Biodegradable Particulate Plugging Agents for Wellbore Flow Control

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Solution Overview

Problem

Current drilling and servicing fluids in the oil and gas industry face challenges with permanent and temporary particulate materials that either have residual effects on well production or fail to prevent sulfate-reducing bacteria (SRB) growth, leading to hydrogen sulfide production and equipment corrosion.

Innovation Solution

A servicing fluid comprising a base fluid and a solid particulate agent, which is a reaction product of a urea-containing compound and an aldehyde-containing compound, is introduced into subterranean formations to seal flow paths and degrade, forming biocidal compounds that prevent SRB growth and control fluid flow.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If permanent particulate materials (sand, clay, barite) are used to seal flow paths, then fluid flow control is achieved, but residual effects on well production occur

Engineering Contradiction:
Improvefluid flow controlVSAvoidresidual effects on production
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

The patent employs biodegradable polymer particles as temporary plugging agents that fulfill their flow control function and then naturally degrade, eliminating residual effects. These particles are designed to be biodegradable through hydrolysis or microbial action, allowing them to serve as disposable plugging materials that leave no harmful residue in the formation.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Solution Approach 2:

The patent changes the chemical composition and degradation characteristics of particulate materials from permanent (sand, clay) to temporary biodegradable polymers. By selecting polymers with specific degradation rates and mechanisms, the plugging effect is temporary and可控, allowing flow control during operations followed by natural degradation to restore formation permeability.

Inventive Principle:
Principle #35Parameter changes

2Reliability

If removable material (calcium carbonate) is used to modify flow, then fluid flow control is achieved, but cleanup solution injection is required to remove it

Engineering Contradiction:
Improvefluid flow controlVSAvoidcleanup requirement
Core Design Contradiction:
ReliabilityVSEase of operation

Solution Approach 1:

The patent uses biodegradable polymer particles that naturally degrade through hydrolysis or microbial action, eliminating the need for chemical cleanup operations. These temporary plugging agents decompose into harmless byproducts, providing flow control during operations without requiring subsequent acid injection or other removal procedures.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Solution Approach 2:

The biodegradable polymers perform self-removal through natural degradation processes. The particles automatically break down via hydrolysis or microbial metabolism, eliminating the need for external cleanup operations. This self-service mechanism simplifies operations by removing the requirement for separate acidizing or flushing steps.

Inventive Principle:
Principle #25Self-service

3Object-generated harmful factors

If temporary materials (biodegradable polymers) are used, then degradation occurs without residual effects, but temperature and cost limitations prohibit use in many applications

Engineering Contradiction:
Improveresidual effectsVSAvoidtemperature and cost limitations
Core Design Contradiction:
Object-generated harmful factorsVSAdaptability or versatility

Solution Approach 1:

The patent employs composite plugging systems combining biodegradable polymer particles with other compatible materials to enhance temperature stability and mechanical properties. These composite formulations maintain biodegradability while extending the operational temperature range and improving cost-effectiveness for diverse well conditions.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent modifies the chemical structure and physical properties of biodegradable polymers to withstand higher temperatures and more demanding well conditions. By adjusting polymer composition, molecular weight, and crosslinking density, the materials maintain their biodegradable nature while expanding their applicability to various temperature ranges and well environments.

Inventive Principle:
Principle #35Parameter changes

4Reliability

If sulfate sources and organic materials are present in well fluids, then SRB population growth occurs, but preventing their introduction is difficult

Engineering Contradiction:
ImproveSRB population controlVSAvoidcontamination prevention
Core Design Contradiction:
ReliabilityVSEase of operation

Solution Approach 1:

The patent converts the presence of organic materials from a harmful factor (SRB food source) into a beneficial mechanism by using biodegradable polymers that degrade into non-SRB-supporting byproducts. The degradation process consumes oxygen and creates an environment unfavorable for SRB growth, transforming potential contamination into a protective effect.

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Solution Approach 2:

The biodegradable polymer acts as an intermediary substance that mediates between the well fluids and SRB populations. During degradation, it consumes oxygen and produces byproducts that inhibit SRB growth, serving as a protective barrier against bacterial contamination without requiring direct intervention to prevent initial introduction.

Inventive Principle:
Principle #24Intermediary (Mediator)

5Object-generated harmful factors

If H2S is produced by SRB, then crude oil/natural gas value is reduced due to refining costs

Engineering Contradiction:
ImproveH2S productionVSAvoidrefining cost
Core Design Contradiction:
Object-generated harmful factorsVSLoss of energy

Solution Approach 1:

The patent applies preliminary protective action by introducing biodegradable polymers that prevent SRB growth before H2S can be produced. The polymers create an oxygen-depleting environment during degradation that inhibits SRB metabolism, preventing H2S generation upstream and eliminating the need for costly H2S removal and refining operations.

Inventive Principle:
Principle #9Preliminary anti-action

Solution Approach 2:

The patent converts the potential harmful effect of organic materials (SRB food source leading to H2S production) into a beneficial outcome by using biodegradable polymers that degrade into non-H2S-producing byproducts. The degradation process prevents SRB activity and H2S generation, transforming a potential contamination source into a protective mechanism.

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

6Object-generated harmful factors

If H2S reacts with steel, then equipment corrosion occurs, but prevention requires multiple additives

Engineering Contradiction:
Improveequipment corrosionVSAvoidadditive package
Core Design Contradiction:
Object-generated harmful factorsVSDevice complexity

Solution Approach 1:

The patent applies preliminary protection by preventing H2S generation at its source through biodegradable polymer degradation. By creating an oxygen-depleting environment that inhibits SRB growth, the system prevents H2S formation upstream, eliminating the need for downstream corrosion inhibitors and simplifying the additive package.

Inventive Principle:
Principle #9Preliminary anti-action

Solution Approach 2:

The patent converts the potential corrosion problem caused by H2S into a beneficial outcome by using biodegradable polymers that prevent H2S generation. The degradation process creates conditions unfavorable for SRB activity, thereby preventing both H2S production and subsequent corrosion without requiring complex corrosion inhibition systems.

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution effectively seals unwanted flow paths, degrades without residual effects, and produces biocidal compounds that inhibit SRB growth, reducing hydrogen sulfide production and equipment corrosion, thereby enhancing well production and safety.

Implementation Method 1

Particulate material has been employed to bridge/seal/plug certain flow paths in the formations where the flow of fluids is undesirable

Methodology Applied
Scientific EffectBridging:

Implementation Method 2

The different materials that have been used historically for these purposes can generally be classified as permanent, removable, or temporary. Examples of temporary materials are those that degrade, decompose, or have gradual solubility in the wellbore fluid.

Methodology Applied
Scientific EffectHydrolysis: Hydrolysis

Implementation Method 3

Biodegradable polymers, such as polylactic acid, are commonly used since they degrade in the presence of small amounts of water

Methodology Applied
Scientific EffectBiodegradation: Decomposition (biological)

Data Source

PatentUS10106720B2Methods and compositions for using temporary, slow degrading, particulate agents in a subterranean formation
Publication Date: 2018.10.23 MAGNABLEND

AI summary

Methods, fluids, and compositions are provided for treating subterranean formations. The fluids can be servicing or drilling fluids including a base fluid and a particulate agent or biocide precursor particulate agent. The particulate agent can seal flow paths in the subterranean formation and subsequently can be degraded to allow flow to resume. The particulate agent may be a reaction product of a urea containing compound and an aldehyde containing compound. An example of such a reaction product is a methylene urea.