Bio-based Elastomer Nanocomposite Silica Dispersion

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Solution Overview

Problem

Traditional rubber products face challenges with mechanical strength, wet-skid resistance, and rolling resistance due to poor silica dispersion, which is exacerbated by the use of silane coupling agents and VOC emissions in the manufacturing process.

Innovation Solution

The development of a bio-based elastomer nanocomposite using poly (itaconate-ter-isoprene-ter-glycidyl methacrylate) that improves silica dispersion through ester groups and epoxy functional groups, eliminating the need for silane coupling agents and reducing VOC emissions, thereby enhancing mechanical properties and wet-skid resistance while lowering rolling resistance.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If silane coupling agent is used to improve silica dispersion, then the dispersion effect of silica is improved, but the manufacturing cost increases and the process becomes more complex

Engineering Contradiction:
Improvesilica dispersion effectVSAvoidmanufacturing process complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The invention extracts and removes the silane coupling agent from the rubber compounding system, replacing it with a bio-based elastomer that has inherent silica dispersing capability through its molecular structure containing ester groups and hydroxyl groups that form hydrogen bonds with silica surface

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The invention changes the chemical parameters of the elastomer by introducing specific functional groups (ester groups and hydroxyl groups) that can interact with silica surface, thereby changing the interaction mechanism from requiring external coupling agents to inherent molecular-level dispersion

Inventive Principle:
Principle #35Parameter changes

2Manufacturing precision

If silane coupling agent is used to improve silica dispersion, then the dispersion effect of silica is improved, but the manufacturing cost increases

Engineering Contradiction:
Improvesilica dispersion effectVSAvoidmanufacturing cost
Core Design Contradiction:
Manufacturing precisionVSEase of manufacture

Solution Approach 1:

The invention extracts and removes the silane coupling agent from the rubber compounding system, replacing it with a bio-based elastomer that has inherent silica dispersing capability through its molecular structure containing ester groups and hydroxyl groups that form hydrogen bonds with silica surface

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The invention uses a cost-effective bio-based elastomer formulation that eliminates the need for expensive silane coupling agents, making the overall manufacturing process more economical despite the specialized polymer structure

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

3Strength

If traditional rubber processing is used, then the mechanical strength is improved, but the wet-skid resistance and rolling resistance are not optimized

Engineering Contradiction:
Improvemechanical strengthVSAvoidwet-skid resistance and rolling resistance
Core Design Contradiction:
StrengthVSObject-affected harmful factors

Solution Approach 1:

The invention creates a composite material system combining bio-based elastomer with silica filler, where the elastomer's molecular structure (containing ester groups and hydroxyl groups) forms hydrogen bonds with silica surface, achieving improved mechanical strength, wet-skid resistance, and rolling resistance through synergistic interaction

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution results in improved mechanical strength, wet-skid resistance, and reduced rolling resistance without the complexity and cost of silane coupling agents, while also eliminating VOC emissions, making it a promising 'green tire' material.

Implementation Method 1

ester groups form a hydrogen bond with silica surface to improve the dispersion effect of silica

Methodology Applied
Scientific EffectHydrogen bonding: Chemical Bonding

Implementation Method 2

Ring-opening crosslinking is occurred between epoxy functional group and '-OH' on silica surface, and it improves the dispersion effect of silica in elastomer and interfacial interaction between silica and rubber elastomer

Methodology Applied
Scientific EffectCrosslinking: Chemical Bonding

Data Source

PatentEP3323841B1White carbon black/poly(itaconate-isoprene-glycidyl methacrylate) bio-based elastomer composite material free of silane coupling agent, and preparation method therefor
Publication Date: 2020.04.22 BEIJING UNIV OF CHEM TECH
  • EP3323841B1 patent drawingFigure 1

AI summary

The present disclosure involves a preparation method of bio-based silica/poly (itaconate-ter-isoprene-ter-glycidyl methacrylate) nanocomposite. Bio-based silica/poly (itaconate-ter-isoprene-ter-glycidyl methacrylate) nanocomposite is environment-friendly, and silica and poly (itaconate-ter-isoprene-ter-glycidyl methacrylate) are derived from non-petroleum base materials, which do not rely on fossil fuel. Compared with nanocomposite without nanocomposite, nanocomposites with glycidyl methacrylate have better silica diffusion, mechanical properties and wet-skid resistance of rubber product are improved while consuming the same time. Further, rolling resistance is decreased so that using silane coupling agent is avoided. Therefore, the processing technology is simplified, and VOC emission is avoided. It is a kind of "green tire" rubber product.