included in a separator has a structure satisfying the following Expressions.