Bi-2212 Superconductor Coil Heat Treatment with Ceramic-Glass Insulation

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

The manufacture of high temperature superconducting Bi-2212 coils is hindered by defects caused by trapped CO2 and other contaminants during the heat-treatment process, leading to incomplete phase formation and reduced current carrying capacity, as existing insulation materials melt at the required reaction temperatures and fail to purge gases effectively from the tightly wound coil.

Innovation Solution

A ceramic-glass yarn insulation is used with a carbonaceous binder that is burned at a lower temperature than the Bi-2212 partial melting point, followed by evacuation and back-filling with pure oxygen to remove contaminants, ensuring a controlled atmosphere for optimal Bi-2212 phase formation.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If glass braid insulation is used for Nb3Sn coils, then electrical insulation is provided, but the glass fully melts at the reaction temperatures needed for Bi-2212 coils

Engineering Contradiction:
Improveelectrical insulation stabilityVSAvoidreaction temperature tolerance
Core Design Contradiction:
ReliabilityVSTemperature

Solution Approach 1:

The patent uses a composite insulation structure consisting of a ceramic core (alumina or silica) surrounded by a glass coating. The ceramic component provides high-temperature stability to withstand Bi-2212 reaction temperatures (800-900°C), while the glass layer provides electrical insulation properties. This composite approach allows the insulation to maintain both electrical functionality and structural integrity at high temperatures where pure glass would melt.

Inventive Principle:
Principle #40Composite materials

2Reliability

If continuous oxygen gas flow is used during heat treatment, then oxidation control is improved, but trapped CO2 gas cannot be purged from the tight winding pack

Engineering Contradiction:
Improvephase formation qualityVSAvoidtrapped contaminant gas
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

The patent implements a periodic heat treatment cycle with distinct phases: first, a binder burn-off stage in air or oxygen atmosphere to combust the organic binder; second, a vacuum evacuation stage to remove generated CO2 and other gases from the winding pack; third, a Bi-2212 formation stage in controlled oxygen atmosphere. This periodic alternation between gas introduction and evacuation ensures contaminant removal while maintaining proper atmosphere for phase formation.

Inventive Principle:
Principle #19Periodic action

Solution Approach 2:

The patent performs binder burn-off as a preliminary action before the main Bi-2212 formation reaction. By removing the organic binder first and evacuating the resulting gases, the patent prevents contaminant formation during the subsequent critical phase formation stage, ensuring pure oxygen atmosphere when the superconducting phase develops.

Inventive Principle:
Principle #10Preliminary action

3Productivity

If the coil is tightly wound to maximize current density, then space utilization is improved, but gas evacuation through small orifices becomes extremely difficult

Engineering Contradiction:
Improvecurrent densityVSAvoidgas evacuation difficulty
Core Design Contradiction:
ProductivityVSEase of manufacture

Solution Approach 1:

The patent incorporates deliberate gaps and ventilation channels in the coil winding structure, segmenting the otherwise continuous dense packing. These segmented pathways allow gas to escape from the interior of the winding pack during vacuum evacuation, while the overall tight winding maintains high current density. The segmentation creates escape routes without significantly reducing the active superconducting material volume.

Inventive Principle:
Principle #1Segmentation

4Ease of operation

If carbonaceous binder is used in ceramic-glass yarn, then flexibility and handling are improved, but CO2 and other contaminants are produced during burn-off

Engineering Contradiction:
Improveyarn flexibilityVSAvoidcombustion contaminants
Core Design Contradiction:
Ease of operationVSObject-generated harmful factors

Solution Approach 1:

The patent accepts the harmful CO2 production from binder combustion but converts this harmful process into a beneficial one by implementing controlled vacuum evacuation. The same tight winding that traps harmful gases also creates a sealed environment where vacuum evacuation can effectively remove all contaminants. The binder combustion is performed in a controlled manner with subsequent vacuum treatment, transforming the harmful contaminant generation into a controlled purging process that ensures clean atmosphere for phase formation.

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This process allows for the production of high current Bi-2212 coils by ensuring a clean oxygen-rich environment, significantly improving the critical current density and reducing defects, with the binder burn-off temperature optimized between 250°C-850°C for effective gas removal and phase formation.

Implementation Method 1

The carbonaceous binder in the yarn is completely burned at a temperature lower than Bi-2212 partial melting point. This produces a byproduct of CO2 and other contaminants

Methodology Applied
Scientific EffectCombustion: Combustion

Implementation Method 2

After cooling the vessel to or approximately to room temperature, the CO2 and other contaminate gases are removed by evacuating the heat-treatment chamber containing the coil

Methodology Applied
Scientific EffectVacuum evacuation: Vacuum

Implementation Method 3

After evacuation, the chamber is back-filled with pure oxygen gas or a desired mixture of gases. In this way all the contaminant gases are removed from the winding pack through the small orifices and completely replaced with the desired gas

Methodology Applied
Scientific EffectGas back-filling:

Implementation Method 4

The atmosphere adjacent to the wire surface is critical to the formation of the optimal phase of Bi-2212

Methodology Applied
Scientific EffectPhase formation through heat treatment: Heat Treatment

Data Source

PatentEP2308061B8Manufacture of high temperature superconductor coils
Publication Date: 2018.03.21 BRUKER OST LLC

AI summary

A method for successfully heat treating magnet coils of braided Bi2Sr2Ca1Cu2Ox (Bi-2212) strand. The Bi-2212 coil is fabricated using standard round wire powder-in- tube techniques, and braided with a ceramic-glass braid with integrated carbonaceous binder. The coil is heated in an atmosphere controlled furnace below the high current density phase reaction sequence to burn off the carbonaceous binder and evacuated to remove unwanted gases from the inner windings. The oxygen environment is then reintroduced and the coil is heat treated to the high Jc reaction temperature and then processed as normal. As the local atmosphere around the surface of the wire, particularly the concentration of oxygen, is critical to a successful reaction sequence, high current Bi-2212 coils can thereby be obtained.