Bimodal LiFePO4 Cathode Material for Energy Density and Cold Performance

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Solution Overview

Problem

Existing rechargeable lithium batteries face challenges in achieving high capacity, improved low-temperature characteristics, and long lifespan while maintaining high energy density.

Innovation Solution

A positive electrode active material composed of first and second particles, where the first particle is a polycrystalline olivine-based lithium iron phosphate with a larger average diameter, and the second particle is a smaller nano-sized particle, both with specific chemical compositions and prepared through distinct methods, are mixed to enhance performance.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If only large particles are used in the positive electrode active material, then energy density is improved, but low-temperature characteristics and capacity deteriorate

Engineering Contradiction:
Improveenergy densityVSAvoidlow-temperature characteristics
Core Design Contradiction:
Quantity of substanceVSReliability

Solution Approach 1:

The positive electrode active material is segmented into two distinct particle size ranges: large particles (3 μm to 10 μm) for energy density and small particles (0.1 μm to 2 μm) for low-temperature performance. This segmentation allows each particle size to fulfill its specific functional role without compromising the other.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

Different regions of the electrode are assigned different particle sizes based on their functional requirements. Large particles dominate the bulk structure for high energy density, while small particles are distributed throughout to ensure good low-temperature characteristics and capacity.

Inventive Principle:
Principle #3Local quality

2Reliability

If only small particles are used in the positive electrode active material, then low-temperature characteristics and capacity are improved, but energy density deteriorates

Engineering Contradiction:
Improvelow-temperature characteristicsVSAvoidenergy density
Core Design Contradiction:
ReliabilityVSQuantity of substance

Solution Approach 1:

The positive electrode active material is segmented into two distinct particle size ranges: large particles (3 μm to 10 μm) for energy density and small particles (0.1 μm to 2 μm) for low-temperature performance. This segmentation allows each particle size to fulfill its specific functional role without compromising the other.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

Different regions of the electrode are assigned different particle sizes based on their functional requirements. Large particles dominate the bulk structure for high energy density, while small particles are distributed throughout to ensure good low-temperature characteristics and capacity.

Inventive Principle:
Principle #3Local quality

3Quantity of substance

If only large particles are used in the positive electrode active material, then energy density is improved, but capacity and lifespan deteriorate

Engineering Contradiction:
Improveenergy densityVSAvoidcapacity
Core Design Contradiction:
Quantity of substanceVSProductivity

Solution Approach 1:

The positive electrode active material is segmented into two distinct particle size ranges: large particles (3 μm to 10 μm) for energy density and small particles (0.1 μm to 2 μm) for low-temperature performance. This segmentation allows each particle size to fulfill its specific functional role without compromising the other.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

Different regions of the electrode are assigned different particle sizes based on their functional requirements. Large particles dominate the bulk structure for high energy density, while small particles are distributed throughout to ensure good low-temperature characteristics and capacity.

Inventive Principle:
Principle #3Local quality

4Reliability

If a bimodal particle size distribution is implemented, then low-temperature characteristics and capacity are improved, but device complexity increases

Engineering Contradiction:
Improvelow-temperature characteristicsVSAvoidparticle size distribution control
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The positive electrode active material is segmented into two distinct particle size ranges: large particles (3 μm to 10 μm) for energy density and small particles (0.1 μm to 2 μm) for low-temperature performance. This segmentation allows each particle size to fulfill its specific functional role without compromising the other.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The particle size parameter is changed to create a bimodal distribution with specific ranges: large particles (3 μm to 10 μm) and small particles (0.1 μm to 2 μm). This parameter optimization achieves the desired performance balance while maintaining manufacturability.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The resulting battery exhibits high capacity, improved low-temperature characteristics, and extended lifespan with enhanced energy density.

Implementation Method 1

Electrical energy is produced (generate) through oxidation and reduction reactions as the lithium ions are intercalated and deintercalated into/from the positive electrode and the negative electrode.

Methodology Applied
Scientific EffectOxidation and reduction reactions: Redox Reactions

Data Source

PatentEP4651232A1Positive electrode active material for rechargeable lithium battery, preparation method of the same, and rechargeable lithium battery including the same
Publication Date: 2025.11.19 SAMSUNG SDI CO LTD
  • EP4651232A1 patent drawingFigure 1
  • EP4651232A1 patent drawingFigure 2
  • EP4651232A1 patent drawingFigure 3

AI summary

A positive electrode active material for a rechargeable lithium battery, a preparation method of the positive electrode active material, and a rechargeable lithium battery including the positive electrode active material are disclosed. The positive electrode active material includes a first particle containing a compound represented by Formula 1 and having a first average particle diameter and a second particle containing a compound represented by Formula 2 and having a second average particle diameter smaller than the first average particle diameter, wherein an amount of the first particle is equal to or greater than an amount of the second particle. A more detailed description of Formulae 1 and 2 is provided in the present disclosure.