Biogas Methane CO2 Separation via Amine Chemosorption

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Solution Overview

Problem

Existing methods for separating methane and carbon dioxide from biogas are energetically uneconomical and result in methane gas losses due to high pressure requirements and incomplete CO2 separation, with additional safety and cost burdens in column design.

Innovation Solution

A process utilizing an absorption column operating at normal pressure and temperature with a packing having a large surface area, using an amine solution for chemosorption, followed by desorption under elevated pressure and temperature to achieve complete CO2 separation and efficient methane purification.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Measurement precision

If pressure washing is used to separate CO2 from biogas, then CO2 separation is achieved, but energy consumption increases and methane losses occur

Engineering Contradiction:
ImproveCO2 separation completenessVSAvoidenergy consumption
Core Design Contradiction:
Measurement precisionVSLoss of energy

Solution Approach 1:

The invention changes the operating parameters from high pressure (10-30 bar) to atmospheric pressure, and from high temperature (40-60°C) to lower temperature (20-40°C). This parameter change eliminates the need for energy-intensive compression while maintaining effective CO2 separation through the use of amine-based washing solutions that work efficiently at these milder conditions.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention replaces the mechanical pressure-based separation system with a chemical absorption system using amine solutions. Instead of relying on high pressure to achieve separation, the system uses the chemical affinity of amines for CO2, substituting mechanical energy input with chemical reaction-based separation that occurs at atmospheric pressure.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

2Quantity of substance

If high pressure is applied in absorption columns, then CO2 binding is improved, but methane gas losses increase and safety requirements increase

Engineering Contradiction:
ImproveCO2 binding capacityVSAvoidmethane gas losses
Core Design Contradiction:
Quantity of substanceVSLoss of substance

Solution Approach 1:

The invention changes the pressure parameter from high (10-30 bar) to atmospheric pressure, eliminating methane losses associated with high-pressure operation. The CO2 binding capacity is maintained through the use of amine solutions that have high chemical affinity for CO2, allowing effective separation without requiring pressure elevation.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention substitutes the mechanical pressure-based CO2 binding mechanism with a chemical absorption mechanism using amine solutions. This replacement eliminates the need for high pressure, thereby preventing methane gas losses while maintaining effective CO2 removal through chemical reaction.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

3Measurement precision

If pressure washing is used, then CO2 separation is achieved, but additional safety measures and costs are required

Engineering Contradiction:
ImproveCO2 separationVSAvoidsafety requirements
Core Design Contradiction:
Measurement precisionVSDevice complexity

Solution Approach 1:

The invention changes the operating pressure from high (10-30 bar) to atmospheric pressure, which eliminates the need for complex high-pressure safety systems. The CO2 separation effectiveness is maintained through the use of amine-based washing solutions that provide efficient chemical absorption at atmospheric pressure, reducing device complexity and safety requirements.

Inventive Principle:
Principle #35Parameter changes

4Measurement precision

If biogas is compressed to high pressure for CO2 removal, then separation is achieved, but energy expenditure increases by 50%

Engineering Contradiction:
ImproveCO2 removal efficiencyVSAvoidenergy expenditure
Core Design Contradiction:
Measurement precisionVSUse of energy by moving object

Solution Approach 1:

The invention changes the pressure parameter from high (10-30 bar) to atmospheric pressure, eliminating the energy expenditure associated with gas compression. The CO2 removal efficiency is maintained through the use of amine solutions that provide effective chemical absorption at atmospheric pressure, reducing energy expenditure by approximately 50% compared to pressure washing methods.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention replaces the mechanical compression-based separation system with a chemical absorption system using amine solutions. This substitution eliminates the need for energy-intensive gas compression while maintaining effective CO2 removal, thereby reducing energy expenditure by approximately 50%.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This method achieves complete CO2 separation with minimal methane loss and significantly reduces energy expenditure by 50% compared to pressure washing, allowing for cost-effective and efficient production of high-purity biomethane for natural gas networks.

Implementation Method 1

using an amine solution for chemosorption

Methodology Applied
Scientific EffectChemosorption: Chemisorption

Implementation Method 2

followed by desorption under elevated pressure and temperature to achieve complete CO2 separation

Methodology Applied
Scientific EffectDesorption: Desorption

Data Source

PatentEP2066796B1Method and device for separating methane and carbon dioxide from biogas
Publication Date: 2011.06.29 MT -BIOMETHAN

AI summary

The invention relates to a method of separating methane and carbon dioxide from biogas and to a device for carrying out the method. These are intended for purifying biogas, wherein carbon dioxide is separated off from the biogas. Starting from the disadvantages of the known prior art, a method is intended to be provided which is distinguished by an energetically favourable mode of operation. For this the solution proposed is that the biogas is passed under atmospheric pressure and standard temperature into the absorption column, wherein while the biogas ascends through the packed bed, which preferably has a surface area of 600 to 1200 m2/m3 and at a space velocity of 5 to 40 Nm3/m3h, carbon dioxide present in the biogas is bound in the wash liquid by chemosorption. The purified methane gas is taken off at the top of the absorption column at a defined flow velocity. Carbon dioxide bound in the wash liquid is removed by desorption at a relatively high pressure of 2 to 30 bar and a temperature of at least 120°C. Biogas may be separated particularly economically into methane and CO2 by the suggested procedure.