BCC Alloy Hydrogen Separation Membrane for High-Temperature Durability

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Solution Overview

Problem

Current hydrogen separation membranes face challenges with high unit costs and low permeability, as well as durability issues due to hydrogen embrittlement and crystallization at high temperatures, limiting their commercialization and effectiveness.

Innovation Solution

A separation membrane with a body-centered cubic (BCC) crystal structure alloy comprising Group 5 elements like V, Nb, or Ta, combined with Iridium (Ir) and optionally additional metals like Zr, Cu, Y, Ni, or Al, which reduces hydrogen solubility and embrittlement, and includes a catalyst layer for enhanced hydrogen permeability and stability.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If Pd-based metals are used for hydrogen separation membranes, then hydrogen selectivity is improved, but unit cost increases and permeability decreases

Engineering Contradiction:
Improvehydrogen selectivityVSAvoidunit cost
Core Design Contradiction:
ReliabilityVSEase of manufacture

Solution Approach 1:

The patent changes the crystal structure parameter from FCC to BCC and modifies alloy composition by adding Group 5 elements and Ir, achieving high hydrogen permeability and selectivity with lower cost materials

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates composite alloy materials combining Group 5 elements (V, Nb, Ta) with Ir and other metals to achieve superior hydrogen separation performance that balances selectivity, permeability, and cost

Inventive Principle:
Principle #40Composite materials

2Ease of manufacture

If amorphous metal separation membranes are used, then manufacturing process is simplified, but durability decreases due to crystallization at high temperatures

Engineering Contradiction:
Improvemanufacturing processVSAvoiddurability
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent changes the crystal structure from amorphous to BCC, providing thermal stability and preventing crystallization at high operating temperatures while maintaining manufacturing feasibility through controlled alloy composition

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent develops BCC alloy membranes that are more stable and durable than amorphous membranes, reducing the need for frequent replacement despite potentially higher initial manufacturing complexity

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

3Ease of manufacture

If porous separation membranes are used, then manufacturing is easier, but gas selectivity decreases due to difficulty in controlling pore size and shape

Engineering Contradiction:
ImprovemanufacturingVSAvoidgas selectivity
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent transitions from porous structures to non-porous BCC alloy materials, achieving high gas selectivity through the inherent properties of the crystalline structure rather than relying on pore geometry control

Inventive Principle:
Principle #31Porous materials

Solution Approach 2:

The patent uses the interstitial sites within the BCC lattice structure to selectively separate hydrogen based on atomic size and diffusion properties, replacing pore-based separation mechanisms

Inventive Principle:
Principle #29Pneumatics and hydraulics

4Productivity

If membranes are used at high temperatures (250-500°C), then hydrogen permeability is improved, but durability decreases due to hydrogen embrittlement and crystallization

Engineering Contradiction:
Improvehydrogen permeabilityVSAvoiddurability
Core Design Contradiction:
ProductivityVSReliability

Solution Approach 1:

The patent changes the crystal structure to BCC and optimizes alloy composition to simultaneously achieve high hydrogen permeability at elevated temperatures while maintaining structural stability and resistance to hydrogen embrittlement

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent converts the potential harm of high-temperature operation into benefit by selecting BCC alloy materials that become more stable and selective at elevated temperatures, turning thermal stress into enhanced performance

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The membrane achieves high hydrogen permeability and improved durability, maintaining performance at high temperatures while inhibiting hydrogen embrittlement and crystallization, thus offering a cost-effective and efficient hydrogen separation solution.

Implementation Method 1

Hydrogen can be selectively separated by hydrogen dissolution and diffusion into the interstitial sites of the FCC lattice of Pd

Methodology Applied
Scientific EffectHydrogen dissolution: Absorption (physical)

Implementation Method 2

Hydrogen can be selectively separated by hydrogen dissolution and diffusion into the interstitial sites of the FCC lattice of Pd

Methodology Applied
Scientific EffectDiffusion: Diffusion

Implementation Method 3

A hydrogen separation membrane including the separation membrane, and a catalyst layer on the separation membrane

Methodology Applied
Scientific EffectCatalysis: Catalysis

Data Source

PatentEP2596851B1Separation membrane, and apparatus including the separation membrane
Publication Date: 2017.08.16 SAMSUNG ELECTRONICS CO LTD
  • EP2596851B1 patent drawingFigure 1A~1B
  • EP2596851B1 patent drawingFigure 2
  • EP2596851B1 patent drawingFigure 3

AI summary

Disclosed is a separation membrane including an alloy including a Group 5 element and Ir, wherein the alloy includes a body centered cubic crystal structure.